Related papers: Doppler dual-comb coherent Raman spectromicroscopy
Dual-comb spectroscopy enables broadband, high-resolution measurements with microsecond temporal resolution, but extending this capability to the 10~12.5 $\mu$m molecular fingerprint region remains technically challenging, particularly for…
Frequency combs have revolutionized the field of optical spectroscopy, enabling researchers to probe molecular systems with a multitude of accurate and precise optical frequencies. While there have been tremendous strides in direct…
A new interferometric technique is demonstrated for measuring Coherent Anti-Stokes Raman Scattering (CARS) signals. Two forward-directed CARS signals are generated, one in each arm of an interferometer. The deterministic nature of the CARS…
We present the first experimental application of coherent Raman spectroscopy (CRS) on the ro-vibrational $\nu_2$ mode spectrum of methane (CH$_4$). Ultrabroadband femtosecond/picosecond (fs/ps) CRS is performed in the molecular fingerprint…
Quantum cascade laser (QCL) frequency combs are a promising candidate for chemical sensing and biomedical diagnostics, requiring only milliseconds of acquisition time to record absorption spectra without any moving parts. They are…
Optical frequency combs based on semiconductor lasers are a promising technology for monolithic integration of dual-comb spectrometers. However, the stabilization of the offset frequency fceo remains a challenging feat due the lack of…
We study the multiorder coherent Raman scattering of a quantum probe field in a far-off-resonance medium with a prepared coherence. Under the conditions of negligible dispersion and limited bandwidth, we derive a Bessel-function solution…
Removing distortions in coherent anti-Stokes Raman scattering (CARS) spectra due to interference with the nonresonant background (NRB) is vital for quantitative analysis. Popular computational approaches, the Kramers-Kronig relation and the…
Improvements to dual-comb interferometers will benefit precision spectroscopy and sensing, distance metrology, tomography, telecommunications etc. A specific requirement of such interferometers is to enforce mutual coherence between the two…
Due to its fast and high resolution characteristics, dual-comb spectroscopy has attracted an increasing amount of interest since its first demonstration. In the terahertz frequency range where abundant absorption lines (finger prints) of…
We exploit Surface-Enhanced Raman Scattering (SERS) to investigate aqueous droplets of genomic DNA deposited onto silver-coated silicon nanowires and we show that it is possible to efficiently discriminate between spectra of tumoral and…
Dissipative Kerr soliton microcombs have inspired various intriguing applications such as spectroscopy, ranging, telecommunication, and high purity microwave generation. Mechanically actuated soliton microcombs provide enhanced…
We present quasi-real-time dual-comb spectroscopy (DCS) using two Yb:fiber combs with ~750 MHz repetition rates. A computational coherent averaging technique is employed to correct timing and phase fluctuations of the measured dual-comb…
We propose a new Fourier-transform spectroscopy technique based on the rotational Doppler effect. The technique offers an application for optical vortex frequency combs, where each frequency component carries a unique amount of orbital…
Frequency combs are powerful tools for many applications and high performances are achieved by stabilizing these lasers. For operation in the mid-infrared, quantum cascade lasers (QCL) are ideal candidates as they present numerous…
We have carried out dual-comb spectroscopy and observed in a simultaneous acquisition a 140-THz-wide spectrum from 1.0 to 1.9 {\mu}m using two fiber-based frequency combs phase-locked to each other. This ultra-broad wavelength bandwidth is…
An experimental realization of high-precision direct frequency comb spectroscopy using counter-propagating femtosecond pulses on two-photon atomic transitions is presented. Doppler broadened background signal, hampering precision…
We demonstrate a single-beam, standoff (>10m) coherent anti-Stokes Raman scattering spectroscopy (CARS) of various materials, including trace amounts of explosives and nitrate samples, under ambient light conditions. The multiplex…
Frequency comb spectroscopy provides broadband access to molecular fingerprints with mode-defined spectral resolution. However, its deployment in non-cooperative gas sensing remains challenging because conventional implementations require…
The spectral resolution of broadband Fourier-transform coherent anti-Stokes Raman spectroscopy is limited by the maximum optical path length difference that can be scanned within a short time in an interferometer. However, alternatives to…