Related papers: Breakdown of the isotropic asymptotic approximatio…
We use the soft photon approximation to extract the Wigner time delay from atomic two-color photoionization experiments. Unlike the strong field approximation, the present method does not require introduction of the Coulomb-laser coupling…
We consider the two-photon ionization of Hydrogen-like atoms. We find an approximate expression of the long-range phase based on an asymptotic expansion of the continuum eigenfunctions within the Wentzel-Kramers-Brillouin approximation.…
No, we cannot! The concept of Wigner time delay was introduced in scattering theory to quantify the delay or advance of an incoming particle in its interaction with the scattering potential. It was assumed that this concept can be…
We investigate signatures of anisotropy on the dynamics of time-resolved near-threshold molecular photoemission, through simulations on a one-dimension asymmetric model molecule. More precisely, we study the relationship between the…
In scattering theory, the Wigner-Smith time delay, calculated through a phaseshift derivative or its multichannel generalization, has been demonstrated to measure the amount of delay or advance experienced by colliding particles during…
Upon absorbing a photon, the ionized electron sails through the target force field in attoseconds to reach free space. This navigation probes details of the potential landscape that get imprinted into the phase of the ionization amplitude.…
We study laser-assisted photodetachment time delays by attosecond pulse trains from the closed-shell negative ions F- and Cl-. We investigate the separability of the delay into two contributions: (i) the Wigner-like delay associated with…
We have implemented the gedanken experiment of an individual atom scattering a wave packet of near-resonant light, and measured the associated Wigner time-delay as a function of the frequency of the light. In our apparatus the atom behaves…
Photoionization of matter is one of the fastest electronic processes in nature. Experimental measurements of photoionization dynamics have become possible through attosecond metrology. However, all experiments reported to date contain a…
Attosecond ionization time-delays at photoelectron energies above typically 10 eV are usually interpreted using the so called asymptotic approximation as a sum of the atomic or molecular delays with a universal laser-induced contribution.…
Streaked photoemission metrology allows the observation of an apparent relative time delay between the detection of photoelectrons from different initial electronic states. This relative delay is obtained by recording the photoelectron…
Determination and interpretation of Wigner-like photoionisation delays is one of the most active fields of attosecond science. Previous results have suggested that large photoionisation delays are associated with structured continua, but a…
We present measurements of single-photon ionization time delays between valence electrons of argon and neon using a coincidence detection technique that allows for the simultaneous measurement of both species under identical conditions.…
We study the temporal aspects of laser-assisted extreme ultraviolet (XUV) photoionization using attosecond pulses of harmonic radiation. The aim of this paper is to establish the general form of the phase of the relevant transition…
Time-delays in the photoionization of molecules are investigated. As compared to atomic ionization, the time-delays expected from molecular ionization present a much richer phenomenon, with a strong spatial dependence due to the anisotropic…
This tutorial presents an introduction to the interaction of light and matter on the attosecond timescale. Our aim is to detail the theoretical description of ultra-short time-delays, and to relate these to the phase of extreme ultraviolet…
Attosecond streaking of atomic photoemission holds the promise to provide unprecedented information on the release time of the photoelectron. We show that attosecond streaking phase shifts indeed contain timing (or spectral phase)…
Time delays of electrons emitted from an isotropic initial state and leaving behind an isotropic ion are assumed to be angle-independent. Using an interferometric method involving XUV attosecond pulse trains and an IR probe field in…
Ultrafast processes in matter, such as the electron emission following light absorption, can now be studied using ultrashort light pulses of attosecond duration ($10^{-18}$s) in the extreme ultraviolet spectral range. The lack of spectral…
More than 100 years after its discovery and its explanation in the energy domain, the duration of the photoelectric effect is still heavily studied. The emission time of a photoelectron can be quantified by the Wigner time delay.…