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We have investigated the steady-sate valley polarization and valley coherence of encapsulated MoS2 monolayer as a function of the temperature and the power density with a continuous wave laser excitation. Both valley polarization and…

Materials Science · Physics 2021-11-01 Fabian Cadiz , Stefan Gerl , Takashi Taniguchi , Kenji Watanabe

Inversion symmetry breaking and three-fold rotation symmetry grant the valley degree of freedom to the robust exciton in monolayer transition metal dichalcogenides (TMDCs), which can be exploited for valleytronics applications. However, the…

Exciton-polaritons in semiconductor microcavities have advanced to become a model system for studying dynamical Bose-Einstein condensation, macroscopic coherence, many-body effects, nonclassical states of light and matter, and possibly…

Quantum Gases · Physics 2017-03-21 C. Schneider , K. Winkler , M. D. Fraser , M. Kamp , Y. Yamamoto , E. A. Ostrovskaya , S. Hoefling

Efficient scattering into the exciton polariton ground state is a key prerequisite for generating Bose-Einstein condensates and low-threshold polariton lasing. However, this can be challenging to achieve at low densities due to the…

Mesoscale and Nanoscale Physics · Physics 2024-01-09 Jamie M. Fitzgerald , Roberto Rosati , Beatriz Ferreira , Hangyong Shan , Christian Schneider , Ermin Malic

We apply the theory of open-quantum systems to describe light emission from coherently driven molecular polaritons. Based on the microscopic Hamiltonian that commonly describes the pure dephasing of isolated molecules, we show that under…

Mesoscale and Nanoscale Physics · Physics 2019-04-26 Tomáš Neuman , Javier Aizpurua

The manipulation of molecular excited state processes through strong coupling has attracted significant interest for its potential to provide precise control of photochemical phenomena. However, the key limiting factor for achieving this…

The generation of squeezed light in semiconductor materials opens opportunities for building on-chip devices that are operated at the quantum level. Here we study theoretically a squeezed light source of polariton dark solitons confined in…

Optics · Physics 2023-07-05 Gang Wang , Kexin Wu , Yang Liu , Weibin Li , Yan Xue

Manipulation of spin and valley degrees of freedom is a key step towards realizing novel quantum technologies, for which atomically thin transition metal dichalcogenides (TMDCs) have been established as promising candidates. In monolayer…

Large exciton-polariton optical nonlinearities present a key mechanism for photonics-based communication, ultimately in the quantum regime. Enhanced nonlinear response from various materials hosting excitons and allowing for their strong…

Mesoscale and Nanoscale Physics · Physics 2024-08-05 Anna M. Grudinina , Nina S. Voronova

We have studied the exciton states in a CdTe quantum ring in an external magnetic field containing a single magnetic impurity. We have used the multiband approximation which includes the heavy hole - light hole coupling effects. The…

Mesoscale and Nanoscale Physics · Physics 2015-06-19 Areg Ghazaryan , Aram Manaselyan , Tapash Chakraborty

Semiconducting transition metal dichalcogenide monolayers have emerged as promising candidates for future valleytronics-based quantum information technologies. Two distinct momentum-states of tightly-bound electron-hole pairs in these…

Mesoscale and Nanoscale Physics · Physics 2017-03-16 Gerd Plechinger , Tobias Korn , John M. Lupton

We theoretically investigate exciton relaxation dynamics in molecular aggregates based on model photosynthetic complexes under various conditions of incoherent excitation. We show that noise-induced quantum coherence is generated between…

Biological Physics · Physics 2014-08-14 Dmitri V. Voronine , Konstantin E. Dorfman , Bin Cao , Amitabh Joshi

Active metamaterials promise to enable arbitrary, temporal control over the propagation of wavefronts of light for applications such as beam steering, optical communication modulators, and holograms. This has been done in the past using…

The optical properties of transition metal dichalcogenide monolayers such as the two-dimensional semiconductors MoS$_2$ and WSe$_2$ are dominated by excitons, Coulomb bound electron-hole pairs. The light emission yield depends on whether…

Materials Science · Physics 2016-03-23 J. P. Echeverry , B. Urbaszek , T. Amand , X. Marie , I. C. Gerber

We analyze the properties of strongly coupled excitons and photons in systems made of semiconducting two-dimensional transition-metal dichalcogenides embedded in optical cavities. Through a detailed microscopic analysis of the coupling we…

Mesoscale and Nanoscale Physics · Physics 2018-10-03 Á. Gutiérrez-Rubio , L. Chirolli , L. Martín-Moreno , F. J. García-Vidal , F. Guinea

We investigate Landau-quantized excitonic absorption and luminescence of monolayer WSe$_2$ under magnetic field. We observe gate-dependent quantum oscillations in the bright exciton and trions (or exciton-polarons) as well as the dark…

Mesoscale and Nanoscale Physics · Physics 2020-03-04 Erfu Liu , Jeremiah van Baren , Takashi Taniguchi , Kenji Watanabe , Yia-Chung Chang , Chun Hung Lui

Here we proposed the valley selective excitations via a two-color (\ensuremath{\omega} + \ensuremath{2\omega}) laser field, made by superimposing two linearly polarized pulses at frequencies \ensuremath{\omega} and \ensuremath{2\omega}. We…

Optics · Physics 2023-06-21 Arqum Hashmi , Shunsuke Yamada , Kazuhiro Yabana , Tomohito Otobe

The band structure of transition metal dichalcogenides (TMDCs) with valence band edges at different locations in the momentum space could be harnessed to build devices that operate relying on the valley degree of freedom. To realize such…

Mesoscale and Nanoscale Physics · Physics 2016-09-06 Oriol Lopez Sanchez , Dmitry Ovchinnikov , Shikhar Misra , Adrien Allain , Andras Kis

Controlling matter-light interactions with cavities is of fundamental importance in modern science and technology. It is exemplified in the strong-coupling regime, where matter-light hybrid modes form, with properties controllable via the…

Mesoscale and Nanoscale Physics · Physics 2021-11-03 Long Zhang , Fengcheng Wu , Shaocong Hou , Zhe Zhang , Yu-Hsun Chou , Kenji Watanabe , Takashi Taniguchi , Stephen R. Forrest , Hui Deng

Monolayer transition metal dichalcogenides are a suitable platform for studying excitonic coherence in the light-matter coupling regime. We present an ab initio time-dependent GW-Bethe-Salpeter equation (GW-BSE) investigation of coherent…

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