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Deciphering the three-dimensional atomic structure of solid-solid interfaces in core-shell nanomaterials is the key to understand their remarkable catalytical, optical and electronic properties. Here, we probe the three-dimensional atomic…

Materials Science · Physics 2023-06-21 Zezhou Li , Zhiheng Xie , Yao Zhang , Xilong Mu , Hai-jing Yin , Ya-wen Zhang , Colin Ophus , Jihan Zhou

This review discusses how low-energy, valence excitations created by swift electrons can render information on the optical response of structured materials with unmatched spatial resolution. Electron microscopes are capable of focusing…

Materials Science · Physics 2012-11-13 F. J. Garcia de Abajo

The study of spin-orbit coupling (SOC) of light is crucial to explore the light-matter interactions in sub-wavelength nanostructures with broken symmetries. In noncentrosymmetric photonic crystals, the SOC results in the splitting of the…

The relations for the polarizability of the metallic nanoparticles, coated with the shell of cyanine dyes, are obtained in the article. The frequency dependencies for light absorption and scattering efficiencies, the heating of the…

Soft Condensed Matter · Physics 2024-01-18 A. V. Korotun , N. A. Smirnova , V. I. Reva , I. M. Titov , G. M. Shilo

We present a theoretical approach to determine the electronic properties of nanoscale systems exhibiting strong electron-electron and electron-phonon interactions and coupled to metallic electrodes. This approach is based on an…

Strongly Correlated Electrons · Physics 2009-11-13 A. Martin-Rodero , A. Levy Yeyati , F Flores , R. C. Monreal

This work sets a road-map towards an experimental realization of strong coupling between free-electrons and photons, and analytically explores entanglement phenomena that emerge in this regime. The proposed model unifies the strong-coupling…

Quantum Physics · Physics 2019-09-11 Ofer Kfir

Advanced computational tools that describe the interaction of electrons with structured nanophotonic materials are crucial for theoretical predictions, specific design tasks, and the interpretation of experimental results. These tools open…

Computational Physics · Physics 2026-02-16 P. Elli Stamatopoulou , Carsten Rockstuhl

Strong light-matter coupling gives rise to polaritons - hybrid excitations whose mixed photonic and matter character enables control over optical, electronic and chemical properties. This Feature Article surveys the main architectures…

Plasmonic cavities can be used to control the atom-photon coupling process at the nanoscale, since they provide ultrahigh density of optical states in an exceptionally small mode volume. Here we demonstrate strong coupling between molecular…

Atomic-layer and two-dimensional (2D) materials have emerged as essential building blocks for next-generation quantum and semiconductor technologies, where atomic-scale control over light-matter interactions is critical. However, their…

Coupling of light into a thin layer of high refractive index material by plasmonic nanoparticles has been widely studied for application in photovoltaic devices, such as thin-film solar cells. In numerous studies this coupling has been…

Optics · Physics 2012-11-29 Antti M. Pennanen , J. Jussi Toppari

The ability to manipulate plasmons is driving new developments in electronics, optics, sensing, energy, and medicine. Despite the massive momentum of experimental research in this direction, a predictive quantum-mechanical framework for…

Materials Science · Physics 2016-10-12 Fabio Caruso , Feliciano Giustino

The possibility of strong coupling between a single molecule and surface plasmons is analyzed on the basis of a microscopic classical description. It is predicted that strong single molecule - plasmon coupling can happen for a silver…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Mykhaylo M. Dvoynenko

A hybrid system composed of an isotropic nanoparticle and a semiconductor heterostructure with a quantum well has been considered. The nanoparticle is supposed to be polarizable in an external electric field. A theoretical model of the…

Mesoscale and Nanoscale Physics · Physics 2012-06-22 V. A. Kochelap , S. M. Kukhtaruk

Cathodoluminescence, i.e. the radiation caused by the interaction of high-energy electron beams with matter, has gained a major interest in the analysis of minerals, semiconductors, and plasmonic resonances in nanoparticles. This radiation…

Frequency shifts, radiative decay rates, the Ohmic loss contribution to the nonradiative decay rates, fluorescence yields, and photobleaching of a two-level atom radiating anywhere inside or outside a complex spherical nanoshell, i.e. a…

Quantum Physics · Physics 2007-05-23 Alexander Moroz

We reveal new aspects of the interaction between plasmons and phonons in 2D materials that go beyond a mere shift and increase in plasmon width due to coupling to either intrinsic vibrational modes of the material or phonons in a supporting…

Electron energy loss spectroscopy is consolidating as a powerful tool to explore electronic (as well as vibrational) excitations of matter, including molecules. Performed in a scanning transmission electron microscope, this technique is…

Chemical Physics · Physics 2021-03-05 Ciro A. Guido , Enzo Rotunno , Matteo Zanfrognini , Stefano Corni , Vincenzo Grillo

Metallic nanostructures provide a toolkit for the generation of coherent light below the diffraction limit. Plasmonic based lasing relies on the population inversion of emitters (such as organic fluorophores) along with feedback provided by…

Recently, the concept of strong light-matter coupling has been demonstrated in semiconductor structures, and it is poised to revolutionize the design and implementation of components, including solid state lasers and detectors. We…