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We report on the study of the third-order nonlinear optical interactions in In$_{x}$Ga$_{1-x}$As$_{y}$P$_{1-y}$/InP strip-loaded waveguides. The material composition and waveguide structures were optimized for enhanced nonlinear optical…

The coherent photogalvanic effect leads to the generation of a current under the absorption interference of coherent beams and allows for the inscription of space-charge gratings leading to an effective second-order susceptibility…

Optics · Physics 2022-11-29 Ozan Yakar , Edgars Nitiss , Jianqi Hu , Camille-Sophie Brès

We use second and third harmonic generation microscopy to investigate the nonlinear optical response of GaAs nanocavities embedded in a gold film and compare them to bare GaAs nanocavities. Our results reveal that the surrounding metallic…

Monolayer transition-metal dichalcogenides (TMDCs) present high second-order optical nonlinearity, which is extremely desirable for, e.g., frequency conversion in nonlinear photonic devices. On the other hand, the atomic thickness of 2D…

Mesoscale and Nanoscale Physics · Physics 2020-11-17 Pilar G. Vianna , Aline dos S. Almeida , Rodrigo M. Gerosa , Dario A. Bahamon , Christiano J. S. de Matos

We report parametric gain by utilizing $ \chi^{(2)} $ non-linearities in a semiconductor Bragg Reflection Waveguide (BRW) waveguide chip. Under the two-mode degenerate type II phase matching, it can be shown that more than 18 dBs of…

We theoretically study the coherent nonlinear response of electrons confined in semiconductor quantum wells under the effect of an electromagnetic radiation close to resonance with an intersubband transition. Our approach is based on the…

Mesoscale and Nanoscale Physics · Physics 2023-04-11 R. Cominotti , H. A. M. Leymann , J. Nespolo , J. -M. Manceau , M. Jeannin , R. Colombelli , I. Carusotto

Phase sensitive amplifiers (PSAs) have the potential to empower substantial advances in emerging generations of optical communication systems as well as classical and quantum on-chip signal processing. The core building block of a PSA is a…

The modification of electronic band structures and the subsequent tuning of electrical, optical, and thermal material properties is a central theme in the engineering and fundamental understanding of solid-state systems. In this scenario,…

Materials Science · Physics 2022-09-12 Valerio Di Giulio , P. A. D. Gonçalves , F. Javier García de Abajo

We realize and investigate a nonlinear metasurface taking advantage of intersubband transitions in ultranarrow GaN/AlN multi-quantum well heterostructures. Owing to huge band offsets, the structures offer resonant transitions in the telecom…

Optical resonances in nanostructures enable strong enhancement of nonlinear processes at the nanoscale, such as second-harmonic generation (SHG), with high-$Q$ modes providing intensified light--matter interactions and sharp spectral…

Nonlinear second harmonic optical activity of graphene covering a gold photon sieve was determined for different polarizations. The photon sieve consists of a subwavelength gold nanohole array placed on glass. It combines the benefits of…

Mesoscale and Nanoscale Physics · Physics 2016-01-14 Michael Lobet , Michael Sarrazin , Francesca Cecchet , Nicolas Reckinger , Alexandru Vlad , Jean-François Colomer , Dan Lis

We present a theoretical framework for nonlinear optics of graphene and other 2D materials in layered structures. We derive a key equation to find the effective electric field and the sheet current density in the 2D material for given…

Optics · Physics 2018-12-27 J. L. Cheng , J. E. Sipe , N. Vermeulen , C. Guo

Probing the polarization of water molecules at charged interfaces by second harmonic generation spectroscopy has been heretofore limited to isotropic materials. Here, we report non-resonant nonlinear optical measurements at the interface of…

Other Condensed Matter · Physics 2017-02-10 Paul E. Ohno , Sarah A. Saslow , Hong-fei Wang , Franz M. Geiger , Kenneth B. Eisenthal

Second-order nonlinearity in solids gives rise to a plethora of unique physical phenomena ranging from piezoelectricity and optical rectification to optical parametric amplification, spontaneous parametric down-conversion, and the…

There is an active demand to develop efficient nanoscale nonlinear sources for applications in photonic circuitry, quantum optics and biosensing. To this end, plasmonic systems have been utilized to boost the nonlinear signal generation,…

Optics · Physics 2019-06-26 Feng Wang , Manoj Manjare , Robert Lemasters , Chentao Li , Hayk Harutyunyan

Monolayer transition metal dichalcogenides (TMDs) exhibit high nonlinear optical (NLO) susceptibilities. Experiments on MoS$_2$ have indeed revealed very large second-order ($\chi^{(2)}$) and third-order ($\chi^{(3)}$) optical…

Unprecedented material compatibility and ease of integration, in addition to the unique and diverse optoelectronic properties of layered materials have generated significant interest in their utilization in nanophotonic devices. While…

Optics · Physics 2018-06-12 Taylor Fryett , Alan Zhan , Arka Majumdar

We report measurements of phase-matched nonlinear x-ray and optical sum-frequency generation from single-crystal silicon using sub-resonant 0.95 eV laser pulses and 9.5 keV hard x-ray pulses from the LCLS free-electron laser. The…

The discovery of second harmonic generation in 1961 marked the birth of nonlinear optics, unlocking a range of applications from frequency conversion to quantum light generation. Yet, phase matching in bulk nonlinear crystals remains a key…

The second-order nonlinear optical (NLO) processes, such as the photogalvanic effect and second-order harmonic generation (SHG), play crucial roles in probing and controlling light-matter interactions for energy and device applications. To…

Materials Science · Physics 2020-08-05 Ruixiang Fei , Wenshen Song , Li Yang
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