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A novel and universal interference structure is found in the photoelectron momentum distribution of atoms in intense infrared laser field. Theoretical analysis shows that this structure can be attributed to a new form of…

The observation of the time delay between the soft emission and the high-energy radiation from cosmological gamma ray bursts can be used as an important observational test of multi-dimensional physical theories. The main source of the time…

Astrophysics · Physics 2014-10-13 T. Harko , K. S. Cheng

For photo-dissociation of a single hydrogen molecule (H2) with combined XUV and IR laser pulses, we demonstrate optical control of the emission direction of the photoelectron with respect to the outgoing neutral fragment (the H-atom).…

The evolution of electron wavepackets determines the course of many physical and chemical phenomena and attosecond spectroscopy aims to measure and control such dynamics in real-time. Here, we investigate radial electron wavepacket motion…

Atomic Physics · Physics 2015-09-04 Niranjan Shivaram , Xiao-Min Tong , Henry Timmers , Arvinder Sandhu

A Kohn-Sham time-dependent local-density-functional scheme is utilized to predict attosecond time delays of xenon 4d photoionization that involves the 4d giant dipole resonance and Cooper minimum. The fundamental effect of electron…

Atomic Physics · Physics 2021-06-08 Maia Magrakvelidze , Mohamed El-Amine Madjet , Himadri S. Chakraborty

Recent advances in attosecond spectroscopy techniques have fueled the interest in the theoretical description of electronic processes taking place in the subfemtosecond time scale. Here we study the coupled dynamic screening of a localized…

Atomic and Molecular Clusters · Physics 2013-01-28 N. E. Koval , D. Sánchez-Portal , A. G. Borisov , R. Díez Muiño

We demonstrate a compact, spectrally-selective, and tunable delay line for single photons emitted by quantum dots. This is achieved by fine-tuning the wavelength of the optical transitions of such "artificial atoms" into a spectral window…

Mesoscale and Nanoscale Physics · Physics 2015-12-30 Johannes S. Wildmann , Rinaldo Trotta , Javier Martín-Sánchez , Eugenio Zallo , Oliver G. Schmidt , Armando Rastelli

Electrons photoemitted by extreme ultraviolet attosecond pulses derive spatially from the first few atomic surface layers and energetically from the valence band and highest atomic orbitals. As a result, it is possible to probe the emission…

Ultrafast processes in matter, such as the electron emission following light absorption, can now be studied using ultrashort light pulses of attosecond duration ($10^{-18}$s) in the extreme ultraviolet spectral range. The lack of spectral…

We propose angle-resolved photoelectron spectroscopy of aerosol particles as an alternative way to determine the electron mean free path of low energy electrons in solid and liquid materials. The mean free path is obtained from fits of…

Two emerging areas of research, attosecond and nanoscale physics, have recently started to merge. Attosecond physics deals with phenomena occurring when ultrashort laser pulses, with duration on the femto- and sub-femtosecond time scales,…

Atomic Physics · Physics 2019-12-03 Marcelo F. Ciappina , Maciej Lewenstein

In this Letter, we investigate the non-dipole effects in time delay of photoelectrons emitted by multi-electron atoms, negative ions, and respective endohedrals. We present the necessary general formulas in the frame of the random phase…

Atomic Physics · Physics 2020-12-02 M. Ya. Amusia , L. V. Chernysheva

Numerical simulations are presented to validate the possible use of cutting-edge attosecond time- resolved photoelectron spectroscopy to observe in real time the creation of an electronic wavepacket and subsequent electronic motion in a…

Atomic and Molecular Clusters · Physics 2015-06-22 Aurelie Perveaux , David Lauvergnat , Fabien Gatti , Gabor Halasz , Agnes Vibok , Benjamin Lasorne

We study a quantum electrodynamics (QED) system made of an two-level atom and a semi-infinite rectangular waveguide, which behaves as a perfect mirror in one end. The spatial dependence of the atomic spontaneous emission has been included…

Quantum Physics · Physics 2017-03-27 Hai-Xi Song , Xiao-Qi Sun , Jing Lu , Lan Zhou

Attosecond science is based on steering of electrons with the electric field of well-controlled femtosecond laser pulses. It has led to, for example, the generation of XUV light pulses with a duration in the sub-100-attosecond regime, to…

Quantum Physics · Physics 2011-07-11 Michael Krüger , Markus Schenk , Peter Hommelhoff

The route towards manipulation of the optoelectronic properties of matter beyond the current limits of electronics starts from a comprehensive study of the ultrafast dynamics triggered by interaction with light. Among them, a fundamental…

We have performed calculations of attosecond laser-atom interactions for laser intensities where interesting two and three photon effects become relevant. In particular, we examine the case of "hole burning" in the initial orbital. Hole…

Atomic Physics · Physics 2014-06-02 P. L. Price , L. D. Noordam , H. B. van Linden van den Heuvell , F. Robicheaux

The effect of the absorption of hard X-ray photons on the solid-state dynamics, at energies below the defect creation threshold, is considered. First, it is shown that due to the sensitivity to parameter choices, the present state of the…

Materials Science · Physics 2015-10-08 Michael Leitner , Markus Stana , Manuel Ross , Bogdan Sepiol

Attosecond science has been transforming our understanding of electron dynamics in atoms, molecules and solids. However, to date almost all of the attoscience experiments have been based on spectroscopic measurements because attosecond…

Measuring the time it takes to remove an electron from an atom or molecule during photoionization using newly developed attosecond spectroscopies has been a focus of many recent experiments. However, the outcome of such measurement depends…

Atomic Physics · Physics 2017-03-08 Lisa Torlina , Olga Smirnova
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