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Natural materials usually consist of isotopic mixtures, for which different isotopic ratios can lead to distinct material properties such as thermal conductivity and nucleation process. However, the knowledge of isotopic interface remains…

We show that the isotope effect leads to a completely different spectroscopic signal in hydrogen-deuterium mixtures, compared to pure elements that have the same crystal structure. This is particularly true for molecular vibrations, which…

Materials Science · Physics 2017-04-12 Ioan B. Magdău , Graeme J. Ackland

Phonon exchange with nuclei in the course of fusion reactions that occur in a solid has not been analyzed previously. This problem has become of interest in connection with claims of observations of anomalies in metal deuterides. If the…

Other Condensed Matter · Physics 2007-05-23 Irfan Chaudhary , Peter Hagelstein

The study of phonon dynamics is pivotal for understanding material properties, yet it faces challenges due to the irreversible information loss inherent in powder inelastic neutron scattering spectra and the limitations of traditional…

Materials Science · Physics 2024-10-29 Yaokun Su , Chen Li

Within the framework of density functional perturbation theory (DFPT), we implement and test a novel "metric wave" response-function approach. It consists in the reformulation of an acoustic phonon perturbation in the curvilinear frame that…

Materials Science · Physics 2019-02-13 Andrea Schiaffino , Cyrus E. Dreyer , David Vanderbilt , Massimiliano Stengel

By applying an unrestricted Hartree-Fock and a Random Phase approximations to a multiband Peierls-Hubbard Hamiltonian, we study the phonon mode structure in models of transition metal oxides in the presence of intrinsic nanoscale…

Strongly Correlated Electrons · Physics 2009-11-10 I. Martin , E. Kaneshita , R. J. McQueeney , Z. G. Yu , A. R. Bishop

By applying an unrestriced Hartree-Fock approximation and a Random Phase approximation to multiband Peierls-Hubbard Hamiltonians, we determine the phonon mode structure in models of transition metal oxides in the presence of intrinsic…

Strongly Correlated Electrons · Physics 2009-09-29 I. Martin , R. J. McQueeney , A. R. Bishop , Z. G. Yu

The phonon renormalization across the semiconductor-to-metal crossover in FeSi is investigated by inelastic neutron scattering combined with \textit{ab-initio} lattice dynamical calculations. A significant part of reciprocal space with a…

Materials Science · Physics 2022-05-03 Nazir Khan , Sven Krannich , Dominic Boll , Rolf Heid , Daniel Lamago , A. Ivanov , David Voneshen , Frank Weber

Isotopic fluctuations in fragment formation are investigated in a quasi-analytical description of the spinodal decomposition scenario. By exploiting the fluctuation-dissipation relations the covariance matrix of density fluctuations is…

Nuclear Theory · Physics 2008-11-26 M. Colonna , F. Matera

We study photonic meta-atoms, a unique class of composite solitary wave, supported in nonlinear waveguides. We establish an analogy to one-dimensional soft-core atoms, allowing to describe the complex dynamics via concepts from atomic…

Optics · Physics 2026-03-19 S. Zhang , I. Babushkin , U. Morgner , A. Demircan , O. Melchert

The physics of mutual interaction of phonon quasiparticles with electronic spin degrees of freedom, leading to unusual transport phenomena of spin and heat, has been a subject of continuing interests for decades. Despite its pivotal role in…

Materials Science · Physics 2022-07-14 Qiyang Sun , Bin Wei , Yaokun Su , Hillary Smith , Jiao Y. Y. Lin , Douglas L. Abernathy , Chen Li

Phonon spectra of solid substitutional solutions with finite concentrations of impurities were analyzed on the microscopic level. The local phonon densities of impurity atoms were calculated, in particular the formation of quasilocal…

Recently, massive efforts have been done on controlling thermal transport via coherent phonons in the various periodic nanostructures. However, the intrinsic lattice difference between the constituent materials inevitably generates the…

Mesoscale and Nanoscale Physics · Physics 2021-06-03 Meng An , Dongsheng Chen , Weigang Ma , Shiqian Hu , Xing Zhang

We study the vibrational motion of membrane resonators upon strong drive in the strongly nonlinear regime. By imaging the vibrational state of rectangular siliconnitride membrane resonators and by analyzing the frequency response using…

Mesoscale and Nanoscale Physics · Physics 2019-04-24 Fan Yang , Felix Rochau , Jana Huber , Alexandre Brieussel , Gianluca Rastelli , Eva M. Weig , Elke Scheer

The nature of the lattice instability connected to the structural transition and superconductivity of (Sr,Ca)$_3$Ir$_4$Sn$_{13}$ is not yet fully understood. In this work density functional theory (DFT) calculations of the phonon…

Superconductivity · Physics 2014-02-20 David A. Tompsett

We present in full detail a newly developed formalism enabling density functional perturbation theory (DFPT) calculations from a DFT+$U$ ground state. The implementation includes ultrasoft pseudopotentials and is valid for both insulating…

Strongly Correlated Electrons · Physics 2020-02-21 Andrea Floris , Iurii Timrov , Burak Himmetoglu , Nicola Marzari , Stefano de Gironcoli , Matteo Cococcioni

The advent of monochromated electron energy-loss spectroscopy has enabled atomic-resolution vibrational spectroscopy, which triggered interest in spatially localized or quasi-localized vibrational modes in materials. Here we report the…

Materials Science · Physics 2023-10-13 De-Liang Bao , Mingquan Xu , Ao-Wen Li , Gang Su , Wu Zhou , Sokrates T. Pantelides

The isoscalar giant monopole resonance (ISGMR) and isovector giant dipole resonance (IVGDR) in finite nuclei are studied in the framework of a relativistic transport approach. The kinetic equations are derived within an effective…

Nuclear Theory · Physics 2016-09-08 S. Yildirim , T. Gaitanos , M. Di Toro , V. Greco

We use vibrational dynamical mean-field theory (VDMFT) to study the vibrational structure of type-I clathrate solids, specifically X$_8$Ga$_{16}$Ge$_{30}$, where X=Ba,Sr. These materials are cage-like chemical structures hosting loosely…

Materials Science · Physics 2024-08-02 Dipti Jasrasaria , Timothy C. Berkelbach

Isotopic substitution in molecular systems can affect fundamental molecular properties including the energy position and spacing of electronic, vibrational and rotational levels, thus modifying the dynamics associated to their coherent…

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