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VOCl and other transition metal oxychlorides are candidate materials for next-generation rechargeable batteries. We have investigated the influence of the underlying magnetic order on the crystallographic and electronic structure by means…

Materials Science · Physics 2019-09-04 Marcus Ekholm , Andreas Schönleber , Sander van Smaalen

Iron-based superconductor Sr$_2$VFeAsO$_3$ is composed of alternate stacking of a superconducting FeAs layer and an insulating vanadium-oxide layer with a perovskite-type structure. Electronic orders stemming from the spin and orbital…

Electron interactions can drive magnetism, superconductivity, and topology. However, the realization of these phases remains limited in van der Waals materials, and the full landscape of strong correlations remains uncharted in any context.…

Ferromagnetism and superconductivity are two key ingredients to create non-Abelian quasiparticle excitations that are expected as building blocks to construct topological quantum computers. Adversely, ferromagnetism and superconductivity…

Van der Waals heterostructures are a core tool in quantum material design. The recent addition of monolayer ferroelectrics expands the possibilities of designer materials. Ferroelectric domains can be manipulated using electric fields, thus…

Fundamental block and staggered orders of magnetic Fe multipoles in Na2FeSe2 are classified by their symmetry and magnetoelectric properties. Our structure model incorporates ferromagnetic or antiferromagnetic coupling between chains. The…

Strongly Correlated Electrons · Physics 2021-04-28 S. W. Lovesey , D. D. Khalyavin

Mn$_3$Si$_2$Te$_6$ is a rare example of a layered ferrimagnet. It has recently been shown to host a colossal angular magnetoresistance as the spin orientation is rotated from the in- to out-of-plane direction, proposed to be underpinned by…

A grand challenge of nanoscience is to master the control of structure and properties in order to go beyond present day functionality. The creation of nanostructures via atom manipulation by means of a scanning probe represents one of the…

Mesoscale and Nanoscale Physics · Physics 2012-09-11 R. X. Cao , B. F. Miao , Z. F. Zhong , L. Sun , B. You , W. Zhang , D. Wu , An Hu , S. D. Bader , H. F. Ding

Iron-chalcogenide superconductors display rich phenomena caused by orbital-dependent band shifts and electronic correlations. Additionally, they are potential candidates for topological superconductivity due to the band inversion between…

We report on the recovery of the short-range static magnetic order and on the concomitant degradation of the superconducting state in optimally F-doped SmFe_(1-x)Ru_(x)AsO_0.85F_0.15 for 0.1< x<0.6. The two reduced order parameters coexist…

Superconductivity · Physics 2015-06-03 S. Sanna , P. Carretta , P. Bonfà , G. Prando , G. Allodi , R. De Renzi , T. Shiroka , G. Lamura , A. Martinelli , M. Putti

We study a spin $S$ quantum Heisenberg model on the Fe lattice of the rare-earth oxypnictide superconductors. Using both large $S$ and large $N$ methods, we show that this model exhibits a sequence of two phase transitions: from a high…

Strongly Correlated Electrons · Physics 2009-11-13 Chen Fang , Hong Yao , Wei-Feng Tsai , JiangPing Hu , Steven A. Kivelson

Orbital-selective correlations have been observed to play an important role in Fe-based superconductors. Here, in contrast to previous site-local Mott transition-based origins, we present a band-theory-based mechanism for orbital-selective…

Strongly Correlated Electrons · Physics 2025-09-09 Mercè Roig , Qiang Zou , Basu Dev Oli , Tatsuya Shishidou , Yue Yu , Huimin Zhang , Daniel F. Agterberg , Lian Li , Michael Weinert

We describe here a theory of a quantum dot in an electrically tunable MoSe$_2$/WSe$_2$ heterostructure. Van der Waals heterostructures allow for tuning their electronic properties beyond their monolayer counterparts. We start by determining…

Mesoscale and Nanoscale Physics · Physics 2024-12-23 Katarzyna Sadecka , Maciej Bieniek , Paulo E. Faria Junior , Arkadiusz Wójs , Paweł Hawrylak , Jarosław Pawłowski

Employing aberration-corrected scanning transmission electron microscopy (STEM), we meticulously investigated the intrinsic chemical heterogeneity of Fe1+yTe, Fe1+yTe0.8Se0.2, and Fe1+yTe0.5Se0.5. Comprehensive analysis reveals the presence…

The alignment of the frontier orbital energies of an adsorbed molecule with the substrate Fermi level at metal-organic interfaces is a fundamental observable of significant practical importance in nanoscience and beyond. Typical density…

Mesoscale and Nanoscale Physics · Physics 2017-03-07 Zhenfei Liu , David A. Egger , Sivan Refaely-Abramson , Leeor Kronik , Jeffrey B. Neaton

Isoelectronic substitution is an ideal tuning parameter to alter electronic states and correlations in iron-based superconductors. As this substitution takes place outside the conducting Fe planes, the electronic behaviour is less affected…

Superconductivity · Physics 2021-05-25 Amalia I. Coldea

We performed Se and F-NMR measurements on single crystals of (TMTSF)2FSO3 to characterize the electronic structures of different phases in the Temperature-Pressure phase diagram, determined by precise transport measurements [Jo et al.,…

Strongly Correlated Electrons · Physics 2016-11-23 Hidetaka Satsukawa , Akio Yajima , Ko-ichi Hiraki , Toshihiro Takahashi , Haeyong Kang , Younjung Jo , Woun Kang , Ok-Hee Chung

We use soft x-ray vector-ptychographic tomography to determine the three-dimensional magnetization field in superparamagnetic nanoparticles self-assembled at the liquid-liquid interface and reveal the magnetic order induced by layered…

Understanding the interplay between nematicity, magnetism and superconductivity is pivotal for elucidating the physics of iron-based superconductors. Here we use neutron scattering to probe magnetic and nematic orders throughout the phase…

The charge ordered La$_{1/3}$Sr$_{2/3}$FeO$_{3-\delta}$ (LSFO) in bulk and nanocrystalline forms are investigated using ac and dc magnetization, M\"{o}ssbauer, and polarised neutron studies. A complex scenario of short range charge and…

Materials Science · Physics 2013-10-01 Sk. Sabyasachi , M. Patra , S. Majumdar , S. Giri , S. Das , V. S. Amaral , O. Iglesias , W. Borghols , T. Chatterji
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