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Metastable cubic tin(II) sulfide ($\pi$-SnS) is an earth-abundant semiconductor whose three-dimensionally bonded chiral lattice may overcome the short minority-carrier lifetime of orthorhombic SnS while maintaining a near-ideal bandgap for…

The theoretical effects of phase separation on encounter-limited charge carrier recombination in organic semiconductor blends are investigated using kinetic Monte Carlo (KMC) simulations of pump-probe experiments. Using model bulk…

Materials Science · Physics 2015-04-06 Michael C. Heiber , Christoph Baumbach , Vladimir Dyakonov , Carsten Deibel

Simulations of charge transport in amorphous semiconductors are often performed in microscopically sized systems. As a result, charge carrier mobilities become system-size dependent. We propose a simple method for extrapolating a…

Statistical Mechanics · Physics 2016-08-03 Pascal Kordt , Thomas Speck , Denis Andrienko

While space-charge-limited current measurements are often used to characterize charge-transport in relatively intrinsic, low-mobility semiconductors, it is currently difficult to characterize lightly or heavily doped semiconductors with…

Applied Physics · Physics 2020-12-02 Jason A. Röhr , Roderick C. I. MacKenzie

We report on systematic numerical study of carrier multiplication (CM) processes in spherically symmetric nanocrystal (NC) and bulk forms of PbSe and PbS representing the test bed for understanding basic aspects of CM dynamics. The adopted…

Mesoscale and Nanoscale Physics · Physics 2015-05-30 Kirill A. Velizhanin , Andrei Piryatinski

We investigate the impact of threading dislocations with an edge component (a or a+c-type) on carrier recombination and diffusion in GaN(0001) layers close to the surface as well as in the bulk. To this end, we utilize cathodoluminescence…

The lifetime of non-equilibrium electrons and holes in semiconductors is crucial for solar cell and optoelectronic applications. Non-adiabatic molecular dynamics (NAMD) simulations based on time-dependent density functional theory (TDDFT)…

Materials Science · Physics 2022-09-19 Shanshan Wang , Menglin Huang , Yu-Ning Wu , Weibin Chu , Jin Zhao , Aron Walsh , Xin-Gao Gong , Su-Huai Wei , Shiyou Chen

Despite the widespread use of Scanning Transmission Electron Microscopy (STEM) for observing the structure of materials at the atomic scale, a detailed understanding of some relevant electron beam damage mechanisms is limited. Recent…

The effect of carrier multiplication (CM) in semiconductor nanocrystals is systematically treated by employing an exciton scattering approach. Using projection operators, we reduce the Coulomb coupled multi-exciton dynamics to scattering…

Mesoscale and Nanoscale Physics · Physics 2010-08-31 Andrei Piryatinski , Kirill A. Velizhanin

State-of-the-art industrial semiconductor device modeling is based on highly efficient Drift-Diffusion (DD) models that include some quantum corrections for nanodevices. In contrast, latest academic quantum transport models are based on the…

Experiments on carrier recombination in two-dimensional organic structures are often interpreted in the frame of the Langevin model with taking into account only the drift of the charge carriers in their mutual electric field. While this…

Disordered Systems and Neural Networks · Physics 2012-01-10 A. V. Nenashev , F. Jansson , S. D. Baranovskii , R. Österbacka , A. V. Dvurechenskii , F. Gebhard

Scanning photocurrent microscopy (SPCM) has been widely used for characterizing charge transport properties, in particular, the minority carrier diffusion length of semiconductors. However, studying lightly doped or intrinsic semiconductors…

Materials Science · Physics 2024-10-10 Xiujun Lian , Hanwei Gao

In developing photovoltaic devices with high efficiencies, quantitative determination of the carrier loss is crucial. In conventional solar-cell characterization techniques, however, photocurrent reduction originating from parasitic light…

We present a new semi-empirical model for calculating electron transport in atomic-scale devices. The model is an extension of the Extended H\"uckel method with a self-consistent Hartree potential. This potential models the effect of an…

Mesoscale and Nanoscale Physics · Physics 2012-04-04 Kurt Stokbro , Dan Erik Petersen , Søren Smidstrup , Anders Blom , Mads Ipsen , Kristen Kaasbjerg

The investigation of novel electronic phases in low-dimensional quantum materials demands for the concurrent development of new measurement techniques that combine surface sensitivity with high spatial resolution and high measurement…

Mesoscale and Nanoscale Physics · Physics 2020-10-14 Berthold Jäck

A simple yet precise optical technique for measuring the ambipolar carrier mobility in semiconductors is presented. Using tightly focused Gaussian laser beams in a photo-reflectance system, the modulated reflectance signal is measured as a…

Instrumentation and Detectors · Physics 2017-11-06 Will Chism

Quantum dot (QD) solids are being widely exploited as a solution-processable technology to develop photovoltaic, light-emission, and photo-detection devices. Charge transport in these materials is the result of a compromise between…

Topological insulators are guaranteed to support metallic surface states on an insulating bulk, and one should thus expect that the electronic transport in these materials is dominated by the surfaces states. Alas, due to the high remaining…

Here we describe an optical method to determine the dynamics of optically excited carriers in nanostructured composite samples. By combining pump-probe time-resolved reflectivity with scattering measurements, we extract the characteristic…

Mesoscale and Nanoscale Physics · Physics 2015-06-05 J. Barreto , T. Roger , A. Kaplan

We have developed and applied a mobility edge model that takes into account drift and diffusion currents to characterize the space charge limited current in organic semiconductors. The numerical solution of the drift-diffusion equation…

Materials Science · Physics 2015-05-30 Javier Dacuña , Alberto Salleo