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Solid-state quantum emitters that couple coherent optical transitions to long-lived spin qubits are essential for quantum networks. Here we report on the spin and optical properties of individual tin-vacancy (SnV) centers in diamond…

The unique combination of outstanding optical quality and attractive spin properties opens new avenues for optical spin control in hybrid organic-inorganic perovskite semiconductors. Using the optically detected magnetic resonance…

Mesoscale and Nanoscale Physics · Physics 2026-04-09 Rongrong Hu , Sergey R. Meliakov , Dmitri R. Yakovlev , Bekir Turedi , Maksym V. Kovalenko , Manfred Bayer , Vasilii V. Belykh

Nanodiamonds containing negatively charged nitrogen vacancy centres (${\text{NV}}^{-}$) have applications as localized sensors in biological material and have been proposed as a platform to probe the macroscopic limits of spatial…

Optically interfaced solid-state defects are promising candidates for quantum communication technologies. The ideal defect system would feature bright telecom emission, long-lived spin states, and a scalable material platform,…

We examine the quantum spin state of a single nitrogen-vacancy (NV) center in diamond at room temperature as it makes a transition from the orbital ground-state (GS) to the orbital excited-state (ES) during non-resonant optical excitation.…

Quantum Physics · Physics 2015-06-03 G. D. Fuchs , A. L. Falk , V. V. Dobrovitski , D. D. Awschalom

Silicon is undoubtedly one of the most promising semiconductor materials for spin-based information processing devices. Its highly advanced fabrication technology facilitates the transition from individual devices to large-scale processors,…

Optically active defects in solids with accessible spin states are promising candidates for solid state quantum information and sensing applications. To employ these defects as quantum building blocks, coherent manipulation of their spin…

We probe the relaxation dynamics of the full three-level spin system of near-surface nitrogen-vacancy (NV) centers in diamond to define a $T_{1}$ relaxation time that helps resolve the $T_{2} \leq 2T_{1}$ coherence limit of the NV's subset…

Mesoscale and Nanoscale Physics · Physics 2017-05-17 Bryan A. Myers , Amila Ariyaratne , Ania C. Bleszynski Jayich

The ability to process and store information on surrounding nuclear spins is a major requirement for group-IV color center-based repeater nodes. We demonstrate coherent control of a ${}^{13}$C nuclear spin strongly coupled to a negatively…

We report theoretical and experimental studies of the longitudinal electron spin and orbital relaxation time of interstitial Li donors in $^{28}$Si. We predict that despite the near-degeneracy of the ground-state manifold the spin…

Other Condensed Matter · Physics 2008-07-25 V. N. Smelyanskiy , A. G. Petukhov , A. M. Tyryshkin , S. A. Lyon , T. Schenkel , J. W. Ager , E. E. Haller

Quantum sensing with spin defects in diamond, such as the nitrogen-vacancy (NV) center, enables the detection of various chemical species on the nanoscale. Molecules or ions with unpaired electronic spins are typically probed by their…

Nitrogen-vacancy centres (NVs) in diamond are attractive for research straddling quantum information science and nanoscale magnetometry and thermometry. While ultrapure bulk diamond NVs sustain the longest spin coherence times among…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 Helena S. Knowles , Dhiren M. Kara , Mete Atature

Optically accessible solid state defect spins serve as a primary platform for quantum information processing, where precise control of the electron spin and ancillary nuclear spins is essential for operation. Using the nitrogen-vacancy (NV)…

Quantum Physics · Physics 2026-02-12 Gergő Thiering , Adam Gali

Nanodiamonds (NDs) hosting nitrogen-vacancy (NV) centers are promising for applications of quantum sensing. Long spin relaxation times ($T_1$ and $T_2$) are critical for high sensitivity in quantum applications. It has been shown that…

Mesoscale and Nanoscale Physics · Physics 2020-08-11 Zaili Peng , Jax Dallas , Susumu Takahashi

We present a theoretical analysis of the electron spin decoherence in single Nitrogen-Vacancy defects in ultra-pure diamond. The electron spin decoherence is due to the interactions with Carbon-13 nuclear spins in the diamond lattice. Our…

Other Condensed Matter · Physics 2009-11-13 J. R. Maze , J. M. Taylor , M. D. Lukin

We report on room-temperature coherent manipulation of the spin of a single nitrogen-vacancy center in diamond and a study of its coherence as a function of magnetic field. We use magnetic resonance to induce Rabi nutations, and apply a…

Quantum Physics · Physics 2007-05-23 R. Hanson , O. Gywat , D. D. Awschalom

Quantum memories provide intermediate storage of quantum information until it is needed for the next step of a quantum algorithm or a quantum communication process. Relevant figures of merit are therefore the fidelity with which the…

Quantum Physics · Physics 2013-01-04 J. H. Shim , I. Niemeyer , J. Zhang , D. Suter

Spin relaxometry using solid-state spin defects, such as the diamond nitrogen-vacancy (NV) center, probes dynamical processes by measuring how environmental fluctuations enhance the spin relaxation rate. In the weak-coupling limit,…

Mesoscale and Nanoscale Physics · Physics 2026-02-03 Ruotian Gong , Alex L. Melendez , Guanghui He , Zhongyuan Liu , Chong Zu , Huan Zhao

We perform pulsed optically detected electron spin resonance to measure the DC magnetic field sensitivity and electronic spin coherence time T_2 of an ensemble of near-surface, high-density nitrogen-vacancy (NV) centers engineered to have a…

Mesoscale and Nanoscale Physics · Physics 2017-05-11 Kento Sasaki , Ed E. Kleinsasser , Zhouyang Zhu , Wen-Di Li , Hideyuki Watanabe , Kai-Mei C. Fu , Kohei M. Itoh , Eisuke Abe

We study the spin and orbital dynamics of single nitrogen-vacancy (NV) centers in diamond between room temperature and 700 K. We find that the ability to optically address and coherently control single spins above room temperature is…

Mesoscale and Nanoscale Physics · Physics 2012-07-18 D. M. Toyli , D. J. Christle , A. Alkauskas , B. B. Buckley , C. G. Van de Walle , D. D. Awschalom