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A prototypical quasi-2D metallic compound, 1T-TaS_2 has been extensively studied due to an intricate interplay between a Mott-insulating ground state and a charge density-wave (CDW) order. In the low-temperature phase, 12 out of 13 Ta_{4+}…

Strongly Correlated Electrons · Physics 2017-09-29 Marie Kratochvilova , Adrian D. Hillier , Andrew R. Wildes , Lihai Wang , Sang-Wook Cheong , Je-Geun Park

The possibility of the strong electron-electron interaction driven insulating phase from the metallic phase in two-dimensions has been suggested for clean systems without intentional disorder, but its rigorous demonstration is still…

Strongly Correlated Electrons · Physics 2021-01-04 Byoung Hee Moon , Gang Hee Han , Miloš M. Radonjić , Hyunjin Ji , Vladimir Dobrosavljević

A new type of disorder-driven electronic percolation transition is found for two-dimensional electron gas (2DEG), based on a quantum cellular automaton model. This transition is shown to be accompanied with a metal-insulator transition, as…

Statistical Mechanics · Physics 2018-10-17 M. N. Najafi

Recent demonstrations of controlled switching between different ordered macroscopic states by impulsive electromagnetic perturbations in complex materials have opened some fundamental questions on the mechanisms responsible for such…

Mesoscale and Nanoscale Physics · Physics 2016-03-22 Damjan Svetin , Igor Vaskivskyi , Serguei Brazovskii , Dragan Mihailovic

Metal-insulator transitions in clean, crystalline solids can be driven by two distinct mechanisms. In a conventional insulator, the charge carrier concentration vanishes, when an energy gap separates filled and unfilled electronic states.…

Layered transition metal dichalcogenides (TMDs) are commonly classified as quasi-two-dimensional materials, meaning that their electronic structure closely resembles that of an individual layer, which results in resistivity anisotropies…

1T-TaS$_2$ is a prototypical charge-density-wave (CDW) system with a Mott insulating ground state. Usually, a Mott insulator is accompanied by an antiferromagnetic state. However, the antiferromagnetic order had never been observed in…

Strongly Correlated Electrons · Physics 2020-06-11 Q. Niu , W. Zhang , Y. T. Chan , E. C. T. O'Farrell , R. Doganov , K. Y. Yip , Kwing To Lai , W. C. Yu , B. Ozyilmaz , G. R. Stewart , J. S. Kim , Swee K. Goh

We use scanning tunneling microscopy to study the temperature evolution of the atomic-scale properties of the nearly-commensurate charge density wave (NC-CDW) state of the low-dimensional material, 1T-TaS$_2$. Our measurements at 203 K, 300…

Strongly Correlated Electrons · Physics 2023-04-28 Boning Yu , Ghilles Ainouche , Manoj Singh , Bishnu Sharma , James Huber , Michael C. Boyer

The layered transition metal dichalcogenides host a rich collection of charge density wave (CDW) phases in which both the conduction electrons and the atomic structure display translational symmetry breaking. Manipulating these complex…

Mesoscale and Nanoscale Physics · Physics 2016-11-15 A. W. Tsen , R. Hovden , D. Z. Wang , Y. D. Kim , J. Okamoto , K. A. Spoth , Y. Liu , W. J. Lu , Y. P. Sun , J. Hone , L. F. Kourkoutis , P. Kim , A. N. Pasupathy

The commensurate charge-density-wave phase of the prototypical transition metal dichalcogenide $1T$-TaS$_2$ is investigated by temperature- and polarization-dependent infrared spectroscopy, revealing distinct charge dynamics parallel and…

Strongly Correlated Electrons · Physics 2026-01-21 Achyut Tiwari , Maxim Wenzel , Renjith Mathew Roy , Christian Prange , Bruno Gompf , Martin Dressel

Using density functional theory with added on-site interactions (DFT+U), we study the electronic structure of bulk, monolayer, and bilayer of the layered transition-metal dichalcogenide $1T-TaS_2$. We show that a two-dimensional…

Materials Science · Physics 2015-06-18 Pierre Darancet , Andrew J. Millis , Chris A. Marianetti

The transition-metal dichalcogenide tantalum disulphide (1$T$-TaS$_2$) hosts a commensurate charge density wave (CCDW) at temperatures below 165~K where it also becomes insulating. The low temperature CCDW phase can be driven into a…

Ultra-thin 2D materials have shown complete paradigm shift of understanding of physical and electronic properties because of confinement effects, symmetry breaking and novel phenomena at nanoscale. Bulk 2H-TaS2 undergoes an incommensurate…

Mesoscale and Nanoscale Physics · Physics 2023-07-18 Divya Rawat , Aksa Thomas , Ajay Soni

Quantum transitions between the Mott insulator and metals by controlling filling in two-dimensional square lattice are characterized by a large dynamical exponent $z=4$ where the origin of unusual metallic properties near the Mott insulator…

Strongly Correlated Electrons · Physics 2007-05-23 Masatoshi Imada , Fakher F. Assaad , Hirokazu Tsunetsugu , Yukitoshi Motome

We report on the dramatic slowing down of the charge carrier dynamics in a quasi-two-dimensional organic conductor, which can be reversibly tuned through the Mott metal-insulator transition (MIT). At the finite-temperature critical endpoint…

Strongly Correlated Electrons · Physics 2015-06-02 B. Hartmann , D. Zielke , J. Polzin , T. Sasaki , J. Müller

Transport through a one channel wire of length $L$ confined between two leads is examined when the 1D electron system has an energy gap $2M$: $M > T_L \equiv v_c/L$ induced by the interaction in charge mode ($v_c$: charge velocity in the…

Condensed Matter · Physics 2009-10-31 Vadim Ponomarenko , Naoto Nagaosa

We investigate the interplay of the electron-electron and electron-phonon interactions in the electronic structure of an exotic insulating state in the layered dichalcogenide 1T-TaS2, where the charge-density-wave (CDW) order coexists with…

Materials Science · Physics 2017-07-12 Doohee Cho , Yong-Heum Cho , Sang-Wook Cheong , Ki-Seok Kim , Han Woong Yeom

Strong electron-electron interaction can induce Mott insulating state, which is believed to host unusual correlated phenomena such as quantum spin liquid when quantum fluctuation dominates and unconventional superconductivity through…

Strongly Correlated Electrons · Physics 2025-04-24 Qiang Gao , Haiyang Chen , Wen-shin Lu , Yang-hao Chan , Zhenhua Chen , Yaobo Huang , Zhengtai Liu , Peng Chen

1T-TaS$_2$ undergoes successive phase transitions upon cooling and eventually enters an insulating state of mysterious origin. Some consider this state to be a band insulator with interlayer stacking order, yet others attribute it to Mott…

Strongly Correlated Electrons · Physics 2020-08-26 Y. D. Wang , W. L. Yao , Z. M. Xin , T. T. Han , Z. G. Wang , L. Chen , C. Cai , Yuan Li , Y. Zhang

Transition metal dichalcogenides are rich in their structural phases, e.g. 1T-TaS2 and 1T-TaSe2 form charge density wave (CDW) under low temperature with interesting and exotic properties. Here, we present a systematic study of different…

Materials Science · Physics 2022-01-12 Tao Jiang , Tao Hu , Guodong Zhao , Yongchang Li , Shaowen Xu , Chao Liu , Yaning Cui , Wei Ren