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The van der Waals layered material CuInP2S6 features interesting functional behavior, including the existence of four uniaxial polarization states, polarization reversal against the electric field through Cu ion migration, a…

We consider nanoflakes of van der Waals ferrielectric CuInP$_2$S$_6$ covered by an ionic surface charge and reveal the appearance of polar states with relatively high polarization ~5 microC/cm$^2$ and stored free charge ~10 microC/cm$%2$,…

Complex oxide heterointerfaces and van der Waals heterostructures present two versatile but intrinsically different platforms for exploring emergent quantum phenomena and designing new functionalities. The rich opportunity offered by the…

Mesoscale and Nanoscale Physics · Physics 2020-03-19 Dawei Li , Xi Huang , Zhiyong Xiao , Hanying Chen , Le Zhang , Yifei Hao , Jingfeng Song , Ding-Fu Shao , Evgeny Y. Tsymbal , Yongfeng Lu , Xia Hong

Ferroelectricity in van der Waals (vdW) layered material has attracted a great deal of interest recently. CuInP$_2$S$_6$ (CIPS), the only vdW layered material whose ferroelectricity in the bulk was demonstrated by direct polarization…

Materials Science · Physics 2023-09-20 Jinyuan Yao , Yongtao Liu , Shaoqing Ding , Yanglin Zhu , Zhiqiang Mao , Sergei V. Kalinin , Ying Liu

Two-dimensional multiferroic van der Waals heterostructures provide a promising platform for the simultaneous control of distinct ferroic orders, with potential applications in magnetoelectric devices and spintronics. The practical…

Materials Science · Physics 2025-09-03 Priyanshu Raj , Sourav Mal , Rana Saha , Prasenjit Sen

Tunable optical materials are indispensable elements in modern optoelectronics, especially in integrated photonics circuits where precise control over the effective refractive index is essential for diverse applications. Two-dimensional…

Favourable band alignment and excellent visible light response are vital for photochemical water splitting. In this work, we have theoretically investigated how ferroelectric polarization and its reversibility in direction can be utilized…

Applied Physics · Physics 2020-09-03 Dimuthu Wijethunge , Lei Zhang , Cheng Tang , Aijun Du

Some van der Waals (vdW) materials exhibit ferroelectricity, making them promising for novel non-volatile memories (NVMs) such as ferroelectric diodes (FeDs). CuInP2S6 (CIPS) is a well-known vdW ferroelectric that has been integrated with…

Van der Waals (vdW) layered materials have rather weaker interlayer bonding than the intra-layer bonding, therefore the exfoliation along the stacking direction enables the achievement of monolayer or few layers vdW materials with emerging…

Interlayer stacking order has recently emerged as a unique degree of freedom to control crystal symmetry and physical properties in two-dimensional van der Waals (vdW) materials and heterostructures. By tuning the layer stacking pattern,…

Using the Landau-Ginzburg-Devonshire phenomenological approach we explore the strain-polarization coupling in the low-dimensional van der Waals ferrielectrics. We evolve the analytical model of the piezoelectric susceptibility of the…

We show how van der Waals (vdW) forces outcompete covalent and ionic forces to control ferroelectric ordering in CuInP2S6 nanoflakes as well as in CuInP2S6 and CuBiP2Se6 crystals. While the self-assembly of these 2D layered materials is…

Materials Science · Physics 2018-05-31 Jeffrey R. Reimers , Sherif Abdulkader Tawfik , Michael J. Ford

The electronic structure of high-quality van der Waals multiferroic CuCrP$_2$S6 crystals was investigated applying photoelectron spectroscopy methods in combination with DFT analysis. Using X-ray photoelectron and near-edge X-ray absorption…

Using Landau-Ginzburg-Devonshire (LGD) phenomenological approach we analyze the bending-induced re-distribution of electric polarization and field, elastic stresses and strains inside ultrathin layers of van der Waals ferrielectrics. We…

The contribution of flexoelectric coupling to the long-range order parameter fluctuations in ferroics can be critically important to the ferron dispersion and related polar, pyroelectric and electrocaloric properties. Here we calculate…

Magnetoelectric coupling in insulating multiferroic materials is invaluable for both fundamental research and multifunctional device applications. However, material realization remains a significant challenge. We employ first-principles…

Materials Science · Physics 2025-07-08 Xilong Xu , Li Yang

Layered two-dimensional van der Waals (vdW) semiconductors and their heterostructures have been shown to exhibit positive photoconductance (PPC) in many studies. A few recent reports have demonstrated negative photoconductance (NPC) as well…

Applied Physics · Physics 2022-06-10 Himani Jawa , Sayantan Ghosh , Abin Varghese , Srilagna Sahoo , Saurabh Lodha

Multiferroic materials provide robust and efficient routes for the control of magnetism by electric fields, which has been diligently sought after for a long time. The two-dimensional (2D) vdW multiferroics is a more exciting endeavour. To…

Materials Science · Physics 2023-10-18 Yangliu Wu , Deju Zhang , Yanning Zhang , Longjiang Deng , Bo Peng

As basic building blocks for next-generation information technologies devices, high-quality p-n junctions based on van der Waals (vdW) materials have attracted widespread interest.Compared to traditional two dimensional (2D) heterojunction…

Mesoscale and Nanoscale Physics · Physics 2023-05-12 Huanfeng Zhu , Jialin Li , Qiang Chen , Wei Tang , Xinyi Fan , Fan Li , Linjun Li

Manipulating nanoscale light-matter interactions on ultrafast time scales is indispensable for future polaritonic devices. Hyperbolic phonon polaritons (HPhPs) in van der Waals materials enable deep subwavelength confinement of…

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