Related papers: Highly-efficient perturbative Raman shifting by en…
Many reports on stimulated Raman scattering in mixtures of Raman-active and noble gases indicate that the addition of a dispersive buffer gas increases the phase-mismatch to higher-order Stokes and antiStokes sidebands, resulting in…
Raman spectroscopy is a widely-used non-destructive material characterization method, which provides information about the vibrational modes of the material and therefore of its atomic structure and chemical composition. Interpretation of…
The inelastic scatterings of matter systems, such as Raman scattering, contain rich information on mechanical vibrations like as resonant frequencies, which lead to various applications, for example, a sensor for specific molecules.…
Bulk glass formation occurs over a very small part of phase space, and "good" glasses (which form even at low quench rates ~ 10K/sec) select an even smaller part of that accessible phase space. An axiomatic theory provides the physical…
This paper is devoted to the mathematical analysis of a time-domain electromagnetic scattering by periodic structures which are known as diffraction gratings. The scattering problem is reduced equivalently into an initial-boundary value…
We perform Raman spectroscopy of optically trapped non interacting \Rb atoms, and observe revivals of the atomic coherence at integer multiples of the trap period. The effect of coherence control methods such as echo and dynamical…
We investigate the spatial beam dynamics inside a multimode graded-index fiber under Raman amplification by adopting a semi-analytical variational approach. The variational analysis provides us with four coupled ordinary differential…
The conventional explanation of plasmon-enhanced Raman scattering attributes the enhancement to the antenna effect focusing the electromagnetic field into sub-wavelength volumes. Here we introduce a new model that additionally accounts for…
We have developed a novel multiscale computational scheme to describe coupled dynamics of light electromagnetic field with electrons and atoms in crystalline solids, where first-principles molecular dynamics based on time-dependent density…
We theoretically propose a method to enhance Raman scattering by injecting a seeded light field which is correlated with the initially prepared atomic spin wave. Such a light-atom correlation leads to an interference in the Raman…
We consider theoretically light scattering by a resonant layer that periodically moves in real space. At small frequencies of motion the scattered light spectrum reveals the frequency shift that is governed by the Doppler effect. At higher…
The application of molecular dynamics (MD) simulations to the interpretation of Raman scattering spectra is hindered by inability of atomistic simulations to account for the dynamic evolution of electronic polarizability, requiring the use…
Graphene is an ideal platform to study the coherence of quantum interference pathways by tuning doping or laser excitation energy. The latter produces a Raman excitation profile that provides direct insight into the lifetimes of…
An electron or electron-positron beam streaming through a plasma is notoriously prone to micro-instabilities. For a dilute ultrarelativistic infinite beam, the dominant instability is a mixed mode between longitudinal two-stream and…
Lately, experimental evidence of unexpectedly extremely high spatial resolution of tip-enhanced Raman scattering (TERS) has been demonstrated. Theoretically, two different contributions are discussed: an electromagnetic effect, leading to a…
Benchmark-quality rovibrational data are reported for the methane dimer from variational nuclear motion computations using an ab initio intermolecular potential energy surface reported by [M. P. Metz et al., Phys. Chem. Chem. Phys., 2019,…
We show that the increasingly popular nonlinear optical technique of time-domain coherent anti-Stokes Raman scattering (CARS), which is usually understood in terms of the semiclassical time-dependent third-order polarization, can be equally…
Light scattering limits the penetration depth of non-invasive Raman spectroscopy in biological media. While safe levels of irradiation may be adequate to analyze superficial tissue, scattering of the pump beam reduces the Raman signal to…
Ultrafast lasers have become one of the most powerful tools in coherent nonlinear optical spectroscopy. Short pulses enable direct observation of fast molecular dynamics, whereas broad spectral bandwidth offers ways of controlling nonlinear…
Understanding the interaction of charge carriers with lattice vibrations in the quasi-equilibrium regime is crucial for semiconductor functionality. However, the structural signatures of these interactions are often too subtle for…