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Quantum-optical descriptions of strong-field processes have attracted significant attention in recent years. Typically, the theoretical modeling has been conducted in the Schr\"odinger picture, where results are only obtainable under…

Using reflective cross-polarized 2D THz time-domain spectroscopy in the range of 1-12 THz, we follow the trajectory of the out-of-equilibrium electron population in the low-bandgap semiconductor InSb. The 2D THz spectra show a set of…

Strongly Correlated Electrons · Physics 2019-06-10 S. Houver , L. Huber , M. Savoini , E. Abreu , S. L. Johnson

Optical second-harmonic generation is demonstrated to be a sensitive probe of the buried interface between the lattice matched semiconductors gallium phosphide and silicon with (001) orientation. Rotational anisotropy measurements of SHG…

Mesoscale and Nanoscale Physics · Physics 2020-10-29 K. Brixius , A. Beyer , J. Güdde , M. Dürr , W. Stolz , K. Volz , U. Höfer

We analytically investigate the effect of a non-centrosymmetric geometry in the optical second harmonic (SH) generation from a particle made of a centrosymmetric material, in the interior of which quadratic optical processes are suppressed.…

Optics · Physics 2019-03-27 Raksha Singla , W. Luis Mochán

We experimentally and theoretically investigate the second order nonlinear optical response of metallo-dielectric multilayer structures composed of Ag and Ta2O5 layers, deposited by magnetron sputtering. Second harmonic generation…

We demonstrate a method to image an object using a self-probing approach based on semiconductor high-harmonic generation. On one hand, ptychography enables high-resolution imaging from the coherent light diffracted by an object. On the…

Using one-dimensional semiconductor Bloch equations, we investigate the multiband dynamics of electrons in a cutoff extension scheme employing an infrared pulse with additional UV injection. An extended three-step model is firstly validated…

Optics · Physics 2022-11-01 Yue Lang , Zhaoyang Peng , Zengxiu Zhao

Time-resolved scanning near-field optical microscopy (tr-SNOM) enables the measurement of the dynamic optical response of functional surfaces beyond the diffraction limit. Experimental challenges are imposed both by the use of a pulsed…

Optics · Physics 2026-04-16 Philipp Schwendke , Julia Stähler , Samuel Palato

Spectroscopy of the centrosymmetric magnetic semiconductors EuTe and EuSe reveals spin-induced optical second harmonic generation (SHG) in the band gap vicinity at 2.1-2.4eV. The magnetic field and temperature dependence demonstrates that…

We have investigated second harmonic generation (SHG) from Ag-coated LiNbO3 (LN) core-shell nanocuboids and found that giant SHG can occur via deliberately designed double plasmonic resonances. By controlling the aspect ratio, we can tune…

Optics · Physics 2014-11-19 Ming-Liang Ren , Si-Yuan Liu , Ben-Li Wang , Bao-Qin Chen , Jiafang Li , Zhi-Yuan Li

We have detected a second-order nonlinear optical response from aggregates of the ampholytic megamolecular polysaccharide sacran extracted from cyanobacterial biomaterials, by using optical second harmonic generation (SHG) microscopy. The…

Third-harmonic generation (THG) is a key nonlinear optical process for ultrafast imaging, terahertz (THz) signal generation, and symmetry-sensitive probes, often dominating in centrosymmetric materials where lower-order responses vanish.…

Optics · Physics 2026-01-09 Sanjay Sarkar , Debottam Mandal , Amit Agarwal

Optical second harmonic generation (SHG) is studied from multilayer graphene films in the presence of DC electric current flowing in the sample plane. Graphene layers are manufactured by chemical vapour deposition (CVD) technique and…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Anton Y. Bykov , Tatiana V. Murzina , Maxim G. Rybin , Elena D. Obraztsova

The enhancement and control of non-linear phenomena at a nanometer scale has a wide range of applications in science and in industry. Among these phenomena, high-harmonic generation in solids is a recent focus of research to realize next…

High-order frequency mixing in graphene using a two-color radiation field consisting of the fundamental and the second harmonic fields of an ultrashort linearly polarized laser pulse is studied. It is shown that the harmonics originated…

Mesoscale and Nanoscale Physics · Physics 2022-05-25 Hamlet K. Avetissian , Garnik F. Mkrtchian , Andreas Knorr

Exploration of optical non-linear response of graphene predominantly relies on ultra-short time domain measurements. Here we propose an alternate technique that uses frequency modulated continuous wavefront optical fields, thereby probing…

Mesoscale and Nanoscale Physics · Physics 2019-03-18 Ashutosh Singh , Saikat Ghosh , Amit Agarwal

Diffractive neural networks (DNNs) are an emerging approach for the realization of photonic artificial intelligence, especially due to their suitability for machine-vision applications and high-dimensional photonic information processing at…

Optics · Physics 2026-03-27 Marie Braasch , Anna Kartashova , Elena Goi , Thomas Pertsch , Sina Saravi

We present a novel spectroscopic technique for second harmonic generation (SHG) using femtosecond laser pulses at 30~kHz repetition rate, which nevertheless provides high spectral resolution limited only by the spectrometer. The potential…

Type I and type II second harmonic generation (SHG) of a beam transformed by the conical refraction phenomenon are presented. We show that, for type I, the second harmonic intensity pattern is a light ring with a point of null intensity…

We have detected second-order nonlinear optical response from an amphoteric mega-saccharides named sacran under a needle/ring electrode stimulus by using an optical second harmonic generation (SHG) microscope. SHG was observed from sacran…