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Ionic structure of high pressure, high temperature fluids is a challenging theoretical problem with applications to planetary interiors and fusion capsules. Here we report a multi-messenger platform using velocimetry and \textit{in situ}…

We present results of an investigation into the formation of nitrogen-bearing molecules in the atmosphere of Titan. We extend a previous model (Li et al. 2015, 2016) to cover the region below the tropopause, so the new model treats the…

Earth and Planetary Astrophysics · Physics 2016-10-05 Karen Willacy , Mark Allen , Yuk Yung

We present measurements on Fe$_2$O$_3$ amorphization and melt under laser-driven shock compression up to 209(10) GPa via time-resolved in situ x-ray diffraction. At 122(3) GPa, a diffuse signal is observed indicating the presence of a…

A combination of quantum mechanics calculations with machine learning (ML) techniques can lead to a paradigm shift in our ability to predict materials properties from first principles. Here we show that on-the-fly training of an interatomic…

The thermodynamic behavior of calcium oxide (\ce{CaO}) under high temperature and pressure conditions is critical for understanding the physics of planetary interiors. This study employs molecular dynamics (MD) simulations, including both…

Materials Science · Physics 2024-12-10 Francesca Menescardi , Davide Ceresoli , Donato Belmonte

Boron phosphide (BP) is a (super)hard semiconductor constituted of light elements, which is promising for high demand applications at extreme conditions. The behavior of BP at high temperatures and pressures is of special interest but is…

It is challenging to search for high Tc superconductivity (SC) in transition metal elements wherein d electrons are usually not favored by conventional BCS theory. Here we report discovery of surprising SC up to 310 GPa with Tc above 20 K…

The measurement of superconductivity at above 200K in compressed samples of hydrogen sulfide and lanthanum hydride at 250K is reinvigorating the search for conventional high temperature superconductors. At the same time it exposes a…

Superconductivity · Physics 2019-10-02 Chris J. Pickard , Ion Errea , Mikhail I. Eremets

We introduce a novel method that combines the accuracy of Quantum Monte Carlo simulations with ab-initio Molecular Dynamics, in the spirit of Car-Parrinello. This method is then used for investigating the structure of a two-dimensional…

Computational Physics · Physics 2017-05-16 Francesco Calcavecchia , Thomas D. Kühne , Markus Holzmann

The high pressure(P)-high temperature(T) phase diagram of solid ammonia has been investigated using diamond anvil cell and resistive heating techniques. The III-IV transition line has been determined up to 20 GPa and 500 K both on…

Materials Science · Physics 2009-11-13 Sandra Ninet , Frédéric Datchi

Compared to the widely investigated crystalline polymorphs of gallium oxide (Ga2O3), knowledge about its amorphous state is still limited. With the help of a machine-learning interatomic potential, we conducted large-scale atomistic…

Materials Science · Physics 2024-04-29 Jiahui Zhang , Junlei Zhao , Jesper Byggmästar , Erkka J. Frankberg , Antti Kuronen

A constant supply of oxygen has been assumed to be necessary for the growth of titanium nanoparticles by sputtering. This oxygen supply can arise from a high background pressure in the vacuum system or from a purposely supplied gas. The…

Materials Science · Physics 2018-10-17 Rickard Gunnarsson , Nils Brenning , Robert Deric Boyd , Ulf Helmersson

The thermodynamic parameters of the superconducting state in Calcium under the pressure at 200 GPa have been determined. The numerical analysis by using the Eliashberg equations in the mixed representation has been conducted. It has been…

Superconductivity · Physics 2012-06-27 R. Szczęśniak , A. P. Durajski

Results solving the long standing puzzle regarding the phase diagram and the pressure evolution of the melting temperature Tm(P) of gallium nitride (GaN), the most promising semiconducting material for innovative modern electronic…

The phase stability and transformation between hexagonal close-packed (hcp) {\alpha}-phase and body-centered cubic (bcc) \b{eta}-phase in titanium (Ti) alloys are critical to their mechanical properties and manufacturing processes for…

Materials Science · Physics 2025-05-06 Huicong Chen , Chenwei Shao , Zhuocheng Xie , Jun Song , Yu Zou

We describe measurements demonstrating laser cooling of an atomic gas by means of collisional redistribution of radiation. The experiment uses rubidium atoms in the presence of several hundred bar of argon buffer gas pressure. Frequent…

Atomic Physics · Physics 2012-01-04 Ulrich Vogl , Anne Saß , Simon Haßelmann , Martin Weitz

It is generally assumed that solid hydrogen will transform into a metallic alkali-like crystal at sufficiently high pressure. However, some theoretical models have also suggested that compressed hydrogen may form an unusual two-component…

Materials Science · Physics 2009-11-10 Stanimir A. Bonev , Eric Schwegler , Tadashi Ogitsu , Giulia Galli

Dynamic compression has been used to synthesize liquid metallic hydrogen at 140 GPa (1.4 million bar) and experimental data and theory predict Al2O3 might be a metallic glass at ~300 GPa. The mechanism of metallization in both cases is…

Disordered Systems and Neural Networks · Physics 2015-05-20 W. J. Nellis

We used by in-situ high energy X-ray diffraction to inestigate the deformation behavior of Grade 2 commercially pure titanium that was hydrogen charged to form hydrides. The results showed that the peak broadening in the diffraction…

Materials Science · Physics 2022-01-26 Qing Tan , Zhiran Yan , Runguang Li , Yang Ren , Yandong Wang , Baptiste Gault , Stoichko Antonov

Based on ab initio calculations and metadynamics simulations, we predict that 2H-MoS$_2$, a layered insulator, will metallize under pressures in excess of 20-30 GPa. In the same pressure range, simulations and enthalpy optimization predict…

Materials Science · Physics 2015-06-12 Liliana Hromadová , Roman Martoňák , Erio Tosatti