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Exciton-polaritons offer a versatile platform for realization of all-optical integrated logic gates due to the strong effective optical nonlinearity resulting from the exciton-exciton interactions. In most of the current excitonic materials…

Lead halide perovskites show remarkable performance when used in photovoltaic and optoelectronic devices. However, the peculiarities of light-matter interactions in these materials in general are far from being fully explored experimentally…

Other Condensed Matter · Physics 2022-02-24 A. V. Trifonov , S. Grisard , A. N. Kosarev , I. A. Akimov , D. R. Yakovlev , J. Höcker , V. Dyakonov , M. Bayer

Perovskites have been the focus of attention due to their multitude of outstanding optoelectronic properties and structural versatility. Two-dimensional halide perovskite such as (C_6H_5C_2H_4NH_3)_2PbI_4, or simply PEPI, forms natural…

Materials Science · Physics 2021-03-04 Tanjung Krisnanda , Qiannan Zhang , Kevin Dini , David Giovanni , Timothy C. H. Liew , Tze Chien Sum

Exciton polaritons, hybrid quasiparticles with part-light part-matter nature in semiconductor microcavities, are extensively investigated for striking phenomena such as polariton condensation and quantum emulation. These phenomena have…

Materials Science · Physics 2022-07-27 Tingting Wang , Zhihao Zang , Yuchen Gao , Chao Lyu , Kai Peng , Kenji Watanabe , Takashi Taniguchi , Xiaoze Liu , Wei Bao , Yu Ye

In semiconductors, exciton or charge carrier diffusivity is typically described as an inherent material property. Here, we show that the transport of excitons (i.e., bound electron-hole pairs) in CsPbBr3 perovskite nanocrystals (NCs)…

Perovskites have attracted much attention due to their remarkable optical properties. While it is well established that excitons dominate their optical response, the impact of higher excitonic states and formation of phonon sidebands in…

Mesoscale and Nanoscale Physics · Physics 2020-11-04 David Feldstein , Raul Perea-Causin , Shuli Wang , Mateusz Dyksik , Kenji Watanabe , Takashi Taniguchi , Paulina Plochocka , Ermin Malic

Strong coupling of two-dimensional semiconductor excitons with plasmonic resonators enables control of light-matter interaction at the subwavelength scale. Here we develop strong coupling in plasmonic nano-gap resonators that allow…

Two-dimensional (2D) layered hybrid perovskites provide an ideal platform for studying the properties of excitons. Here, we report on a strong triplet-exciton and longitudinal-optical (LO) phonon coupling in 2D (C6H5CH2CH2NH3, PEA)2PbBr4…

Mesoscale and Nanoscale Physics · Physics 2021-02-26 Yunuan Wang , Feilong Song , Yu Yuan , Jianchen Dang , Xin Xie , Sibai Sun , Sai Yan , Yanbing Hou Zhidong Lou , Xiulai Xu

Strong coupling between lead halide perovskite materials and optical resonators enables both the polaritonic control of the photophysical properties of these emerging semiconductors and the observation of novel fundamental physical…

To assess the potential optoelectronic applications of metal-halide perovskites, it is critical to have a detailed understanding of the nature, strength, and dynamics of the interactions between carriers and the polar lattices. Here, we…

Materials Science · Physics 2022-10-28 Xing He , Naveen Kumar Tailor , Soumitra Satapathi , Jakoah Brgoch , Ding-Shyue Yang

We report on optical spectroscopy (photoluminescence and photoluminescence excitation) on two-dimensional self-organized layers of $(C_{6}H_{5}C_{2}H_{4}-NH_{3})_{2}PbI_{4}$ perovskite. Temperature and excitation power dependance of the…

The effects of the electron-phonon interaction on optical excitations can be understood in terms of exciton-phonon coupling, and require a careful treatment in low-dimensional materials with strongly bound excitons or strong electron-hole…

Materials Science · Physics 2022-02-17 Gabriel Antonius , Steven G. Louie

We investigate the microscopic description of exciton-polaritons that involves electrons, holes and photons within a two-dimensional microcavity. We show that in order to recover the simplified exciton-photon model that is typically used to…

Quantum Gases · Physics 2021-09-06 Jesper Levinsen , Guangyao Li , Meera M. Parish

Exciton-polaritons, elementary excitations arising from the strong coupling regime between photons and excitons in insulators or semiconductors, represent a promising platform for studying quantum fluids of light and realizing prospective…

We investigate the two-pulse photon echo response of excitons in the mixed lead halide perovskite crystal \sample in dependence on the excitation intensity and polarization of the incident laser pulses. Using spectrally narrow picosecond…

Control is exerted over the exciton-polariton physics in metal - Poly(9,9-dioctyl fluorene) - metal microcavities via conformational changes to the polymer backbone. Using thin-film samples containing increasing fractions of $\beta$-phase…

Soft Condensed Matter · Physics 2018-11-21 F. Le Roux , D. D. C. Bradley

Understanding the interplay between bright and dark exciton states is crucial for deciphering the luminescence properties of low-dimensional materials. The origin of the outstanding brightness of lead halide perovskites remains elusive.…

Mesoscale and Nanoscale Physics · Physics 2024-04-16 Mohamed-Raouf Amara , Caixia Huo , Christophe Voisin , Qihua Xiong , Carole Diederichs

Halide perovskites, such as methylammonium lead bromide (MAPbBr$_3$), host tightly bound three-dimensional excitons which are robust at room temperature. Excellent optical properties of MAPbBr$_3$ allow for designing of optical single-mode…

We study experimentally and theoretically the exciton-phonon interaction in MoSe2 monolayers encapsulated in hexagonal BN, which has an important impact on both optical absorption and emission processes. The exciton transition linewidth…

The optical responses of semiconducting transition metal dichalcogenides are dominated by excitons. Being able to strongly interact with light and other materials excitations, excitons in semiconductors are prototypes for investigating…

Mesoscale and Nanoscale Physics · Physics 2021-01-28 Xuke Jiang , Masoud Taleb , Florian Diekmann , Kai Rossnagel , Nahid Talebi