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The relaxor ferroelectric PbMg1/Nb2/3O3 was investigated by means of broad-band dielectric and Fourier Transform Infrared (FTIR) transmission spectroscopy in the frequency range from 1 MHz to 15 THz at temperatures between 20 and 900 K…

Materials Science · Physics 2009-11-10 S. Kamba , M. Kempa , V. Bovtun , J. Petzelt , K. Brinkman , N. Setter

The relaxors Pb(Zn$_{1/3}$Nb$_{2/3}$)O$_{3}$ (PZN) and Pb(Mg$_{1/3}$Nb$_{2/3}$)O$_{3}$ (PMN) have very similar properties based on the dielectric response around the critical temperature $T_{c}$ (defined by the structural transition under…

Materials Science · Physics 2009-11-10 C. Stock , R. J. Birgeneau , S. Wakimoto , J. S. Gardner , W. Chen , Z. -G. Ye , G. Shirane

We have performed a series of neutron diffuse scattering measurements on a single crystal of the solid solution Pb(Zn$_{1/3}$Nb$_{2/3}$)O$_3$ (PZN) doped with 8% PbTiO$_3$ (PT), a relaxor compound with a Curie temperature T$_C \sim 450$ K,…

Materials Science · Physics 2009-11-11 Guangyong Xu , P. M. Gehring , G. Shirane

We suggest considering the Burns temperature in lead containing relaxor ferroelectrics as the temperature, at which Pb becomes off-center and nearly randomly occupies positions around the center on a sphere with the radius, which increases…

Disordered Systems and Neural Networks · Physics 2007-05-23 S. A. Prosandeev , S. B. Vakhrushev , N. M. Okuneva , P. A. Markovin , I. P. Raevski , I. N. Zaharchenko , M. S. Prosandeeva

From the new infrared (IR) reflectivity and time-domain terahertz (THz) spectra combined with available high-frequency dielectric data above the MHz range in a broad temperature range of 10-900 K, a full picture of the soft and central mode…

Materials Science · Physics 2017-12-19 D. Nuzhnyy , J. Petzelt , V. Bovtun , M. Kempa , S. Kamba , J. Hlinka , B. Hehlen

Relaxor ferroelectric perovskites are highly polarizable and can exhibit giant coupling between elastic strain and an applied electric field. Here, we report an in situ extended X-ray absorption fine structure (EXAFS) study of a…

The low-energy part of the vibration spectrum in PbMg$_{1/3}$Nb$_{2/3}$O$_3$ (PMN) relaxor ferroelectric has been studied by neutron scattering above and below the Burns temperature, T$_d$. The transverse acoustic and the lowest transverse…

Materials Science · Physics 2007-05-23 S N Gvasaliya , B Roessli , R A Cowley , P Hubert , S G Lushnikov

The crystal structure of the PbMg$_{1/3}$Ta$_{2/3}$O$_3$ (PMT) relaxor ferroelectric was studied under hydrostatic pressure up to $\sim 7$ GPa by means of powder neutron diffraction. We find a drastic pressure-induced decrease of the lead…

Materials Science · Physics 2007-05-23 S. N. Gvasaliya , V. Pomjakushin , B. Roessli , Th. Straessle , S. Klotz , S. G. Lushnikov

Neutron and x-ray diffraction techniques have been used to study the competing long and short-range polar order in the relaxor ferroelectric Pb(Mg$_{1/3}$Nb$_{2/3}$)O$_{3}$ (PMN) under a [111] applied electric field. Despite reports of a…

Materials Science · Physics 2009-11-13 C. Stock , Guangyong Xu , P. M. Gehring , H. Luo , X. Zhao , H. Cao , J. F. Li , D. Viehland , G. Shirane

We develop a theory to study the characteristics of dipolar / strain fluctuations in perovskite relaxors. In addition to the soft TO and TA phonons, we take into account another freedom of motion associated with the random hopping of…

Materials Science · Physics 2007-05-23 Y. Yamada , T. Takakura

High-pressure and variable temperature single crystal synchrotron X-ray measurements combined with first-principles based molecular dynamics simulations study diffuse scattering in the relaxor ferroelectric system PSN…

Materials Science · Physics 2015-05-13 P. Ganesh , E. Cockayne , M. Ahart , R. E. Cohen , B. Burton , R. J. Hemley , Yang Ren , Wenge Yang , Z-G Ye

Electric field dependent mechanical properties of relaxor ferroelectric material Pb(Mn1/3Nb2/3)O3-PbTiO3 are investigated with the nanoindentation technique. Giant electric-field-tunable apparent elastic modulus (up to -39%), hardness (-9%…

Mesoscale and Nanoscale Physics · Physics 2014-02-12 Hao Zhou , Yongmao Pei , Faxin Li , Haosu Luo , Daining Fang

A Landau-type phenomenological cluster theory was presented to model the freezing process of local polarization in relaxors. Based on the theory, the proportion of frozen polarization in Pb(Mg$_{1/3}$Nb$_{2/3}$)O$_3$-PbTiO$_3$ (PMNT) was…

Materials Science · Physics 2009-11-07 Zhi-Rong Liu , Yong Zhang , Bing-Lin Gu , Xiao-Wen Zhang

The microstructure and phase transition in relaxor ferroelectric Pb(Mg1/3Nb2/3)O3 (PMN) and its solid solution with PbTiO3 (PT), PMN-xPT, remain to be one of the most puzzling issues of solid state science. In the present work we have…

Materials Science · Physics 2009-11-07 Z. -G. Ye , Y. Bing , J. Gao , A. A. Bokov , P. Stephens , B. Noheda , G. Shirane

Synchrotron x-ray scattering studies of anti-ferroelectric nanoregions (AFR) as fluctuations, which give rise to 1/2(hk0) superlattice reflections (alpha spots), were systematically performed in Pb(Mg1/3Nb2/3)O3 (PMN) ferroelectric relaxor.…

Materials Science · Physics 2007-05-23 A. Tkachuk , Haydn Chen

The paper suggests to treat the infrared reflectivity spectra of single crystal perovskite relaxors as fine-grained ferroelectric ceramics: locally frozen polarization makes the dielectric function strongly anisotropic in the phonon…

Materials Science · Physics 2009-11-11 J. Hlinka , T. Ostapchuk , D. Noujni , S. Kamba , J. Petzelt

A complete understanding of the mechanisms for dielectric relaxation in relaxor ferroelectrics remains elusive. We used a structural refinement framework that integrates several types of experimental data to identify the nanoscale…

We report appearance of the net magnetization in Mn-based antiperovskite compounds as a result of the external strain gradient (flexomagnetic effect). In particular, we describe the mechanism of the magnetization induction in the Mn_{3}GaN…

Materials Science · Physics 2009-09-11 Pavel Lukashev , Renat F. Sabirianov

Relaxor ferroelectrics, which can exhibit exceptional electromechanical coupling are some of the most important functional materials with applications ranging from ultrasound imaging to actuators and sensors in microelectromechanical…

Spatial variability of polarization relaxation kinetics in relaxor ferroelectric 0.9Pb(Mg1/3Nb2/3)O3-0.1PbTiO3 is studied using time-resolved Piezoresponse Force Microscopy. Local relaxation attributed to the reorientation of polar…

Materials Science · Physics 2013-05-29 S. V. Kalinin , B. J. Rodriguez , J. D. Budai , S. Jesse , A. N. Morozovska , A. A. Bokov , Z. -G. Ye