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Hybrid light-matter polaritonic states have shown great promise for altering already known and enabling novel chemical reactions and controlling photophysical phenomena. This field has recently become one of the most prominent and active…

Quantum Physics · Physics 2025-05-23 Braden M. Weight , Yu Zhang

The Hamiltonian for quantum electrodynamics becomes non-Hermitian if the unrenormalized electric charge $e$ is taken to be imaginary. However, if one also specifies that the potential $A^\mu$ in such a theory transforms as a pseudovector…

High Energy Physics - Theory · Physics 2011-07-19 Carl M. Bender , Ines Cavero-Pelaez , Kimball A. Milton , K. V. Shajesh

We study the quantum discord (QD) and the classical correlations (CC) in a reference model for strongly correlated electrons, the one-dimensional bond-charge extended Hubbard model. We show that the comparison of QD and CC and of their…

Quantum Physics · Physics 2013-05-29 Michele Allegra , Paolo Giorda , Arianna Montorsi

We extend our assessment of the potential of perturbative coupled cluster (CC) expansions for a test set of open-shell atoms and organic radicals to the description of quadruple excitations. Namely, the second- through sixth-order models of…

Chemical Physics · Physics 2016-05-17 Janus J. Eriksen , Devin A. Matthews , Poul Jørgensen , Jürgen Gauss

Basis set convergence of correlation effects on molecular atomization energies beyond the CCSD (coupled cluster with singles and doubles) approximation has been studied near the one-particle basis set limit. Quasiperturbative connected…

Chemical Physics · Physics 2008-08-17 Amir Karton , Peter R. Taylor , Jan M. L. Martin

In computational chemistry of molecular materials, strong static correlation effects appear when electronic states, often involving the ground state, become quasi-degenerate, as occurs, for example, in bond-breaking processes. Such…

Chemical Physics · Physics 2026-03-20 Braden M. Weight , Zheng Pei , Sergei Tretiak

We consider a one-dimensional effective quantum electrodynamics (QED) model of the relativistic hydrogen-like atom using delta-potential interactions. We discuss the general exact theory and the Hartree-Fock approximation. The present…

Mathematical Physics · Physics 2023-06-27 Timothée Audinet , Julien Toulouse

We propose an approach that enables to use it for construction of rotations of coherent states, in particular, it gives a possibility to construct Hadamard gate for the coherent states. Our approach is based on representation of arbitrary…

Quantum Physics · Physics 2011-08-09 Sergey A. Podoshvedov

Cavity quantum electrodynamics (QED) studies the interaction between a quantum emitter and a single radiation-field mode. When an atom is in strong coupling with a cavity mode1,2, it is possible to realize key quantum information processing…

Quantum Physics · Physics 2009-11-13 K. Hennessy , A. Badolato , M. Winger , D. Gerace , M. Atature , S. Gulde , S. Falt , E. L. Hu , A. Imamoglu

We present an excited-state-specific coupled-cluster approach in which both the molecular orbitals and cluster amplitudes are optimized for an individual excited state. The theory is formulated via a pseudoprojection of the traditional…

Chemical Physics · Physics 2023-11-27 Harrison Tuckman , Eric Neuscamman

QED formulated in prescribed classical background electromagnetic fields is a standard framework for strong-field and laser\textendash matter interactions. It is usually treated as a theory modified by externally imposed fields, obscuring…

Plasma Physics · Physics 2026-02-19 Keita Seto

We employ the closed-shell perturbed relativistic coupled-cluster (RCC) theory developed by us earlier [Phys. Rev. A {\bf 77}, 062516 (2008)] to evaluate the ground state static electric dipole polarizabilities (\alpha s) of several atomic…

Atomic Physics · Physics 2013-12-09 Yashpal Singh , B. K. Sahoo , B. P. Das

We present the implementation of relativistic coupled cluster quadratic response theory (QR-CC), following our development of relativistic equation of motion coupled cluster quadratic response theory (QR-EOMCC) [X. Yuan et al., J. Chem.…

Chemical Physics · Physics 2025-11-17 Xiang Yuan , Loïc Halbert , Lucas Visscher , André Severo Pereira Gomes

In previous work [1] new bounded coherent states construction, based on a Keldysh conjecture, was introduced. As was shown in [1] the particular group structure arising from the model leads to new symmetry transformations for the coherent…

Strongly Correlated Electrons · Physics 2014-08-29 Diego Julio Cirilo-Lombardo

The ever-growing intersection of quantum electrodynamics (QED) and molecular processes has shown remarkable and unanticipated advancements in altering molecular properties and reactivity by exploiting light-matter couplings. In recent…

Chemical Physics · Physics 2023-11-09 Xinyang Li , Yu Zhang

Predictions of the spectroscopic properties of low-lying states are critical for nuclear structure studies, but are problematic for nuclei with an odd nucleon due to the interplay of the unpaired single particle with nuclear collective…

Nuclear Theory · Physics 2017-12-06 S. Quan , W. P. Liu , Z. P. Li , M. S. Smith

In this paper we discuss the topics concerning the local excitation and coherent state in 2D CFT. It is shown that the local excitation of primary operator can be taken as a coherent state of the global conformal group. We also discuss the…

High Energy Physics - Theory · Physics 2015-12-15 Wu-Zhong Guo

We present a study of the two dimensional circular quantum dot model Hamiltonian using a range of quantum chemical ab initio methods. Ground and excited state energies are computed on different levels of perturbation theories including the…

Chemical Physics · Physics 2022-03-23 Faruk Salihbegović , Alejandro Gallo , Andreas Grüneis

We investigate the convergence of coupled-cluster correlation energies and related quantities with respect to the employed basis set size for the uniform electron gas to gain a better understanding of the basis set incompleteness error. To…

Materials Science · Physics 2024-02-27 Nikolaos Masios , Felix Hummel , Andreas Grüneis , Andreas Irmler

In a previous work [Phys. Rev. Lett. 123, 047202 (2019)] a translationally invariant framework called quantum-electrodynamical Bloch (QED-Bloch) theory was introduced for the description of periodic materials in homogeneous magnetic fields…

Mesoscale and Nanoscale Physics · Physics 2022-05-20 Vasil Rokaj , Markus Penz , Michael A. Sentef , Michael Ruggenthaler , Angel Rubio