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High-power infrared laser systems with broadband tunability are of great importance due to their wide range of applications in spectroscopy and free-space communications. These systems require nonlinear optical (NLO) crystals for wavelength…

High harmonic generation (HHG) provides a flexible framework for the development of coherent light sources in the extreme-ultraviolet and soft x-ray regimes. However it suffers from low conversion efficiencies as the control of the HHG…

Optics · Physics 2014-09-16 Alberto Castro , Angel Rubio , E. K. U. Gross

We investigate second harmonic (SH) generation in a doubly resonant metamaterial. We show that SH generation can be enhanced when the resonant condition is satisfied for the SH frequency as well as for the fundamental frequency. A unit cell…

The two-dimensional ferroelectrics GeS, GeSe, SnS and SnSe are expected to have large spontaneous in-plane electric polarization and enhanced shift-current response. Using density functional methods, we show that these materials also…

Mesoscale and Nanoscale Physics · Physics 2017-10-03 Suman Raj Panday , Benjamin M. Fregoso

High-order harmonic generation (HHG) in solids - the frequency up-conversion of an optical signal - is governed by symmetries. At terahertz (THz) frequencies, HHG is a key technology to access high frequency spectral windows that are…

Trigonal selenium and tellurium crystalize in helical chain-like structures and thus possess interesting properties such as current-induced spin polarization, gyrotropic effects and nonlinear optical responses. By performing systematic ab…

Computational Physics · Physics 2019-07-17 Meijuan Cheng , Shunqing Wu , Zi-Zhong Zhu , Guang-Yu Guo

We study optical harmonic generation on the 1S exciton-polariton in the semiconductor ZnSe. Intense and spectrally narrow exciton resonances are found in optical second (SHG), third (THG), and fourth (FHG) harmonic generation spectra. The…

Optics · Physics 2020-07-29 Johannes Mund , Dmitri R. Yakovlev , Marina A. Semina , Manfred Bayer

High harmonic generation (HHG) is an extreme nonlinear process where intense pulses of light drive matter to emit high harmonics of the driving frequency, reaching the extreme ultraviolet (XUV) and x-ray spectral ranges. So far, the HHG…

We report theoretical calculations of high harmonic generation (HHG) by intense infrared lasers in atomic and molecular targets taking into account the macroscopic propagation of both fundamental and harmonic fields. On the examples of Ar…

Atomic Physics · Physics 2011-02-28 Cheng Jin , Anh-Thu Le , C. D. Lin

The emerging field of silicon photonics seeks to unify the high bandwidth of optical communications with CMOS microelectronic circuits. Many components have been demonstrated for on-chip optical communications, including those that utilize…

Optics · Physics 2015-05-20 Jacob S. Levy , Mark A. Foster , Alexander L. Gaeta , Michal Lipson

Since de discovery of graphene, the family of 2-dimensional materials has attracted much recent attention. In this work, the nonlinear optical properties of few-layer MoS2 two-dimensional crystals are studied using femtosecond laser pulses.…

Mesoscale and Nanoscale Physics · Physics 2013-06-20 Leandro M. Malard , Thonimar V. Alencar , Ana Paula M. Barboza , Kin Fai Mak , Ana M. de Paula

We report on theoretical study of second-harmonic generation (SHG) in plasmonic nanostructures interacting with two-level quantum emitters (QE) under incoherent energy pump. We generalize driven-dissipative Tavis-Cummings model by…

Optics · Physics 2021-03-17 Maxim Sukharev , Oleksiy Roslyak , Andrei Piryatinski

We developed a novel technique for frequency measurement and synthesis, based on the operation of a femtosecond comb generator as transfer oscillator. The technique can be used to measure frequency ratios of any optical signals throughout…

Optics · Physics 2009-11-07 Jörn Stenger , Harald Schnatz , Christian Tamm , Harald R. Telle

We describe a novel scheme of detecting rotational anisotropy second harmonic generation (RA-SHG) signals using a lock-in amplifier referenced to a fast scanning RA-SHG apparatus. The method directly measures the $n^{th}$ harmonics of the…

Optics · Physics 2018-12-26 Baozhu Lu , Darius H. Torchinsky

High-harmonic generation (HHG) is widely used for up-conversion of amplified (near) infrared ultrafast laser pulses to short wavelengths. We demonstrate that Ramsey-comb spectroscopy, based on two such pulses derived from a frequency-comb…

Atomic Physics · Physics 2019-11-21 L. S. Dreissen , C. Roth , E. L. Gründeman , J. J. Krauth , M. Favier , K. S. E. Eikema

The generation process of second harmonic (SH) radiation from holes periodically arranged on a metal surface is investigated. Three main modulating factors affecting the optical response are identified: the near-field distribution at the…

Mesoscale and Nanoscale Physics · Physics 2015-01-08 Sergio G. Rodrigo , V. Laliena , L. Martín-Moreno

Second harmonic generation is considered in lossy negative-index metamaterials. It is shown that energy transfer from fundamental to harmonic takes place in the entire sample for the range of phase mismatch values. Note that in conventional…

Owing to the discrete frequency spectrum of whispering gallery resonators (WGRs), the resonance and phase-matching conditions for the interacting waves in the case of second-harmonic generation (SHG) cannot generally be fulfilled…

Optics · Physics 2021-04-23 Jan Szabados , Nicolás Amiune , Boris Sturman , Ingo Breunig

A novel mechanism of efficient second harmonic generation in domain wall series is reported. By employing angle modulation, obvious intensity peaks of second harmonic appear at specific incident angles utilizing the continuous laser source…

Optics · Physics 2010-10-11 Huaijin Ren , Xuewei Deng , Xianfeng Chen

The second-order $\chi^{2}$ process underpins many important nonlinear optical applications in the field of classical and quantum optics. Generally, the $\chi^{2}$ process manifests itself only in a non-centrosymmetric dielectric medium via…

Optics · Physics 2022-06-29 Yadong Wang , Daniel Burt , Kunze Lu , Donguk Nam