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Liquid chromatography mass spectrometry (LC-MS)-based metabolomics and exposomics aim to measure detectable small molecules in biological samples. The results facilitate hypothesis-generating discovery of metabolic changes and disease…

Quantitative Methods · Quantitative Biology 2026-01-06 Xujun Che , Xiuxia Du , Depeng Xu

Chemical formula annotation for tandem mass spectrometry (MS/MS) data is the first step toward structurally elucidating unknown metabolites. While great strides have been made toward solving this problem, the current state-of-the-art method…

Quantitative Methods · Quantitative Biology 2023-10-24 Samuel Goldman , Jiayi Xin , Joules Provenzano , Connor W. Coley

Mass spectrometry (MS) stands as a cornerstone analytical technique for molecular identification, yet de novo structure elucidation from spectra remains challenging due to the combinatorial complexity of chemical space and the inherent…

Machine Learning · Computer Science 2026-03-20 Jianan Nie , Peng Gao

Tandem Mass Spectrometry is a cornerstone technique for identifying unknown small molecules in fields such as metabolomics, natural product discovery and environmental analysis. However, certain aspects, such as the probabilistic…

Artificial Intelligence · Computer Science 2026-01-19 Laura Mismetti , Marvin Alberts , Andreas Krause , Mara Graziani

To facilitate the understanding and to quantitatively assess the material transport in fluids, a modern characterisation method has emerged in fluid dynamics in the last decades footed in dynamical systems theory. It allows to examine the…

The discovery and identification of molecules in biological and environmental samples is crucial for advancing biomedical and chemical sciences. Tandem mass spectrometry (MS/MS) is the leading technique for high-throughput elucidation of…

Electrospray tandem mass spectrometry (ESI-MS/MS) is commonly used in high throughput metabolomics. One of the key obstacles to the effective use of this technology is the difficulty in interpreting measured spectra to accurately and…

Computational Engineering, Finance, and Science · Computer Science 2014-06-10 F. Allen , R. Greiner , D. Wishart

Generative molecular design has moved from proof-of-concept to real-world applicability, as marked by the surge in very recent papers reporting experimental validation. Key challenges in explainability and sample efficiency present…

Biomolecules · Quantitative Biology 2024-03-05 Jeff Guo , Philippe Schwaller

Machine learning methods for identifying molecular structures from tandem mass spectra (MS/MS) have advanced rapidly, yet current approaches still exhibit significant error rates. In high-stakes applications such as clinical metabolomics…

Machine Learning · Computer Science 2026-03-12 Mira Jürgens , Gaetan De Waele , Morteza Rakhshaninejad , Willem Waegeman

Determining atomistic structures from characterization data is one of the most common yet intricate problems in materials science. Particularly in amorphous materials, proposing structures that balance realism and agreement with experiments…

Disordered Systems and Neural Networks · Physics 2026-03-25 Jiawei Guo , Daniel Schwalbe-Koda

A vast majority of mass spectrometry data remains uncharacterized, leaving much of its biological and chemical information untapped. Recent advances in machine learning have begun to address this gap, particularly for tasks such as spectral…

Molecular design requires systematic and broadly applicable methods to extract structure-property relationships. The focus of this study is on learning thermodynamic properties from molecular-liquid simulations. The methodology relies on an…

Materials Science · Physics 2023-07-04 Bernadette Mohr , Diego van der Mast , Tristan Bereau

Compound identification and structure annotation from mass spectra is a well-established task widely applied in drug detection, criminal forensics, small molecule biomarker discovery and chemical engineering. We propose SpecTUS: Spectral…

Machine Learning · Computer Science 2026-02-23 Adam Hájek , Michal Starý , Elliott Price , Filip Jozefov , Helge Hecht , Aleš Křenek

Identifying a small molecule from its mass spectrum is the primary open problem in computational metabolomics. This is typically cast as information retrieval: an unknown spectrum is matched against spectra predicted computationally from a…

Machine Learning · Computer Science 2023-01-30 Michael Murphy , Stefanie Jegelka , Ernest Fraenkel , Tobias Kind , David Healey , Thomas Butler

Structural identifiability analysis of fractional-order equivalent circuit models (FO-ECMs), obtained through electrochemical impedance spectroscopy (EIS) is still a challenging problem. No peer-reviewed analytical or numerical proof does…

Systems and Control · Electrical Eng. & Systems 2021-03-02 Tohid Soleymani Aghdam , Seyed Mohammad Mahdi Alavi , Mehrdad Saif

Automated molecular structure elucidation remains challenging, as existing approaches often depend on pre-compiled databases or restrict themselves to single spectroscopic modalities. Here we introduce SpectraLLM, a large language model…

Quantitative Methods · Quantitative Biology 2026-05-12 Yunyue Su , Jiahui Chen , Zao Jiang , Zhenyi Zhong , Liang Wang , Qiang Liu , Zhaoxiang Zhang

Metabolites, small molecules that are involved in cellular reactions, provide a direct functional signature of cellular state. Untargeted metabolomics experiments usually relies on tandem mass spectrometry to identify the thousands of…

Quantitative Methods · Quantitative Biology 2015-01-29 Kai Dührkop , Sebastian Böcker

Combinatorial optimization (CO) problems, central to operation research and theoretical computer science, present significant computational challenges due to their NP-hard nature. While large language models (LLMs) have emerged as promising…

Machine Learning · Computer Science 2025-06-16 Xijun Li , Jiexiang Yang , Jinghao Wang , Bo Peng , Jianguo Yao , Haibing Guan

Grain-edge segmentation (GES) and lithology semantic segmentation (LSS) are two pivotal tasks for quantifying rock fabric and composition. However, these two tasks are often treated separately, and the segmentation quality is implausible…

Computer Vision and Pattern Recognition · Computer Science 2026-04-17 Yili Ren , Shiqi Wen , Li Hou , Dingwen Xiao , Weiming Zhang , Caleb Chen Cao , Lin Wang , Zilu Zheng , Qianxiao Su , Mingjun Zhao , Lei Chen

Accurate diagnosis of glaucoma is challenging, as early-stage changes are subtle and often lack clear structural or appearance cues. Most existing approaches rely on a single modality, such as fundus or optical coherence tomography (OCT),…

Computer Vision and Pattern Recognition · Computer Science 2026-03-24 Zhiwei Wang , Yuxing Li , Meilu Zhu , Defeng He , Edmund Y. Lam
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