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A quantum-mechanical model to calculate the electron energy-loss spectra (EELS) for the system of a closely located metallic nanoshell and a molecule has been developed. At the resonance between the molecular excitation and plasmon modes in…

Atomic Physics · Physics 2014-10-07 I. Yu. Goliney , Ye. V. Onykienko

We theoretically analyse the hybrid Mie-exciton optical modes arising from the strong coupling of excitons in organic dyes or transition-metal dichalcogenides with the Mie resonances of high-index dielectric nanoparticles. Detailed analytic…

Mesoscale and Nanoscale Physics · Physics 2018-10-29 C. Tserkezis , P. A. D. Gonçalves , C. Wolff , F. Todisco , K. Busch , N. A. Mortensen

We study spatial coherence properties of a system composed of periodic silver nanoparticle arrays covered with a fluorescent organic molecule (DiD) film. The evolution of spatial coherence of this composite structure from the weak to the…

Semiconductor nanoparticles and nanostructures in the strong coupling regime exhibit an intriguing energy scale in the optical frequencies, which is specified by the Rabi splitting between the upper and lower exciton-polariton states.…

Optics · Physics 2019-11-19 Burak Gerislioglu , Arash Ahmadivand

Hybrid molecular-plasmonic nanostructures have demonstrated their potential for surface enhanced spectroscopies, sensing or quantum control at the nanoscale. In this work, we investigate the strong coupling regime and explicitly describe…

Quantum Physics · Physics 2017-07-05 H. Varguet , B. Rousseaux , D. Dzsotjan , H. Jauslin , S. Guerin , G. Colas des Francs

Nanoparticles supporting a distinct series of Mie resonances have enabled a new class of nanoantennas and provide efficient ways to manipulate light at the nanoscale. The ability to flexibly tune the optical resonances and scattering…

Optics · Physics 2021-05-26 Yiwei Dong , Yuanqing Yang

We consider the interaction of electromagnetic radiation of arbitrary polarization with multi-level atoms in a self-consistent manner, taking into account both spatial and temporal dependencies of local fields. This is done by numerically…

Mesoscale and Nanoscale Physics · Physics 2015-03-19 Maxim Sukharev , Abraham Nitzan

We investigate the dynamics of photon echo exhibited by exciton-plasmon systems under strong coupling conditions. Using a self-consistent model based on coupled Maxwell-Bloch equations we investigate femtosecond time dynamics of ensembles…

Mesoscale and Nanoscale Physics · Physics 2017-04-05 Adam Blake , Maxim Sukharev

The interaction between free electrons and nanoscale optical fields has emerged as a unique platform to investigate ultrafast processes in matter and explore fundamental quantum phenomena. In particular, optically modulated electrons are…

Mesoscale and Nanoscale Physics · Physics 2024-11-07 Adamantios P. Synanidis , P. A. D. Gonçalves , Claus Ropers , F. Javier García de Abajo

The interaction between intense light-matter not only promotes emerging applications in quantum and nonlinear optics but also facilitates changes in material properties. Plasmons can significantly enhance not only molecular chirality but…

Optics · Physics 2025-02-03 Nan Gao , Haoran Liu , Yurui Fang

Near-fields around nanophotonic structures and waveguides can be used to optically interface particles ranging from atoms and molecules to microscopic biological and synthetic particles. Due to the strong, non-linear dependence of the…

Warm-dense matter (WDM) is a highly-excited state that lies at the confluence of solids, plasmas, and liquids and that cannot be described by equilibrium theories. The transient nature of this state when created in a laboratory, as well as…

Localized plasmonic modes of metallic nanoparticles may hybridize like those of atoms forming a molecule. However, the rapid decay of the plasmonic fields outside the metal severely limits the range of these interactions to tens of…

Optics · Physics 2013-03-05 Adi Salomon , Yehiam Prior , Radoslaw Kolkowski , Joseph Zyss

We study the core hole-electron correlation in coherently coupled molecules by energy dispersive near edge X-ray absorption fine-structure spectroscopy. In a transient phase, which exists during the transition between two bulk arrangements,…

Materials Science · Physics 2013-12-03 M. Scholz , F. Holch , C. Sauer , M. Wiessner , A. Schöll , F. Reinert

Probing optical excitations with nanometer resolution is important for understanding their dynamics and interactions down to the atomic scale. Electron microscopes currently offer the unparalleled ability of rendering spatially-resolved…

Quantum Physics · Physics 2020-07-16 Valerio Di Giulio , Mathieu Kociak , F. Javier García de Abajo

Intermixed light-matter quasiparticles - polaritons - possess unique optical properties owned to their compositional nature. These intriguing hybrid states have been extensively studied over the past decades in a wide range of realizations…

Free-electron interactions with light and matter have long served as a cornerstone for exploring the quantum and ultrafast dynamics of material excitation. In recent years, this paradigm has evolved from a classical description of radiation…

Optics · Physics 2026-02-20 Fatemeh Chahshouri , Sven Ebel , Mitja Funk , Nahid Talebi

We investigate - both experimentally and theoretically - the inelastic interaction between fast electrons and the electromagnetic field scattered by metallic apertures and nanostructures on dielectric membranes using photon induced…

Propagation of light through dielectrics lies at the heart of optics. However, this ubiquitous process is commonly described using phenomenological dielectric function $\varepsilon$ and magnetic permeability $\mu$, i.e. without addressing…

Quantum Physics · Physics 2016-11-30 Harald R. Haakh , Sanli Faez , Vahid Sandoghdar

The coherent oscillations of mobile charge carriers near the surface of good conductors-surface plasmons-are been exploited in many applications in information technologies, clean energy, high-density data storage, photovoltaics, chemistry,…

Mesoscale and Nanoscale Physics · Physics 2023-12-20 Jacob Khurgin , Anton Yu. Bykov , Anatoly V. Zayats