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Hyperfine interactions between electron and nuclear spins have been widely used in material science, organic chemistry, and structural biology as a sensitive probe to the local chemical environment through spatial identification of nuclear…

Mesoscale and Nanoscale Physics · Physics 2022-12-28 Jinkyung Kim , Kyungju Noh , Yi Chen , Fabio Donati , Andreas J. Heinrich , Christoph Wolf , Yujeong Bae

A system's internal dynamics and its interaction with the environment can be determined by tracking how external perturbations affect its transition rates between states. Quantitative measurements of these rates are crucial for optimizing…

The efficient transfer of quantum states into a long-lived storage unit such as solid-state spin ensembles is widely recognized as a critical challenge with significant implications for quantum communication, sensing and computing…

Quantum Physics · Physics 2025-12-22 P. Oehrl , F. Fesquet , K. E. Honasoge , M. Handschuh , A. Marx , R. Gross , K. G. Fedorov , H. Huebl

Electron spin resonance with a scanning tunneling microscope (ESR-STM) combines the high energy resolution of spin resonance spectroscopy with the atomic scale control and spatial resolution of STM. Here we describe the upgrade of a…

Instrumentation and Detectors · Physics 2019-01-30 Fabian D. Natterer , François Patthey , Tobias Bilgeri , Patrick R. Forrester , Nicolas Weiss , Harald Brune

Recent advances in scanning tunneling microscopy have enabled quantum-coherent control of single surface spins via all-electric electron spin resonance (ESR). Such control requires magnetoelectric coupling, since spin resonance is a…

Mesoscale and Nanoscale Physics · Physics 2025-10-31 Xue Zhang , Jose Reina-Gálvez , Di'an Wu , Jan Martinek , Andreas J. Heinrich , Taeyoung Choi , Christoph Wolf

The recent development of all-electrical electron spin resonance (ESR) in a scanning tunneling microscope (STM) setup has opened the door to vast applications. Despite the fast growing number of experimental works on STM-ESR, the…

Mesoscale and Nanoscale Physics · Physics 2019-07-17 J. Reina Gálvez , C. Wolf , F. Delgado , N. Lorente

Control of quantum systems typically relies on the interaction with electromagnetic radiation. In this study, we experimentally show that the electromagnetic near-field of a spatially modulated freespace electron beam can be used to drive…

In this study, we report a conceptually novel broadband high-frequency electron spin resonance (HFESR) spectroscopic technique. In contrast to the ordinary force-detected ESR technique, which detects the magnetization change due to the…

Applied Physics · Physics 2018-08-02 Hideyuki Takahashi , Tsubasa Okamoto , Kento Ishimura , Shigeo Hara , Eiji Ohmichi , Hitoshi Ohta

Scanning transmission electron microscopy (STEM) has advanced rapidly in the last decade thanks to the ability to correct the major aberrations of the probe forming lens. Now atomic-sized beams are routine, even at accelerating voltages as…

Individual magnetic molecules are promising building blocks for quantum technologies because of their chemical tunability, nanoscale dimensions, and ability to self-assemble into ordered arrays. However, harnessing their properties in…

The optical spin noise spectroscopy (SNS) is a minimally invasive route towards obtaining dynamical information about electrons and atomic gases by measuring mesoscopic time-dependent spin fluctuations. Recent improvements of the…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 Fuxiang Li , Avadh Saxena , Darryl Smith , Nikolai A. Sinitsyn

Semiconductor spin noise spectroscopy (SNS) has emerged as a unique experimental tool that utilizes spin fluctuations to provide profound insight into undisturbed spin dynamics in doped semiconductors and semiconductor nanostructures. The…

Mesoscale and Nanoscale Physics · Physics 2011-03-28 G. M. Müller , M. Oestreich , M. Römer , J. Hübner

In this paper we propose that electron spin resonance (ESR) measurements enable us to detect the long-range spin nematic order. We show that the frequency of the paramagnetic resonance peak in the ESR spectrum is shifted by the…

Strongly Correlated Electrons · Physics 2018-03-22 Shunsuke C. Furuya , Tsutomu Momoi

On-chip Electron Spin Resonance (ESR) of magnetic molecules requires the ability to precisely position nanosized samples in antinodes of the electro-magnetic field for maximal magnetic interaction. A method is developed to entrap…

Mesoscale and Nanoscale Physics · Physics 2009-08-28 N. Groll , S. Bertaina , M. Pati , N. S. Dalal , I. Chiorescu

Scanning Transmission Electron Microscopy (STEM) has become the main stay for materials characterization on atomic level, with applications ranging from visualization of localized and extended defects to mapping order parameter fields. In…

Instrumentation and Detectors · Physics 2019-01-15 Xin Li , Ondrej Dyck , Sergei V. Kalinin , Stephen Jesse

We propose a method of two-beam spin noise spectroscopy to test the spin transport at equilibrium via analysis of correlations between time-shifted spin fluctuations at different space locations. This method allows one to determine the…

Mesoscale and Nanoscale Physics · Physics 2016-06-24 Yuriy V. Pershin , Valeriy A. Slipko , Dibyendu Roy , Nikolai A. Sinitsyn

New phenomenon is experimentally identified: ferroelectrical spin wave resonance (FE SWR), which consist in characteristic splitting of vibration (electronic-vibration) levels in optical spectra of interacting localized centers. Spectral…

Other Condensed Matter · Physics 2015-05-14 D. P. Yearchuck , E. D. Yerchak , A. I. Kirilenko , V. I. Popechits

Free electron beams such as those employed in electron microscopes have evolved into powerful tools to investigate photonic nanostructures with an unrivaled combination of spatial and spectral precision through the analysis of electron…

Quantum Physics · Physics 2021-04-22 F. Javier García de Abajo , Valerio Di Giulio

The complex range of interactions between electrons and electromagnetic fields gave rise to countless scientific and technological advances. A prime example is photon-induced nearfield electron microscopy (PINEM), enabling the detection of…

Nuclear electric resonance (NER) spectroscopy is currently experiencing a revival as a tool for nuclear spin-based quantum computing. Compared to magnetic or electric fields, local electron density fluctuations caused by changes in the…

Quantum Physics · Physics 2025-01-30 Johannes K. Krondorfer , Andreas W. Hauser