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Related papers: Ligand-Controlled Phonon Dynamics in CsPbBr3 Nanoc…

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The discovery of localized plasmon polariton resonances has been pivotal in enabling tunability of the optical resonance. Recently, extensive research efforts have aimed to expand these achievements to other polaritonic states that exhibit…

During the last years, giant optical anisotropy demonstrated its paramount importance for light manipulation which resulted in numerous applications ranging from subdiffraction light guiding to switchable nanolasers. In spite of recent…

Metal halide perovskites have emerged as an exciting class of materials for applications in solar energy harvesting, optical devices, catalysis, and other photophysical applications. Many of the exciting properties of halide perovskites are…

Materials Science · Physics 2024-04-18 Colin M. Hylton-Farrington , Richard C. Remsing

Atomic dynamics takes a fundamental part in numbers of physical properties of solids like high-Tc superconductivity, semiconducting transports, and thermoelectricity. Perovskite CH3NH3PbI3 exhibits outstanding photovoltaic performances, but…

The pure CsPbBr$_3$ perovskite is an archetypal example of a strongly anharmonic crystal that poses a major challenge for computational methods to describe its thermodynamic properties. Its lattice dynamics exhibits characteristics of a…

Mesoscale and Nanoscale Physics · Physics 2024-01-04 Jonathan Lahnsteiner , Max Rang , Menno Bokdam

Bound states in the continuum (BICs) are a fascinating class of eigenstates that trap energy within the continuum, enabling breakthroughs in ultra-low-threshold lasing, high-Q sensing, and advanced wave-matter interactions. However, their…

Applied Physics · Physics 2026-04-29 Sheng-Nan Liang , Zhen-Hui Qin , Shu-Mao Wu , Hua-Yang Chen , Si-Yuan Yu , Yan-Feng Chen

Lead-free metal halide perovskites are emerging as less-toxic alternatives to their lead-based counterparts. However, their applicability in optoelectronic devices is limited, and the charge transport dynamics remain poorly understood.…

Hyperbolic phonon polaritons (HPhPs) in orthorhombic-phase molybdenum trioxide ($\alpha$-MoO3) show in-plane hyperbolicity, great wavelength compression and ultra-long lifetime, therefore holding great potential in nanophotonic…

Materials Science · Physics 2020-11-25 Weikang Dong , Ruishi Qi , Tiansheng Liu , Yi Li , Ning Li , Ze Hua , Zirui Gao , Shuyuan Zhang , Kaihui Liu , Jiandong Guo , Peng Gao

The surface ligands in colloidal metal halide perovskites influence not only their intrinsic optoelectronic properties but also their interaction with other materials and molecules. We explore donor-acceptor interactions of CsPbBr3…

The vibrational modes in organic/inorganic layered perovskites are of fundamental importance for their optoelectronic properties. The hierarchical architecture of the Ruddlesden-Popper phase of these materials allows for distinct…

We study the energetics of quasi-particle excitations in CsPbBr3 perovskite nanocrystals using path integral molecular dynamics simulations. Employing detailed molecular models, we elucidate the interplay of anharmonic lattice degrees of…

Chemical Physics · Physics 2023-07-14 Yoonjae Park , David T. Limmer

Understanding the interplay between bright and dark exciton states is crucial for deciphering the luminescence properties of low-dimensional materials. The origin of the outstanding brightness of lead halide perovskites remains elusive.…

Mesoscale and Nanoscale Physics · Physics 2024-04-16 Mohamed-Raouf Amara , Caixia Huo , Christophe Voisin , Qihua Xiong , Carole Diederichs

Nonlinear phononics is the phenomenon in which a coherent dynamics in a material along a set of phonons is launched after its infrared-active phonons are selectively excited using external light pulses. The microscopic mechanism underlying…

Materials Science · Physics 2023-08-23 Alaska Subedi

The interaction between the electrons and the lattice vibrations in a solid is responsible for various important effects, such as formation of polarons, temperature dependent bandgaps, phonon-limited carrier transport, and conventional…

Surface phonon polaritons hold much potential for subwavelength control and manipulation of light at the infrared to terahertz wavelengths. Here, aided by monochromatic scanning transmission electron microscopy - electron energy loss…

Mesoscale and Nanoscale Physics · Physics 2021-03-16 Yuehui Li , Ruishi Qi , Ruochen Shi , Ning Li , Yuanwei Sun , Bingyao Liu , Peng Gao

The band-gaps of CsPbI$_3$ perovskite nanocrystals are measured by absorption spectroscopy at cryogenic temperatures. Anomalous band-gap shifts are observed in CsPbI$_3$ nanocubes and nanoplatelets, which are modeled accurately by band-gap…

The exploitation of phonon-polaritons in nanostructured materials offers a pathway to manipulate infrared (IR) light for nanophotonic applications. Notably, hyperbolic phonons polaritons (HP2) in polar bidimensional crystals have been used…

Empirical A-site cation substitution has advanced the stability and efficiency of hybrid organic-inorganic lead halide perovskites solar cells and the functionality of X-ray detectors. Yet, the fundamental mechanisms underpinning their…

The recent emergence of quantum confined nanomaterials in the field of radiation detection, in particular lead halide perovskite nanocrystals, offers potentially revolutionary scalability and performance advantages over conventional…

Two-dimensional hybrid organic-inorganic metal halide perovskites offer enhanced stability for perovskite-based applications. Their crystal structure's soft and ionic nature gives rise to strong interactions between charge carriers and…