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Blinking and multiphoton emission in metal halide perovskite quantum dots (PQDs) limit their use as single-photon quantum emitters. Conventional models distinguish between trion-related A-type blinking and defect-assisted BC-type blinking,…

Mesoscale and Nanoscale Physics · Physics 2026-02-13 Adam Olejniczak , Jehyeok Ryu , Francesco Di Stasio , Yury Rakovich , Victor Krivenkov

III-nitride quantum dots (QDs) are a promising system actively studied for their ability to maintain single photon emission up to room temperature. Here, we report on the evolution of the emission properties of self-assembled GaN/AlN QDs…

Lead halide perovskite nanocrystals are promising materials for classical and quantum light emission. To understand these outstanding properties, a thorough analysis of the band-edge exciton emission is needed which is not reachable in…

Mesoscale and Nanoscale Physics · Physics 2023-04-07 Mohamed-Raouf Amara , Zakaria Said , Caixia Huo , Aurélie Pierret , Christophe Voisin , Weibo Gao , Qihua Xiong , Carole Diederichs

Tailored quantum states of light can be created via a transfer of collective quantum states of matter to light modes. Such collective quantum states emerge in interacting many-body systems if thermal fluctuations are overcome by sufficient…

Atomic Physics · Physics 2018-11-14 F. Ripka , H. Kübler , R. Löw , T. Pfau

The coherence of collective modes, such as phonons, and their modulation of the electronic states are long sought in complex systems, which is a cross-cutting issue in photovoltaics and quantum electronics. In photovoltaic cells and lasers…

Materials Science · Physics 2020-03-23 Z. Liu , C. Vaswani , L. Luo , D. Cheng , X. Yang , X. Zhao , Y. Yao , Z. Song , R. Brenes , R. Kim , J. Jean , V. Bulovic , Y. Yan , K. -M. Ho , J. Wang

Chemically prepared colloidal semiconductor quantum dots have long been proposed as scalable and color-tunable single emitters in quantum optics, but they have typically suffered from prohibitively incoherent emission. We now demonstrate…

We investigate room temperature lasing of terahertz quantum cascade lasers using quantum dot chains as active material suitable for wireless communication and imaging technologies. Bandstructure calculations for such extended systems of…

Mesoscale and Nanoscale Physics · Physics 2021-03-10 Alexander Mittelstädt , Ludwig A. Th. Greif , Stefan T. Jagsch , Andrei Schliwa

The power conversion efficiency of photovoltaic devices based on semiconductor perovskites has reached ~20% after just several years of research efforts. With concomitant discoveries of other promising applications in lasers, light-emitting…

The high optoelectronic quality of halide perovskites lends them to be utilized in optoelectronic devices and recently in emerging quantum emission applications. Advancements in perovskite nanomaterials have led to the discovery of…

Highly correlated photon sources can be realized through cooperative coupling among quantum systems, giving rise to superradiant collective emission. In solid-state ensembles, however, such collective behaviour is confined to subwavelength…

Applied Physics · Physics 2026-05-18 Marco Marangi , Alexander M. Dubrovkin , Anton N. Vetlugin , Giorgio Adamo , Cesare Soci

Quantum emitters of single indistinguishable photons play a key role in quantum technologies. Among condensed matter systems, colloidal perovskite quantum dots have emerged as promising candidates, exhibiting high-purity single photon…

Colloidal semiconductor quantum dots (QDs) are excellent luminescent nanomaterials for a broad range of optoelectronic applications. Their photoluminescence blinking, however, hinders their practical use in many aspects. It has been shown…

Optics · Physics 2024-02-27 Zhiyuan Wang , Jianwei Tang , Jiahao Han , Juan Xia , Tianzi Ma , Xue-Wen Chen

Photoluminescence intermittency remains one of the biggest challenges to realizing perovskite quantum dots (QDs) as scalable single photon emitters. We compare CsPbBr3 QDs capped with different ligands, lecithin, and a combination of oleic…

Colloidal perovskite quantum dots (PQDs) are an exciting platform for on-demand quantum, and classical optoelectronic and photonic devices. However, their potential success is limited by the extreme sensitivity and low stability arising…

Current technologies for X-ray detection rely on scintillation from expensive inorganic crystals grown at high-temperature, which so far has hindered the development of large-area scintillator arrays. Thanks to the presence of heavy atoms,…

Instrumentation and Detectors · Physics 2016-11-21 M. D. Birowosuto , D. Cortecchia , W. Drozdowski , K. Brylew , W. Lachmanski , A. Bruno , C. Soci

Biexcitons are a manifestation of many-body excitonic interactions crucial for quantum information and quantum computation in the construction of coherent combinations of quantum states. However, due to their small binding energy and low…

Colloidal core/shell InP/ZnSe quantum dots (QDs), recently produced using an improved synthesis method, have a great potential in life-science applications as well as in integrated quantum photonics and quantum information processing as…

Mesoscale and Nanoscale Physics · Physics 2017-11-22 Vigneshwaran Chandrasekaran , Mickaël D. Tessier , Dorian Dupont , Pieter Geiregat , Zeger Hens , Edouard Brainis

Perovskite quantum dots (PQDs) provide a robust solution-based approach to efficient solar cells, bright light-emitting devices, and quantum sources of light. Quantifying heterogeneity and understanding coupling between dots is critical for…

We report the first doping of crystalline methylammonium lead bromide (MAPbBr$_3$) perovskite thin-films with CdSe/CdZnS core/shell quantum dots (QDs), using a soft-chemistry method that preserves their high quantum yield and other…

Chemical Physics · Physics 2021-10-26 Justine Baronnier , Julien Houel , Christophe Dujardin , Florian Kulzer , Benoit Mahler

Superfluorescence, the cooperative burst of spontaneous emission from an ensemble of dipoles, arises when microscopic oscillators spontaneously synchronize their phases. Here we show that this process can be reversed in time within quantum…