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We present a Riemannian optimization framework for Hartree-Fock theory formulated directly in the Sobolev space $H^1$. The orthonormality constraints are interpreted geometrically via infinite-dimensional Stiefel and Grassmann manifolds…

Quantum Physics · Physics 2026-03-18 Evgueni Dinvay

Variational algorithms are promising candidates to be implemented on near-term quantum computers. The variational quantum eigensolver (VQE) is a prominent example, where a parametrized trial state of the quantum mechanical wave function is…

Understanding how systems built out of modular components can be jointly optimized is an important problem in biology, engineering, and machine learning. The backpropagation algorithm is one such solution and has been instrumental in the…

Machine Learning · Computer Science 2026-03-05 Christian Pehle , Jean-Jacques Slotine

A significant hurdle in the noisy intermediate-scale quantum (NISQ) era is identifying functional quantum circuits. These circuits must also adhere to the constraints imposed by current quantum hardware limitations. Variational quantum…

Quantum Physics · Physics 2024-10-03 Akash Kundu

Optimization problems in disciplines such as machine learning are commonly solved with iterative methods. Gradient descent algorithms find local minima by moving along the direction of steepest descent while Newton's method takes into…

Quantum Physics · Physics 2018-08-20 Patrick Rebentrost , Maria Schuld , Leonard Wossnig , Francesco Petruccione , Seth Lloyd

Decentralized optimization with orthogonality constraints is found widely in scientific computing and data science. Since the orthogonality constraints are nonconvex, it is quite challenging to design efficient algorithms. Existing…

Optimization and Control · Mathematics 2024-01-09 Lei Wang , Xin Liu

Determining the ultimate limits of quantum communication, such as the quantum capacity of a channel and the distillable entanglement of a shared state, remains a central challenge in quantum information theory, primarily due to the…

Quantum Physics · Physics 2025-10-15 Chengkai Zhu , Hongyu Mao , Kun Fang , Xin Wang

We propose a general random subspace framework for unconstrained nonconvex optimization problems that requires a weak probabilistic assumption on the subspace gradient, which we show to be satisfied by various random matrix ensembles, such…

Optimization and Control · Mathematics 2022-11-21 Coralia Cartis , Jaroslav Fowkes , Zhen Shao

Accelerating the convergence of second-order optimization, particularly Newton-type methods, remains a pivotal challenge in algorithmic research. In this paper, we extend previous work on the \textbf{Quadratic Gradient (QG)} and rigorously…

Optimization and Control · Mathematics 2026-04-01 John Chiang

As with many tasks in engineering, structural design frequently involves navigating complex and computationally expensive problems. A prime example is the weight optimization of laminated composite materials, which to this day remains a…

Quantum Physics · Physics 2024-09-20 Arne Wulff , Boyang Chen , Matthew Steinberg , Yinglu Tang , Matthias Möller , Sebastian Feld

Efficient ground state search is fundamental to advancing combinatorial optimization problems and quantum chemistry. While the Variational Imaginary Time Evolution (VITE) method offers a useful alternative to Variational Quantum Eigensolver…

Quantum Physics · Physics 2026-04-10 Ryo Suzuki , Shohei Watabe

Gradient descent with momentum has been widely applied in various signal processing and machine learning tasks, demonstrating a notable empirical advantage over standard gradient descent. However, momentum-based distributed Riemannian…

Optimization and Control · Mathematics 2026-02-17 Jun Chen , Tianyi Zhu , Haishan Ye , Lina Liu , Guang Dai , Yong Liu , Yunliang Jiang , Ivor W. Tsang

Parametrized quantum optical circuits are a class of quantum circuits in which the carriers of quantum information are photons and the gates are optical transformations. Classically optimizing these circuits is challenging due to the…

Quantum Physics · Physics 2020-12-02 Filippo M. Miatto , Nicolás Quesada

Variational quantum circuits are increasingly studied as continuous-function approximators, but quantum regression remains difficult to train when global losses, finite-shot stochasticity, and circuit-depth growth combine to produce weak or…

Machine Learning · Computer Science 2026-05-14 Qingyu Meng , Yangshuai Wang

Shape optimization based on the shape calculus is numerically mostly performed by means of steepest descent methods. This paper provides a novel framework to analyze shape-Newton optimization methods by exploiting a Riemannian perspective.…

Optimization and Control · Mathematics 2014-05-14 Volker Schulz

Training quantum neural networks (QNNs) using gradient-based or gradient-free classical optimisation approaches is severely impacted by the presence of barren plateaus in the cost landscapes. In this paper, we devise a framework for…

Quantum Physics · Physics 2024-06-04 Yidong Liao , Min-Hsiu Hsieh , Chris Ferrie

Optimization under the symplecticity constraint is an approach for solving various problems in quantum physics and scientific computing. Building on the results that this optimization problem can be transformed into an unconstrained problem…

Optimization and Control · Mathematics 2024-06-21 Bin Gao , Nguyen Thanh Son , Tatjana Stykel

Classical algorithms for predicting the equilibrium geometry of strongly correlated molecules require expensive wave function methods that become impractical already for few-atom systems. In this work, we introduce a variational quantum…

The von Neumann and quantum R\'enyi entropies characterize fundamental properties of quantum systems and lead to theoretical and practical applications in many fields. Quantum algorithms for estimating quantum entropies, using a quantum…

Quantum Physics · Physics 2023-10-13 Youle Wang , Benchi Zhao , Xin Wang

We propose a novel evolutionary algorithm for optimizing real-valued objective functions defined on the Grassmann manifold Gr}(k,n), the space of all k-dimensional linear subspaces of R^n. While existing optimization techniques on Gr}(k,n)…

Optimization and Control · Mathematics 2025-03-31 Andrew Lesniewski