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We demonstrate the deceleration of heavy polar molecules in low-field seeking states by combining a cryogenic source and a travelling-wave Stark decelerator. The cryogenic source provides a high intensity beam with low speed and…

Cryogenic buffer-gas beams are a promising method for producing bright sources of cold molecular radicals for cold collision and chemical reaction experiments. In order to use these beams in studies of reactions with controlled collision…

Chemical Physics · Physics 2015-06-18 M. I. Fabrikant , Tian Li , N. J. Fitch , N. Farrow , Jonathan D. Weinstein , H. J. Lewandowski

We present experiments on decelerating and trapping ammonia molecules using a combination of a Stark decelerator and a traveling wave decelerator. In the traveling wave decelerator a moving potential is created by a series of ring-shaped…

Stark deceleration is a technique that uses time-varying inhomogeneous electric fields to decelerate polar molecules for various molecular beam and trapping experiments. New ring-geometry Stark decelerators with continuously varying…

Chemical Physics · Physics 2017-12-20 Yomay Shyur , Jason A. Bossert , H. J. Lewandowski

A Stark decelerator is an effective tool for controlling motional degrees of freedom of polar molecules. Due to technical limitations, many of the current Stark decelerators focus on molecules in low-field-seeking quantum states and are…

Atomic Physics · Physics 2017-05-25 Demitri Y. Balabanov , Liam M. Duffy

We report on the electrostatic trapping of neutral SrF molecules. The molecules are captured from a cryogenic buffer-gas beam source into the moving traps of a 4.5 m long traveling-wave Stark decelerator. The SrF molecules in…

We describe the production of cold, slow-moving LiH molecules. The molecules are produced in the ground state using laser ablation and supersonic expansion, and 68% of the population is transferred to the rotationally excited state using…

Atomic Physics · Physics 2015-05-13 S. K. Tokunaga , J. M. Dyne , E. A. Hinds , M. R. Tarbutt

We report on the production, deceleration and detection of a SrF molecular beam. The molecules are captured from a supersonic expansion and are decelerated in the X$^2\Sigma^+ (v=0, N=1)$ state. We demonstrate the removal of up to 40% of…

Stark deceleration enables the production of cold and dense molecular beams with applications in trapping, collisional studies, and precision measurement. Improving the efficiency of Stark deceleration, and hence the achievable molecular…

Chemical Physics · Physics 2020-07-22 David Reens , Hao Wu , Alexander Aeppli , Anna McAuliffe , Piotr Wcisło , Tim Langen , Jun Ye

We have designed and implemented a new Stark decelerator based on wire electrodes, which is suitable for ultrahigh vacuum applications. The 100 deceleration stages are fashioned out of 0.6 mm diameter tantalum and the array's total length…

Atomic Physics · Physics 2010-09-28 Adela Marian , Henrik Haak , Peter Geng , Gerard Meijer

We report on the deceleration of a beam of SrF molecules from 290 to 120~m/s. Following supersonic expansion, the molecules in the $X^2\Sigma$ ($v=0$, $N=1$) low-field seeking states are trapped by the moving potential wells of a…

Atomic Physics · Physics 2019-07-17 S. C. Mathavan , A. Zapara , Q. Esajas , S. Hoekstra

Stark deceleration allows for precise control over the velocity of a pulsed molecular beam and, by the nature of its limited phase-space acceptance, reduces the energy width of the decelerated packet. We describe an alternate method of…

Atomic Physics · Physics 2015-05-13 L. P. Parazzoli , N. Fitch , D. S. Lobser , H. J. Lewandowski

With a Stark decelerator, beams of neutral polar molecules can be accelerated, guided at a constant velocity, or decelerated. The effectiveness of this process is determined by the 6D volume in phase space from which molecules are accepted…

Atomic and Molecular Clusters · Physics 2009-11-13 Ludwig Scharfenberg , Henrik Haak , Gerard Meijer , Sebastiaan Y. T. van de Meerakker

We present an analysis of the deceleration and trapping of heavy diatomic molecules in low-field seeking states by a moving electric potential. This moving potential is created by a 'ring-decelerator', which consists of a series of…

High peak power, tunable, narrowband terahertz emitters are becoming sought after given their portability, efficiency, and ability to be deployed in the field for industrial, medical, and military applications. The use of accelerator…

Producing large samples of slow molecules from thermal-velocity ensembles is a formidable challenge. Here we employ a centrifugal force to produce a continuous molecular beam with a high flux at near-zero velocities. We demonstrate…

Chemical Physics · Physics 2018-12-04 S. Chervenkov , X. Wu , J. Bayerl , A. Rohlfes , T. Gantner , M. Zeppenfeld , G. Rempe

Operating the SLAC/KEK DDS (Damped Detuned Structure) X-band linacs at high gradients (in excess of 70MV/m) has recently been found to be limited by the accelerator structures breaking down and as a consequence severe damage occurs to the…

Accelerator Physics · Physics 2008-11-26 R. M. Jones , N. M. Kroll , T. Higo , R. H. Miller , R. D Ruth

We here report on the experimental realization of a microwave decelerator for neutral polar molecules, suitable for decelerating and focusing molecules in high-field-seeking states. The multi-stage decelerator consists of a cylindrical…

Chemical Physics · Physics 2015-06-04 Simon Merz , Nicolas Vanhaecke , Wolfgang Jäger , Melanie Schnell , Gerard Meijer

Recently, a decelerator for neutral polar molecules has been presented that operates on the basis of macroscopic, three-dimensional, traveling electrostatic traps (Osterwalder et al., Phys. Rev. A 81, 051401 (2010)). In the present paper, a…

High-harmonic generation (HHG) normally requires a careful adjustment of the driving laser intensity (typically $10^{14} - 10^{15}$ W/cm$^2$) and gas medium parameters to enable good phase matching conditions. In contrast with conventional…

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