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Quantum spin rings represent an intriguing platform for studying unconventional magnetic order and exotic quantum phases, and they are also promising materials for emerging quantum technologies. Conventional spin systems consist of a set of…
The emergence of spinon quasiparticles, which carry spin but lack charge, is a hallmark of collective quantum phenomena in low-dimensional quantum spin systems. While the existence of spinons has been demonstrated through scattering…
The design and control of atomic-scale spin structures constitute major challenges for spin-based quantum technology platforms, including quantum dots, color centers, and molecular spins. Here, we showcase a strategy for designing the…
Spin-1/2 Heisenberg antiferromagnetic chains are excellent one-dimensional platforms for exploring quantum magnetic states and quasiparticle fractionalization. Understanding its quantum magnetism and quasiparticle excitation at the atomic…
Achieving long-range ferrimagnetic order in purely organic systems remains a major challenge in molecular magnetism. Here we report the synthesis and characterization of heterospin-coupling motifs, formed by covalently linking spin-1/2 and…
Quantum spin networks having engineered geometries and interactions are eagerly pursued for quantum simulation and access to emergent quantum phenomena such as spin liquids. Spin-1/2 centers are particularly desirable because they readily…
Assemblies of interacting quantum particles often surprise us with properties that are difficult to predict. One of the simplest quantum many-body systems is the spin 1/2 Heisenberg antiferromagnetic chain, a linear array of interacting…
Carbon-based nanostructures possessing {\pi}-electron magnetism have attracted tremendous interest due to their great potential for nano spintronics. In particular, quantum chains with magnetic molecular units synthesized by on-surface…
A fundamental motif in frustrated magnetism is the fully mutually coupled cluster of $N$ spins, with each spin coupled to every other spin. Clusters with $N=2$ and $3$ have been extensively studied as building blocks of square and…
We study the motion of a charged quantum particle, constrained on the surface of a cylinder, in the presence of a radial magnetic field. When the spin of the particle is neglected, the system essentially reduces to an infinite family of…
The Penrose tiling is a perfectly ordered two dimensional structure with fivefold symmetry and scale invariance under site decimation. Quantum spin models on such a system can be expected to differ significantly from more conventional…
Artificial quantum systems have emerged as indispensable platforms to realize exotic topological matter in a well-controlled manner. Here, we demonstrate topological quantum Heisenberg spin lattices, engineered with spin chains and…
We introduce a model compound featuring a spin-1/2 frustrated square lattice partially coupled by spin-5/2. A significant magnetization plateau exceeding 60 T could be observed, indicating a quantum state formed by $S$ = 1/2 spins in the…
Triangulenes are prototypical examples of open-shell nanographenes. Their magnetic properties, arising from the presence of unpaired $\pi$ electrons, can be extensively tuned by modifying their size and shape or by introducing heteroatoms.…
Understanding exotic forms of magnetism in quantum spin systems is an emergent topic of modern condensed matter physics. Quantum dynamics can be described by particle-like carriers of information, known-as quasiparticles that appear from…
The ground states of artificial molecules made of two vertically coupled quantum rings are studied within the spin density functional theory for systems containing up to 13 electrons. Quantum tunneling effects on the electronic structure of…
We report structural and magnetic properties of the spin-$\frac12$ quantum antiferromagnet Cu[C$_6$H$_2$(COO)$_4$][C$_2$H$_5$NH$_3$]$_2$ by means of single-crystal x-ray diffraction, magnetization, heat capacity, and electron spin resonance…
A semiclassical theory of a quantum spin$-S$ model with competing ring and Heisenberg exchange terms on the triangular lattice is obtained. A mechanism for the generation of $Z_2$ vortices is exhibited. The vortices are shown to carry a…
This study deals with the further development of nuclear spin model of scalable quantum register, which presents the one-dimensional chain of the magnetic atoms with nuclear spins 1/2, substituting the basic atoms in the plate of nuclear…
Dangling edge spins of dimerized two-dimensional spin-1 Heisenberg antiferromagnets are shown to exhibit nonordinary quantum critical correlations, akin to the scaling behavior observed in recently explored spin-1/2 systems. Based on…