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We investigated the precise crystal structures and electronic states in a quasi-two-dimensional molecular conductor ${\alpha}$-(BETS)$_2$I$_3$ at ambient pressure. The electronic resistivity of this molecular solid shows metal-to-insulator…

The electric conductivity of Dirac electrons in the organic conductor $\alpha$-STF$_2$I$_3$ (STF = bis(ethylenedithio)diselenadithiafulvalene), which has an isostructure of ET(=bis(ethylenedithio)tetrathiafulvalene), has been theoretically…

Mesoscale and Nanoscale Physics · Physics 2022-04-28 Yoshikazu Suzumura , Toshio Naito

Effect of spin-orbit coupling (SOC) on Dirac electrons in the organic conductor $\alpha$-(BETS)$_2$I$_3$ [BETS = bis(ethylenedithio)tetraselenafulvalene] has been examined by calculating electric conductivity and spin magnetic…

Materials Science · Physics 2021-11-23 Yoshikazu Suzumura , Takao Tsumuraya

We report on the Shubnikov de Haas (SdH) oscillations in the quasi two-dimensional molecular conductor $\alpha-$(BETS)$_{2}$I$_{3}$ [BETS: bis(ethylenedithio)tetraselenafulvalene] laminated on polyimide films at 1.7 K. From the SdH phase…

The electric conductivity of Dirac electrons in the organic conductor $\alpha$-(BEDT-TTF)$_2$I$_3$ [BEDT-TTF = bis(ethylenedithio)tetrathiafulvalene] under pressure has been examined using a two-dimensional tight-binding (TB) model with…

Mesoscale and Nanoscale Physics · Physics 2021-03-30 Yoshikazu Suzumura , Masao Ogata

We report a $^{13}$C-NMR study on the ambient-pressure metallic phase of the layered organic conductor $\theta$-(BEDT-TTF)$_{2}$I$_{3}$ [BEDT-TTF: bisethylenedithio-tetrathiafulvalene], which is expected to connect the physics of correlated…

Materials Science · Physics 2012-05-31 Michihiro Hirata , Kazuya Miyagawa , Kazushi Kanoda , Masafumi Tamura

We present magnetoresistance studies of the quasi-two-dimensional organic conductor $\kappa$-(BETS)$_2$Mn[N(CN)$_2$]$_3$, where BETS stands for bis\-(ethylene\-dithio)\-tetra\-selena\-fulvalene. Under a moderate pressure of 1.4\,kbar,…

Strongly Correlated Electrons · Physics 2018-01-09 M. V. Kartsovnik , V. N. Zverev , W. Biberacher , S. V. Simonov , I. Sheikin , N. D. Kushch , E. B. Yagubskii

The quasi-two-dimensional molecular semimetallic conductor $\alpha$-STF$_2$I$_3$ is isostructural with $\alpha$-ET$_2$I$_3$.The latter possesses a unique band structure showing a zero-gap state with Dirac cones under high pressure, whereas…

Materials Science · Physics 2020-01-09 Toshio Naito , Ryusei Doi , Yoshikazu Suzumura

A Dirac electron system in solids mimics a relativistic quantum physics that is compatible with Maxwell's equations, by which we anticipate unified electromagnetic responses. We find a large orbital diamagnetism only along the interplane…

Mesoscale and Nanoscale Physics · Physics 2022-01-20 S. Fujiyama , H. Maebashi , N. Tajima , T. Tsumuraya , H-B. Cui , M. Ogata , R. Kato

The Seebeck coefficient, which is proportional to a ratio of the thermoelectric conductivity to electrical conductivity has been examined for Dirac electrons in the organic conductor $\alpha$-(BEDT-TTF)$_2$I$_3$ [BEDT-TTF denotes a molecule…

Materials Science · Physics 2023-05-11 Yoshikazu Suzumura , Masao Ogata

Having been extensively studied during last decades in the fields of thermoelectics and ionic conductors, the $\alpha $ phase of Cu$_{2}$Se with antfluoride crystal structure has recently emerged as a topological zero-gap semimetal with a…

Materials Science · Physics 2026-05-05 Thomas Steele , Becker Sharif , David Lederman , Xiangang Wan , Sergey Y. Savrasov

We demonstrated X-ray structural analysis of the pressure-induced superconductor, $\beta'$-ET$_2$ICl$_2$ under extremely high-pressure conditions, where ET denotes bis(ethylenedithio)tetrathiafulvalene. This material has been known as the…

Superconductivity · Physics 2025-09-29 T. Kobayashi , K. Yoshimi , H. Ma , S. Sekine , H. Taniguchi , N. Matsunaga , A. Kawamoto , Y. Uwatoko

The low-temperature electronic state of the layered organic charge-transfer salt $\kappa$-(BETS)$_2$FeCl$_4$ was probed by interlayer electrical resistance measurements under magnetic field. Both above and below $T_{\mathrm{N}}=0.47\,$K,…

Strongly Correlated Electrons · Physics 2016-11-09 Michael Kunz , Werner Biberacher , Natalia D. Kushch , Akira Miyazaki , Mark V. Kartsovnik

We review the role of strong electronic correlations in quasi--two-dimensional organic charge transfer salts such as (BEDT-TTF)$_2X$, (BETS)$_2Y$ and $\beta'$-[Pd(dmit)$_2$]$_2Z$. We begin by defining minimal models for these materials. It…

Strongly Correlated Electrons · Physics 2007-05-23 B. J. Powell , Ross H. McKenzie

We report on magnetization, specific heat and resistivity experiments on single crystals of the novel heavy Fermion compound Ce$_3$PdIn$_{11}$. At ambient pressure the compound exhibits two successive transitions at T$_{1}$ = 1.63 K and…

Strongly Correlated Electrons · Physics 2015-12-03 M. Kratochvílová , J. Prokleška , K. Uhlířová , M. Dušek , V. Sechovský , J. Custers

We employed first-principles density-functional theory (DFT) calculations to characterize Dirac electrons in quasi-two-dimensional molecular conductor $\alpha$-(BETS)$_2$I$_3$ [= $\alpha$-(BEDT-TSeF)$_2$I$_3$] at a low temperature of 30K.…

Strongly Correlated Electrons · Physics 2021-01-18 Takao Tsumuraya , Yoshikazu Suzumura

We show a zero-gap semiconducting (ZGS) state in the quasi-two-dimensional organic conductor $\alpha$-(BEDT-TTF)$_2$I$_3$ salt, which emerges under uniaxial pressure along the a-axis (the stacking axis of the BEDT-TTF molecule). The ZGS…

Materials Science · Physics 2009-11-11 Shinya Katayama , Akito Kobayashi , Yoshikazu Suzumura

The band structure and magnetic properties of organic charge-transfer salt $\lambda$-(BEDSe-TTF)$_2$GaCl$_4$ (BEDSe-TTF: bis(ethylenediseleno)tetrathiafulvalene; abbreviated as $\lambda$-BEDSe) are investigated. The reported crystal…

Strongly Correlated Electrons · Physics 2022-07-15 A. Ito , T. Kobayashi , D. P. Sari , I. Watanabe , Y. Saito , A. Kawamoto , H. Tsunakawa , K. Satoh , H. Taniguchi

A zero-gap state (ZGS) has been found in a bulk system of two-dimensional organic conductor, $\alpha$-(BEDT-TTF)$_2$I$_3$ salt which consists of four sites of donor molecules in a unit cell. In the present paper, the characteristic of the…

Strongly Correlated Electrons · Physics 2009-11-13 Shinya Katayama , Akito Kobayashi , Yoshikazu Suzumura

The conducting state of the quasi-two-dimensional organic conductor, $\alpha$-(BEDT-TTF)$_2$I$_3$, at ambient pressure is investigated with $^{13}$C NMR measurements, which separate the local electronic states at three nonequivalent…

Materials Science · Physics 2011-10-04 Michihiro Hirata , Kyohei Ishikawa , Kazuya Miyagawa , Kazushi Kanoda
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