Related papers: Parity-Doublet Coherence Times in Optically Trappe…
We report optical trapping of a polyatomic molecule, calcium monohydroxide (CaOH). CaOH molecules from a magneto-optical trap are sub-Doppler laser cooled to $20(3)~\mu\text{K}$ in free space and loaded into an optical dipole trap. We…
We investigate using optically trapped linear polyatomic molecules as probes of nuclear spin-dependent parity violation. The presence of closely spaced, opposite-parity $\ell$-doublets is a general feature of such molecules, allowing…
Qubit coherence times are critical to the performance of any robust quantum computing platform. For quantum information processing using arrays of polar molecules, a key performance parameter is the molecular rotational coherence time. We…
Polyatomic molecules have been identified as sensitive probes of charge-parity violating and parity-violating physics beyond the Standard Model (BSM). For example, many linear triatomic molecules are both laser-coolable and have parity…
Precision searches for time-reversal symmetry violating interactions in polar molecules are extremely sensitive probes of high energy physics beyond the Standard Model. To extend the reach of these probes into the PeV regime, long coherence…
Coherence, the stability of the relative phase between quantum states, lies at the heart of quantum mechanics. Applications such as precision measurement, interferometry, and quantum computation are enabled by physical systems that have…
Collisions between ultracold calcium monohydroxide (CaOH) molecules are realized and studied. Inelastic collision rate constants are measured for CaOH prepared in ground and excited vibrational states, and the electric field dependence of…
The coherence time of an optically trapped neutral atom is a crucial parameter for quantum technologies. We found that optical dipole traps with higher-order spatial forms inherently offer lower decoherence rates compared to those with…
We investigate a parity-time (PT) symmetric system that consists of two symmetrically coupled asymmetric dimers. The enclosed magnetic flux controls the PT phase transition. The system can reenter the exact PT-symmetric phase from a broken…
The preparation of large, low-entropy, highly coherent ensembles of identical quantum systems is foundational for many studies in quantum metrology, simulation, and information. Here, we realize these features by leveraging the favorable…
Polar polyatomic molecules provide an ideal but largely unexplored platform to encode qubits in rotational states. Here, we trap cold (100-600 mK) formaldehyde (H$_2$CO) inside an electric box and perform a Ramsey-type experiment to observe…
Polyatomic molecular ions contain many desirable attributes of a useful quantum system, including rich internal degrees of freedom and highly controllable coupling to the environment. To date, the vast majority of state-specific…
Exposing a molecule to intense light pulses may bring this molecule to a nonstationary quantum state, thus launching correlated dynamics of electronic and nuclear subsystems. Although much had been achieved in the understanding of…
Optical control of polyatomic molecules promises new opportunities in precision metrology, fundamental chemistry, quantum information, and many-body science. Contemporary experimental and theoretical efforts have mostly focused on cycling…
Recently a number of diatomic and polyatomics molecules has been identified as a prospective systems for Doppler/Sisyphus cooling. Doppler/Sisyphus cooling allows to decrease the kinetic energy of molecules down to microkelvin temperatures…
Ultracold polar molecules uniquely combine a rich structure of long-lived internal states with access to controllable long-range, anisotropic dipole-dipole interactions. In particular, the rotational states of polar molecules confined in…
We study the effects of parity-time(PT)-symmetry on the photon blockade and distinguish the different blockade mechanisms in a double-cavity optomechanical system. By studying the light statistics of the system, we find the completely…
The violation of parity (P) and time-reversal (T) symmetry is enhanced in the LaS, LaO and LuO molecules due to the existence of states of opposite parity with small energy differences and the presence of heavy nuclei. We calculate the…
Advanced quantum technologies, such as quantum simulation, computation, and metrology are thriving for the implementation of large-scale configurations of identical quantum systems. Sets of atoms and molecules have the advantage of having…
Precision metrology and quantum measurement often demand matter be prepared in well defined quantum states for both internal and external degrees of freedom. Laser-cooled neutral atoms localized in a deeply confining optical potential…