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Theoretical studies on M$_{13}$ (M = Fe, Co, Ni) and M$_{13}$Pt$_n$ (for $n$ = 3, 4, 5, 20) clusters including the spin-orbit coupling are done using density functional theory. The magnetic anisotropy energy (MAE) along with the spin and…

We report magnetocrystalline anisotropy of pure and Fe/Si substituted SmCo5. The calculations were performed using the advanced density functional theory (DFT) including onsite electron-electron correlation and spin orbit coupling. Si…

Materials Science · Physics 2019-12-10 Rajiv K. Chouhan , A. K. Pathak , D. Paudyal

The magnetic properties of Fe$_2$Ta and Fe$_2$W in the hexagonal Laves phase are computed using density functional theory in the generalised gradient approximation, with the full potential linearised augmented plane wave method. The alloy…

Materials Science · Physics 2017-08-23 Alexander Edström

Density functional theory (DFT), including its extensions designed to treat strongly correlated localized electron systems such as DFT+$U$ and DFT+dynamical mean field theory, has proven exceedingly useful in studying the magnetic…

Materials Science · Physics 2025-06-09 Y. Lee , Z. Ning , R. Flint , R. J. McQueeney , I. I. Mazin , Liqin Ke

In the disordered local moment picture, we calculated the magnetization (M) and magnetic anisotropy energy (MAE) of FePt, CoPt, and MnAl ordered alloys and body-centered tegragonal FeCo (bct-FeCo) disordered alloy, assuming spatially…

Materials Science · Physics 2016-10-12 Naofumi Kobayashi , Kazushige Hyodo , Akimasa Sakuma

We introduce an efficient finite-element approach for large-scale real-space pseudopotential density functional theory (DFT) calculations incorporating noncollinear magnetism and spin-orbit coupling. The approach, implemented within the…

Materials Science · Physics 2025-06-11 Nikhil Kodali , Phani Motamarri

The orbital contribution to the magnetic properties of Fe in systems of decreasing dimensionality (bulk, surfaces, wire and free clusters) is investigated using a tight-binding hamiltonian in an $s, p,$ and $d$ atomic orbital basis set…

Materials Science · Physics 2008-04-22 Marie-Catherine Desjonquères , Cyrille Barreteau , Gabriel Autes , Daniel Spanjaard

Magnetic axis rotation (MAR) in ferromagnetic (FM) layers is crucial for strain-mediated converse magnetoelectric coupling. Employing the density functional theory (DFT), we computationally study the magnetic anisotropy of selected deformed…

Materials Science · Physics 2022-12-02 Zefeng Cai , Ben Xu

Magnetocrystalline anisotropy in transition metal alloys (FePt, CoPt, FePd, MnAl, MnGa, and FeCo) was studied using first-principles calculations to elucidate its specific mechanism. The tight-binding linear muffin-tin orbital method in the…

Materials Science · Physics 2014-03-04 Yohei Kota , Akimasa Sakuma

Nd-Fe-B magnets are the most widely used high performance magnets in the world today, and remain the subject of both experimental and computational research aimed at understanding and optimizing them. Atomistic spin dynamics (ASD) is one…

Materials Science · Physics 2026-04-01 Veronica T. C. Lai , Christopher E. Patrick

The solution of the mean spherical approximation (MSA) integral equation for isotropic multicomponent dipolar hard sphere fluids without external fields is used to construct a density functional theory (DFT), which includes external fields,…

Statistical Mechanics · Physics 2015-05-28 I. Szalai , S. Dietrich

We present an investigation on the large magnetic anisotropy of Fe_{2}P, based on {\it Ab Initio} density-functional theory calculations, with a full potential linear muffin-tin orbital (FP-LMTO) basis. We obtain an uniaxial magnetic…

Ab-initio calculation of magnetocrystalline anisotropy energy (MCAE) often requires a strict convergence criterion and a dense k-point mesh to sample the Brillouin zone, making its convergence problematic and time-consuming. The force…

Mesoscale and Nanoscale Physics · Physics 2018-12-10 Junfeng Qiao , Weisheng Zhao

Uniaxially strained Fe--Co disordered alloys have emerged as promising candidates for cost-effective rare-earth-free permanent magnets due to their high magnetocrystalline anisotropy energy (MAE). Using first-principles, fully relativistic…

The development of quantitative models for radiation damage effects in iron, iron alloys and steels, particularly for the high temperature properties of the alloys, requires understanding of magnetic interactions, which control the phase…

Materials Science · Physics 2015-06-17 D. Nguyen-Manh , Pui-Wai Ma , M. Yu. Lavrentiev , S. L. Dudarev

Magnetocrystalline anisotropy, a crucial factor in magnetic properties and applications like magnetoresistive random-access memory, often requires extensive $k$-point mesh in first-principles calculations. In this study, we develop a…

Materials Science · Physics 2025-02-18 Hiroto Saito , Takashi Koretsune

We have investigated crystalline magnetic anisotropy in the electric field (EF) for the Fe-Pt surface which have a large perpendicular anisotropy, by means of the first-principles approach. The anisotropy is reduced linearly with respect to…

Materials Science · Physics 2015-05-13 Masahito Tsujikawa , Tatsuki Oda

Density functional theory (DFT) has long struggled to treat light rare-earth magnetism. We show that this difficulty arises from an overestimate of the $4f$ charge asphericity, and thus the magnetic anisotropy energy, due to the inadequacy…

Materials Science · Physics 2025-08-28 Liqin Ke , R. Flint , Y. Lee

Multi-configurational wave-function theory (MC-WFT) that combines complete active space self-consistent field (CASSCF) approach with subsequent state interaction (SI) treatment of spin-orbit coupling (SOC), abbreviated as CASSCF-SO, plays…

Chemical Physics · Physics 2025-03-11 Zhe-Bin Guan , Hong Jiang

The nature of low-impurity ferromagnetism remains a challenging problem in the solid-state community due to the strong dependence of magnetic properties on composition, concentration, and structural geometry of diluted alloys. To address…