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Measurements of spin dynamics of electrons in a degenerate two dimensional electron gas, where the Dyakonov-Perel mechanism is dominant, have been used to investigate the electron scattering time (tp*) as a function of energy near the Fermi…

Other Condensed Matter · Physics 2008-03-11 W. J. H. Leylanda , R. T. Harley , M. Henini , A. J. Shields , I. Farrer , D. A. Ritchie

Molecular aggregates on plasmonic nanoparticles have emerged as attractive systems for the studies of cavity quantum electrodynamics. They are highly tunable, scalable, easy to synthesize and offer sub-wavelength confinement, all while…

Electron hydrodynamics arises when momentum-relaxing scattering processes are slow compared to momentum-conserving ones. While the microscopic details necessary to satisfy this condition are material-specific, experimentally accessible…

Materials Science · Physics 2022-04-14 Georgios Varnavides , Adam S. Jermyn , Polina Anikeeva , Prineha Narang

It was recently shown [Y. Suzuki, L. Lacombe, K. Watanabe, and N. T. Maitra, Phys. Rev. Lett. 119, 263401 (2017)] that peak and valley structures in the exact exchange-correlation potential of time-dependent density functional theory are…

Chemical Physics · Physics 2018-07-04 Lionel Lacombe , Yasumitsu Suzuki , Kazuyuki Watanabe , Neepa T. Maitra

We investigate the impact of dissipation on the energy balance in the electron dynamics of metal clusters excited by strong electro-magnetic pulses. The dynamics is described theoretically by Time-Dependent Density-Functional Theory (TDDFT)…

Mesoscale and Nanoscale Physics · Physics 2017-02-01 M. Vincedon , E. Suraud , P. -G. Reinhard

Surface plasmon mediated hot carrier generation is widely utilized for the manipulation of the electron-photon interactions in many types of optoelectronic devices including solar cells, photodiodes, and optical modulators. A diversity of…

Nonequilibrium dynamics governed by electron-phonon (e-ph) interactions plays a key role in electronic devices and spectroscopies and is central to understanding electronic excitations in materials. The real-time Boltzmann transport…

Materials Science · Physics 2023-11-14 Ivan Maliyov , Jia Yin , Jia Yao , Chao Yang , Marco Bernardi

During the last decade, significant progress has been achieved in the rapidly growing field of the dynamics of {\it hot} carriers in metals. Here we present an overview of the recent achievements in the theoretical understanding of electron…

Materials Science · Physics 2007-05-23 J. M. Pitarke , V. P. Zhukov , R. Keyling , E. V. Chulkov , P. M. Echenique

To investigate inelastic electron scattering, which is ubiquitous in various fields of study, we carry out ab initio study of the real-time dynamics of a one-dimensional electron wave packet scattered by a hydrogen atom using different…

Atomic Physics · Physics 2020-06-24 Yeonghun Lee , Xiaolong Yao , Massimo V. Fischetti , Kyeongjae Cho

We present a real-time investigation of ultrafast carrier dynamics in single-wall carbon nanotube bundles using femtosecond time-resolved photoelectron spectroscopy. The experiments allow to study the processes governing the subpicosecond…

Materials Science · Physics 2009-11-07 Tobias Hertel , Roman Fasel , Gunnar Moos

We develop a semiclassical kinetic theory for electron spin relaxation in semiconductors. Our approach accounts for elastic as well as inelastic scattering and treats Elliott-Yafet and motional-narrowing processes, such as D'yakonov-Perel'…

Materials Science · Physics 2009-11-10 Franz X. Bronold , Avadh Saxena , Darryl L. Smith

Understanding ion relaxation dynamics in overlapping electric double layers (EDLs) is critical for the development of efficient nanotechnology based electrochemical energy storage, electrochemomechanical energy conversion and…

Chemical Physics · Physics 2014-11-04 Vaibhav Thakore , James J. Hickman

The ability to manipulate plasmons is driving new developments in electronics, optics, sensing, energy, and medicine. Despite the massive momentum of experimental research in this direction, a predictive quantum-mechanical framework for…

Materials Science · Physics 2016-10-12 Fabio Caruso , Feliciano Giustino

Employing time-resolved photoelectron spectroscopy we analyze the relaxation dynamics of hot electrons in the charge density wave / Mott material 1T-TaS_2. At 1.2 eV above the Fermi level we observe a hot electron lifetime of 12 +- 5 fs in…

Strongly Correlated Electrons · Physics 2020-07-01 Isabella Avigo , Friedemann Queisser , Ping Zhou , Manuel Ligges , Kai Rossnagel , Ralf Schützhold , Uwe Bovensiepen

Low-energy electrons scattered in the conduction band of a dielectric solid should behave like Bloch electrons and will interact with perturbations of the atomic lattice, i.e. with phonons. Thus the phonon-based description of low-energy…

Materials Science · Physics 2009-11-13 Hans-Joachim Fitting , Vsevolod S. Kortov , Guillaume Petite

We report extensive all-electron time-dependent density-functional calculations and nonresonant inelastic x-ray scattering measurements of the dynamical structure factor of 3d transition metals. For small wave vectors, a plasmon peak is…

In this paper we describe an ultrafast scanning electron microscope setup developed for the research of inelastic scattering of electrons at optical near-fields of periodic dielectric nanostructures. Electron emission from the Schottky…

Applied Physics · Physics 2018-08-01 M. Kozák , J. McNeur , N. Schönenberger , J. Illmer , A. Li , A. Tafel , P. Yousefi , T. Eckstein , P. Hommelhoff

The description of electron-electron scattering presents challenges in the microscopic modeling of the interaction of ultrashort intense laser pulses with solids. We extend the semiclassical approach based on the Vlasov equation [Phys. Rev.…

Plasma Physics · Physics 2025-02-06 Mizuki Tani , Tomohito Otobe , Yasushi Shinohara , Kenichi L. Ishikawa

Presence of a metal nanoparticle near a quantum dipole emitter, when a localized surface plasmon mode is excited via the resonant coupling with an excited quantum dipole, changes dramatically the relaxation dynamics: it is no longer…

Optics · Physics 2015-06-18 Khachatur V. Nerkararyan , Sergey I. Bozhevolnyi

We analyze theoretically the demagnetization dynamics in a ferromagnetic model system due to the interplay of spin-orbit coupling and electron-electron Coulomb scattering. We compute the $k$-resolved electronic reduced spin-density matrix…

Materials Science · Physics 2022-08-05 Svenja Vollmar , Kai Leckron , Hans Christian Schneider