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We study the effects of crystal anisotropy on optical phonon resonances in the second harmonic generation (SHG) from silicon carbide (SiC) in its Reststrahl region. By comparing experiments and simulations for isotropic 3C-SiC and…

Materials Science · Physics 2016-11-02 Alexander Paarmann , Ilya Razdolski , Sandy Gewinner , Wieland Schoellkopf , Martin Wolf

The spatial extent of excitons in molecular systems underpins their photophysics and utility for optoelectronic applications. Phonons are reported to lead to both exciton localization and delocalization. However, a microscopic understanding…

Coupling to phonon modes is a primary mechanism of excitonic dephasing and energy loss in semiconductors. However, low-energy phonons in colloidal quantum dots and their coupling to excitons are poorly understood, since their experimental…

Mesoscale and Nanoscale Physics · Physics 2019-10-22 Albert Liu , Diogo B. Almeida , Wan-Ki Bae , Lazaro A. Padilha , Steven T. Cundiff

We investigate polarization properties of neutral exciton emission in single self-assembled InAs/GaAs quantum dots. The in-plane shape and strain anisotropy strongly couple the heavy and light hole states and lead to large optical…

Mesoscale and Nanoscale Physics · Physics 2013-04-18 C. Tonin , R. Hostein , V. Voliotis , R. Grousson , A. Lemaitre , A. Martinez

Nanoscale single-crystals possess modified phonon dispersions due to the truncation of the crystal. The introduction of surfaces alters the population of phonons relative to the bulk and introduces anisotropy arising from the breaking of…

Mesoscale and Nanoscale Physics · Physics 2020-02-27 Kyle M. McElhinny , Gokul Gopalakrishnan , Martin V. Holt , David A. Czaplewski , Paul G. Evans

We apply the model introduced in Phys. Rev. B 75, 064202 (2007), cond-mat/0610469, to calculate the anisotropy effect in the interaction of two level systems with phonons in disordered crystals. We particularize our calculations to cubic…

Disordered Systems and Neural Networks · Physics 2009-11-13 Dragoş-Victor Anghel , Dmitry Churochkin

Anisotropy in strongly correlated materials is a central parameter in determining the electronic ground state and is tuned through the local crystalline electric field. This is notably the case in the CeCo$_{x}$Rh$_{1-x}$In$_{5}$ system…

Strongly Correlated Electrons · Physics 2024-11-28 D. J. Brener , I. Rodriguez Mallo , H. Lane , J. A. Rodriguez-Rivera , K. Schmalzl , M. Songvilay , K. Guratinder , C. Petrovic , C. Stock

First-principles calculations demonstrate an exceptional decoupling of charge and thermal transport along the \textit{a}-axis in CuBiSCl$_2$. The material achieves superior electron mobility (138 cm$^2$/V$\cdot$s at 300 K) through…

Materials Science · Physics 2025-04-03 Yu Wu , Ying Chen , Shuming Zeng , Liujiang Zhou , Chenhan Liu

Polaritons are a hybrid class of quasiparticles originating from the strong and resonant coupling between light and matter excitations. Recent years have witnessed a surge of interest in novel polariton types, arising from directional,…

Experimental phonon imaging in diamond anvils cell is demonstrated to be an adequate tool to extract the complete set of elastic constants of single-crystalline silicon up to the ZB$\rightarrow \beta-$Sn transition (10 GPa). Contrary to…

Materials Science · Physics 2015-05-19 F. Decremps , L. Belliard , M. Gauthier , B. Perrin

Phonons diffraction and interference patterns are observed at the atomic scale, using molecular dynamics simulations in systems containing crystalline silicon and nanometric obstacles as voids or amorphous-inclusions. The diffraction…

Boron arsenide (c-BAs) is at the forefront of research on ultrahigh thermal conductivity materials. We present a Raman scattering study of isotopically tailored cubic boron arsenide single crystals for 11 isotopic compositions spanning the…

Materials Science · Physics 2021-01-27 Akash Rai , Sheng Li , Hanlin Wu , Bing Lv , David G. Cahill

The phonon scattering processes on the three solid phases of ethanol are investigated by means of thermal conductivity, light and neutron scattering measurements as well as molecular dynamics simulations on single-crystalline models for the…

Cubic boron arsenide (BAs) is a promising semiconductor for next-generation electronics due to its outstanding ambipolar mobility and thermal conductivity, the latter of which is attributed to the suppression of three-phonon scattering.…

We investigate light-matter coupling in metallic crystals where plasmons coexist with phonons exhibiting large oscillator strength. We demonstrate theoretically that this coexistence can lead to strong light-matter interactions without…

Mesoscale and Nanoscale Physics · Physics 2019-04-25 David Hagenmüller , Johannes Schachenmayer , Cyriaque Genet , Thomas W. Ebbesen , Guido Pupillo

Phonon modes and their association with the electronic states have been investigated for the metallic EuCu$_{2}$As$_{2}$ system. In this work, we present the Raman spectra of this pnictide system which clearly shows the presence of seven…

Strongly Correlated Electrons · Physics 2025-01-10 Debasmita Swain , Mainak Dey Sarkar , Andrzej Ptok , G. Vaitheeswaran , Anushree Roy , Sitikantha D Das

The common wisdom that the phonon mechanism of electron pairing in the weak-coupling Bardeen-Cooper-Schrieffer (BCS) superconductors leads to conventional s-wave Cooper pairs is revised. An inevitable anisotropy of sound velocity in…

Superconductivity · Physics 2009-11-13 A. S. Alexandrov

Ultrasonic standing waves in a cylindrical enclosure can achieve very high local pressures at the acoustic nodes (~1 MPa). When the acoustic wave passes through a phononic crystal comprised of steel and glycerin, there are regions of…

Materials Science · Physics 2021-07-16 Edward A. Rietman

Charged colloidal crystals exhibit a subtle interplay between electrostatic screening and elastic deformation. In an anisotropic elastic medium the coupling between dilation and the local ionic environment becomes direction dependent,…

Soft Condensed Matter · Physics 2026-04-21 Hao Wu , Zhong-Can Ou-Yang

Optical properties of the lead halide perovskites nanocrystals are controlled by confined excitons and rich spectrum of confined acoustic and optical phonons. We study experimentally and theoretically the exciton-phonon interaction in…

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