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We analyse the influence of optically generated non-equilibrium phonons on the spin relaxation and effective spin temperature of an individual Cr atom inserted in a quantum dot. Using a three pulses pump-probe technique, we show that the…

Mesoscale and Nanoscale Physics · Physics 2020-02-05 V. Tiwari , K. Makita , M. Arino , M. Morita , S. Kuroda , H. Boukari , L. Besombes

A theoretical approach to the influence of one-dimensional lattice fluctuations on electronic properties in weakly localized spin-Peierls systems is proposed using the renormalization group and the functional integral techniques. The…

Condensed Matter · Physics 2009-10-28 Claude Bourbonnais , Benoit Dumoulin

We investigate the fundamental mechanism of spin phonon coupling in the negatively charged nitrogen vacancy center $(\mathrm{NV}^-)$ in diamond in order to calculate the spin lattice relaxation time $T_1$ and its temperature dependence from…

Mesoscale and Nanoscale Physics · Physics 2018-12-31 Johannes Gugler , Thomas Astner , Andreas Angerer , Jörg Schmiedmayer , Johannes Majer , Peter Mohn

We investigate transition rates between different spin configurations for $S \ge 1$ spins weakly coupled to a $d$-dimensional phonon bath. This study is motivated by understanding observed magnetization relaxation as a function of…

Materials Science · Physics 2009-11-13 Kyungwha Park

Magnetic resonance is a prime method for the study of chemical and biological structures and their dynamical processes. The interpretation of these experiments relies on considering the spin of electrons as the sole relevant degree of…

Fe3GeTe2 has emerged as one of the most fascinating van der Waals crystals due to its two-dimensional (2D) itinerant ferromagnetism, topological nodal lines and Kondo lattice behavior. However, lattice dynamics, chirality of phonons and…

Electronic spin superposition states enable nanoscale sensing through their sensitivity to the local environment, yet their sensitivity to vibrational motion also limits their coherence times. In molecular spin systems, chemical tunability…

Quantum Physics · Physics 2026-02-04 Stefan H. Lohaus , Kay T. Xia , Yongqiang Cheng , Ryan G. Hadt

Fermi's golden rule (FGR) offers an empirical framework for understanding the dynamics of spin-lattice relaxation in magnetic molecules, encompassing mechanisms like direct (one-phonon) and Raman (two-phonon) processes. These principles…

Chemical Physics · Physics 2024-07-23 Rui-Hao Bi , Yu Su , Yao Wang , Lei Sun , Wenjie Dou

We derive a simple system of equations to describe the magnetization relaxation of a molecular spin in weak interaction with a thermal bath for the whole temperature domain. Using this for the intermediate temperature domain where the…

Materials Science · Physics 2022-12-27 Le Tuan Anh Ho , Liviu Ungur , Liviu F. Chibotaru

The physics of interacting nuclear spins arranged in a crystalline lattice is typically described using a thermodynamic framework: a variety of experimental studies in bulk solid-state systems have proven the concept of a spin temperature…

Mesoscale and Nanoscale Physics · Physics 2009-07-21 P. Maletinsky , M. Kroner , A. Imamoglu

In this article, we report negative thermal expansion and spin frustration in hexagonal GdInO$_{3}$. Rietveld refinement of the XRD patterns reveal that the negative thermal expansion in the temperature range of 50-100K stems from the…

Materials Science · Physics 2017-02-15 Barnita Paul , Swastika Chatterjee , Anushree Roy , A. Midya , P. Mandal , Vinita Grover , A. K. Tyagi

We study spin-lattice relaxation times of electron spins in Er$^{3+}$:CaWO$_4$ at millikelvin temperature, detected via their coupling to a low-mode volume superconducting resonator. At large magnetic field supporting strong phonon-emission…

High degree of preservation of spin states during energy relaxation processes mediated by optical phonons is demonstrated in a single quantum dot. Optical-phonon resonance and relevant suppression of spin relaxation are clearly identified…

Materials Science · Physics 2013-05-29 H. Kumano , H. Kobayashi , S. Ekuni , Y. Hayashi , M. Jo , H. Sasakura , S. Adachi , S. Muto , I. Suemune

Magnetic relaxation in coordination compounds is largely dominated by the interaction of the spin with phonons. Large zero-field splitting and exchange coupling values have been empirically found to strongly suppress spin relaxation and…

Electron spin relaxation due to the D'yakonov-Perel' mechanism is investigated in bilayer graphene with only the lowest conduction band being relevant. The spin-orbit coupling is constructed from the symmetry group analysis with the…

Mesoscale and Nanoscale Physics · Physics 2013-05-14 L. Wang , M. W. Wu

The spin-1/2 Ising model with a spin-phonon coupling on decorated planar lattices partially amenable to lattice vibrations is examined within the framework of the generalized decoration-iteration transformation and the harmonic…

Statistical Mechanics · Physics 2015-05-30 Jozef Strecka , Onofre Rojas , Sergio Martins de Souza

We investigate the emergence of an astonishingly long pre-thermal plateau in a classical phonon field, here a harmonic chain with on-site pinning. Integrability is broken by a weak anharmonic on-site potential with strength $\lambda$. In…

Statistical Mechanics · Physics 2020-05-13 François Huveneers , Jani Lukkarinen

We use inelastic neutron scattering to study acoustic phonons and spin excitations in single crystals of NaFeAs, a parent compound of iron pnictide superconductors. NaFeAs exhibits a tetragonal-to-orthorhombic structural transition at…

We demonstrate a bipartition technique using a super-lattice architecture to access correlations between alternating planes of a mesoscopic array of spin-3 chromium atoms trapped in a 3D optical lattice. Using this method, we observe that…

The lattice dynamic properties and spin-phonon coupling in DyMn$_2$O$_5$ are studied by using the density-functional theory. The calculated phonon frequencies are in very good agreement with experiments. We then compare the phonon modes…

Materials Science · Physics 2009-11-13 Tianqi Shen , Kun Cao , Guang-Can Guo , Lixin He