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Ferroelectric relaxors are complex materials with distinct properties. The understanding of their dielectric susceptibility, which strongly depends on both temperature and probing frequency, have interested researchers for many years. Here…

Materials Science · Physics 2017-08-30 J. Liu , F. Li , Y. Zeng , Z. Jiang , D. Wang , Z. -G. Ye , C. -L. Jia

119Sn nuclear magnetic resonance (NMR) spectra and spin-lattice relaxation rate (1/T1) in SnO2 nanoparticles were measured as a function of temperature and compared with those of SnO2 bulk sample. A 15% loss of 119Sn NMR signal intensity…

Materials Science · Physics 2011-12-09 Tusharkanti Dey , P. Khuntia , A. V. Mahajan , Nitesh Kumar , A. Sundaresan

Nuclear magnetic resonance, electron paramagnetic resonance and magnetization measurements show that bulk Li$_x$ZnPc are strongly correlated one-dimensional metals. The temperature dependence of the nuclear spin-lattice relaxation rate…

Strongly Correlated Electrons · Physics 2008-08-25 M. Filibian , P. Carretta , M. C. Mozzati , P. Ghigna , G. Zoppellaro , M. Ruben

Raman scattering in relaxor ferroelectric PbMg1/3Ta2/3O3 (PMT) was investigated in the single crystalline form in the temperature range of 20 - 295 K. Anomalous temperature dependence of the integrated intensity and the Raman line contours…

Materials Science · Physics 2007-05-23 S. G. Lushnikov , S. N. Gvasaliya , R. S. Katiyar

The lead-halide perovskites, including CH$_{3}$NH$_{3}$PbBr$_{3}$, are components in cost effective, highly efficient photovoltaics, where the interactions of the molecular cations with the inorganic framework are suggested to influence the…

Materials Science · Physics 2015-10-14 I. P. Swainson , C. Stock , S. F. Parker , L. Van Eijck , M. Russina , J. W. Taylor

We report a numerical implementation of the Landau-Lifshitz-Baryakhtar theory, which dictates that the micromagnetic relaxation term obeys the symmetry of the magnetic crystal, i. e. replacing the single intrinsic damping constant with a…

Mesoscale and Nanoscale Physics · Physics 2014-02-17 Mykola Dvornik , Arne Vansteenkiste , Bartel Van Waeyenberge

We have performed elastic diffuse neutron scattering studies on the relaxor Pb(Mg$_{1/3}$Nb$_{2/3}$)O$_3$ (PMN). The measured intensity distribution near a (100) Bragg peak in the (hk0) scattering plane assumes the shape of a butterfly with…

Materials Science · Physics 2009-11-10 Guangyong Xu , G. Shirane , J. R. D. Copley , P. M. Gehring

A first-principles-based model is developed to investigate the influence of lead vacancies on the properties of relaxor ferroelectric Pb(Sc1/2Nb1/2)O3 (PSN). Lead vacancies generate large, inhomogeneous, electric fields that reduce barriers…

Materials Science · Physics 2009-11-11 L. Bellaiche , Jorge Iniguez , Eric Cockayne , B. P. Burton

We report neutron inelastic scattering experiments on single crystal PbMg$_{1/3}$Nb$_{2/3}$O$_{3}$ doped with 32\% PbTiO$_{3}$, a relaxor ferroelectric that lies close to the morphotropic phase boundary. When cooled under an electric field…

Materials Science · Physics 2016-01-06 John A. Schneeloch , Zhijun Xu , B. Winn , C. Stock , P. M. Gehring , R. J. Birgeneau , Guangyong Xu

Hybrid lead-halide perovskites have emerged as an excellent class of photovoltaic materials. Recent reports suggest that the organic molecular cation is responsible for local polar fluctuations that inhibit carrier recombination. We combine…

Full-potential linearized augmented plane wave (FP-LAPW) method with the generalized gradient approximation (GGA) for the exchange-correlation potential has been applied for the study of structural, elastic and electronic properties of the…

Superconductivity · Physics 2008-11-27 I. R. Shein , V. V. Bannikov , A. L. Ivanovskii

The potential of lead-halide perovskites for realistic applications is currently hindered by their limited long-term stability under functional activation. While the role of lattice flexibility in the thermal response of perovskites has…

A physical mechanism for the freezing of polar nanoregions (PNRs) in relaxor ferroelectrics is presented. Assuming that the activation energy for the reorientation of a cluster of PNRs scales with the mean volume of the cluster, the…

Disordered Systems and Neural Networks · Physics 2009-11-13 R. Pirc , R. Blinc

We present a detailed dielectric study of the relaxation effects that occur in several perovskite rare-earth manganites, including the multiferroics TbMnO3 and DyMnO3. We demonstrate that the strong magnetocapacitive effects, observed for…

Strongly Correlated Electrons · Physics 2009-06-17 F. Schrettle , P. Lunkenheimer , J. Hemberger , V. Yu. Ivanov , A. A. Mukhin , A. M. Balbashov , A. Loidl

Roles of orbital and lattice degrees of freedom in strongly correlated systems are investigated to understand electronic properties of perovskite Mn oxides such as La_{1-x}Sr_{x}MnO_{3}. An extended double-exchange model containing Coulomb…

Strongly Correlated Electrons · Physics 2007-05-23 Yukitoshi Motome , Masatoshi Imada

It is now well established that the unique properties of relaxor ferroelectrics are due to the presence of polar nanoregions (PNR's). We present recent results from Neutron and Raman scattering of single crystals of PZN, PZN-xPT, and PMN.…

Materials Science · Physics 2009-11-10 D. La-Orauttapong , O. Svitelskiy , J. Toulouse

The stability of the disordered glassy phase in the relaxors PbMg1/3Nb2/3O3 and (PbMg1/3Nb2/3O3)0.88(PbTiO3)0.12, called PMN and PMN-PT, was investigated by preparing partially polarized samples and allowing them to age at zero field in the…

Materials Science · Physics 2009-11-13 Eugene V. Colla , Derek Vigil , John Timmerwilke , M. B. Weissman , D. D. Viehland , Brahim Dkhil

We analyze scattering of the transverse optic modes by spherically symmetric Polarized Nano Regions (PNR) in the paraelectric phase of relaxor ferroelectrics. Calculations have done in the frame of mean-field model early supposed by E.Iolin…

Materials Science · Physics 2015-03-17 Eugene Iolin

We consider a standard Ginzburg-Landau model of a ferroelectric whose electrical polarization is coupled to gradients of elastic strain. At the harmonic level, such flexoelectric interaction is known to hybridize acoustic and optic phonon…

Materials Science · Physics 2023-07-27 G. G. Guzmán-Verri , C. H. Liang , P. B. Littlewood

The recent discovery of nematic liquid crystals with polar order (ferroelectric nematic) has created immense interest. Despite intensive research, several physical properties of this liquid crystal are yet to be investigated and understood.…

Soft Condensed Matter · Physics 2022-11-28 Abinash Barthakur , Jakub Karcz , Przemyslaw Kula , Surajit Dhara
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