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Related papers: Phonons reflect dynamic spin-state order in LaCoO$…

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We present an inelastic neutron scattering study of the low energy crystal-field excitations in the lightly doped cobalt perovskite La_0.998Sr_0.002CoO_3. In contrast to the parent compound LaCoO_3 an inelastic peak at energy transfer ~0.75…

Strongly Correlated Electrons · Physics 2008-02-22 A. Podlesnyak , K. Conder , E. Pomjakushina , A. Mirmelstein , P. Allenspach , D. I. Khomskii

We report neutron scattering measurements of spin density wave order within the superconducting state of a single crystal of predominately stage-4 La2CuO4+y with a Tc(onset) of 42 K. The low temperature elastic magnetic scattering is…

Superconductivity · Physics 2009-10-31 Y. S. Lee , R. J. Birgeneau , M. A. Kastner , Y. Endoh , S. Wakimoto , K. Yamada , R. W. Erwin , S. H. Lee , G. Shirane

We investigate the spin state of LaCoO3 using state-of-the-art photoemission spectroscopy and ab initio band structure calculations. The GGA+U calculations provide a good description of the ground state for the experimentally estimated…

Strongly Correlated Electrons · Physics 2007-07-10 S. K. Pandey , Ashwani Kumar , S. Patil , V. R. R. Medicherla , R. S. Singh , K. Maiti , D. Prabhakaran , A. T. Boothroyd , A. V. Pimpale

In bilayer CrI3, experimental and theoretical studies suggest that the magnetic order is closely related to the layer staking configuration. In this work, we study the effect of dynamical lattice distortions, induced by non-linear phonon…

Mesoscale and Nanoscale Physics · Physics 2020-08-26 M. Rodriguez-Vega , Ze-Xun Lin , A. Leonardo , A. Ernst , G. Chaudhary , M. G. Vergniory , Gregory A. Fiete

We present detailed ab-initio lattice dynamical analysis of the Fe-O infinite-layer compounds CaFeO2 and SrFeO2 in various magnetic configurations. These indicate strong spin-phonon coupling in SrFeO2 in contrast to that in case of CaFeO2.…

Materials Science · Physics 2016-09-13 M. K. Gupta , R. Mittal , S. L. Chaplot , Cedric Tassel , Hiroshi Kageyama

Neutrons have played an important role in advancing our understanding of the pairing mechanism and the symmetry of the superconducting energy gap in the iron arsenide compounds. Neutron measurements of the phonon density-of-state are in…

Superconductivity · Physics 2014-07-15 R. Osborn , S. Rosenkranz , E. A. Goremychkin , A. D. Christianson

Although the rutile structure of TiO$_2$ is stable at high temperatures, the conventional quasiharmonic approximation predicts that several acoustic phonons decrease anomalously to zero frequency with thermal expansion, incorrectly…

Materials Science · Physics 2015-08-19 Tian Lan , C. W. Li , O. Hellman , D. Kim , J. A. Muñoz , H. Smith , D. L. Abernathy , B. Fultz

We show that in YVO3 new hard phonons gradually become zone center active below ~210 K verifying that a lattice phase transition takes place at about that temperature. The Debye-Waller factor found from EXAFS measurements show an additional…

We present a detailed study on the magnetic order in the undoped mother compound LaOFeAs of the recently discovered Fe-based superconductor LaO$_{1-x}$F$_x$FeAs. In particular, we present local probe measurements of the magnetic properties…

Our success in description of recent electron-spin-resonance results on Mott insulator LaCoO3, Phys. Rev. B 67 (2003) 172401, lies in taking into account strong electron correlations among d electrons and the relativistic spin-orbit…

Strongly Correlated Electrons · Physics 2009-11-10 R. J. Radwanski , Z. Ropka

Quasi-2D van der Waals ferromagnet Fe$_4$GeTe$_2$, featuring the simultaneous presence of high Curie temperature ($T_\mathrm{C}$ $\sim 270$ K) and a spin-reorientation transition at $T_\mathrm{SR}$ $\sim 110$ K, is a rare system where…

Coupling between spin and lattice degrees of freedom are important in geometrically frustrated magnets where they can lead to degeneracy lifting and novel orders. We show that moderate spin-lattice couplings in triangular and Kagome…

Strongly Correlated Electrons · Physics 2008-02-20 Fa Wang , Ashvin Vishwanath

By means of neutron inelastic scattering, magnetic excitations and phonons were measured for a single crystal of slightly overdoped superconductor Ca10Pt4As8(Fe1-xPtxAs)10 (x ~ 0.2) with the transition temperature Tc of ~33 K. Below Tc,…

The analysis of phonon anomalies provides valuable information about the cooperative dynamics of lattice, spin and charge degrees of freedom. Significant is the anomalous temperature dependence of the external modes observed in…

Strongly Correlated Electrons · Physics 2010-05-24 Ch. Hartinger , F. Mayr , A. Loidl , T. Kopp

\lco{} is known for its two-step spin crossover as a function of temperature. Despite efforts spanning over half a century, the origin of this phenomenon is still debated, particularly regarding how the microscopic spin states are involved…

Strongly Correlated Electrons · Physics 2024-11-18 Akihiko Ikeda , Yasuhiro H. Matsuda , Keisuke Sato , Joji Nasu

Spin-phonon coupling originated from spin-lattice correlation depends upon different exchange interactions in transition metal oxides containing 3d magnetic ions. Spin-lattice coupling can influence the coupling mechanism in magnetoelectric…

Strongly Correlated Electrons · Physics 2021-09-09 P. Pal , Shalini Badola , P. K. Biswas , Ranjana R. Das , Surajit Saha , S. D. Kaushik , P. N. Vishwakarma , A. K. Singh

The spin excitations from the nonmagnetic charge-ordered insulating state of $\alpha$-(BEDT-TTF)$_2$I$_3$ at ambient pressure have been investigated by probing the static and low-frequency dynamic spin susceptibilities via site-selective…

Strongly Correlated Electrons · Physics 2016-09-08 Kyohei Ishikawa , Michihiro Hirata , Dong Liu , Kazuya Miyagawa , Masafumi Tamura , Kazushi Kanoda

We present Co $L_3$-edge resonant inelastic x-ray scattering (RIXS) of bulk LaCoO$_3$ across the thermally-induced spin-state crossover around 100~K. Owing to a high energy resolution of 25~meV, we observe unambiguously the dispersion of…

We have measured near normal incidence far infrared (FIR) reflectivity spectra of a single crystal of TbMnO3 from 10K to 300K in the spectral range of 50 cm$^{-1}$ to 700 cm$^{-1}$. Fifteen transverse optic (TO) and longitudinal optic (LO)…

Materials Science · Physics 2015-05-13 Pradeep Kumar , Surajit Saha , C. R. Serrao , A. K. Sood , C. N. R. Rao

In this study, we present a comprehensive analysis of the Raman active phonon modes in orthorhombic LaInO$_3$ based on a combination of polarization-angle resolved Raman spectroscopy and density functional theory calculations. By using…