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The planned measurement of optical resonances in singly-ionised lawrencium (Z = 103) requires accurate theoretical predictions to narrow the search window. We present high-precision, ab initio calculations of the electronic spectra of…

Atomic Physics · Physics 2019-12-18 E. V. Kahl , J. C. Berengut , M. Laatiaoui , E. Eliav , A. Borschevsky

Planned optical spectroscopy experiments in lawrencium (Lr, Z = 103) require accurate theoretical predictions of the location of spectral lines in order to narrow the experimental search window. We present ab initio calculations of the…

Atomic and Molecular Clusters · Physics 2021-12-01 E. V. Kahl , S. Raeder , E. Eliav , A. Borschevsky , J. C. Berengut

Theory can provide important support at all the stages of spectroscopic experiments, from planning the measurements to the interpretation of the results. Such support is particularly valuable for the challenging experiments on heavy,…

Atomic Physics · Physics 2025-09-19 L. F. Pašteka , E. Eliav , M. L. Reitsma , A. Borschevsky

We report calculation of the energy spectrum and the spectroscopic properties of the superheavy element ion: Rf^+. We use the 4-component relativistic Dirac-Coulomb Hamiltonian and the multireference configuration interaction (MRCI) model…

Atomic Physics · Physics 2021-08-24 Harry Ramanantoanina , Anastasia Borschevsky , Michael Block , Mustapha Laatiaoui

We report first results obtained during the commissioning of the Laser Resonance Chromatography (LRC) apparatus, which is conceived to enable atomic structure investigations in the region of the heaviest elements beyond nobelium. In our…

We employ a technique that combines the configuration interaction method with the singles-doubles coupled-cluster method to perform calculation of the energy levels, transition amplitudes, lifetimes, g-factors, and magnetic dipole and…

Atomic Physics · Physics 2020-05-08 V. A. Dzuba , V. V. Flambaum , B. M. Roberts

The LiFr diatomic represents a promising candidate for indirect laser cooling that has not yet been investigated not theoretically or experimentally. The potential energy curves of the ground and low_lying excited states of the LiFr…

Atomic Physics · Physics 2023-12-29 Maksim Shundalau , Patrizia Lamberti

This work presents accurate ab initio determination of the hyperfine splitting for the ground state and few low-lying excited states of 113Cd+; important candidates for the frequency standard in the microwave region, using coupled-cluster…

Atomic Physics · Physics 2009-11-13 Gopal Dixit , H. S. Nataraj , B. K. Sahoo , R. K. Chaudhuri , Sonjoy Majumder

Radium compounds have attracted recently considerable attention due to both development of experimental techniques for high-precision laser spectroscopy of molecules with short-lived nuclei and amenability of certain radium compounds for…

In this study a comprehensive calculations of energies, hyperfine structure constants, Land\'e g$_J$ factors and isotope shifts have been performed for the lowest 71 states of Na-like Ar$^{7+}$, Kr$^{25+}$ and Xe$^{43+}$ ions. Radiative…

Atomic Physics · Physics 2025-01-22 Shikha Rathi , Lalita Sharma

In this chapter we focus first on the theoretical methods and relevant computational approaches to calculate the electronic structure of atoms, molecules, and clusters containing heavy elements for which relativistic effects become…

Chemical Physics · Physics 2021-10-05 Simone Taioli , Stefano Simonucci

The 12C+12C fusion reaction is famous for its complication of molecular resonances, and plays an important role in both nuclear structure and astrophysics. It is extremely difficult to measure the cross sections of 12C+12C fusions at…

Nuclear Experiment · Physics 2020-05-26 Xiaodong Tang , Shaobo Ma , Xiao Fang , Brian Bucher , Adam Alongi , Craig Cahillane , Wanpeng Tan

Accurate ab initio calculations of the energy levels of the superheavy elements Z=112 are presented. Relativistic Hartree-Fock and configuration interaction methods are combined with the many-body perturbation theory to construct the…

Atomic Physics · Physics 2010-09-20 T. H. Dinh , V. A. Dzuba , V. V. Flambaum

Recently a breakthrough has been achieved in laser-spectroscopic studies of short-lived radioactive compounds with the first measurements of the radium monofluoride molecule (RaF) UV/vis spectra. We report results from high accuracy…

High-precision calculations of the energy levels of the superheavy element Z=120 are presented. The relativistic Hartree-Fock and configuration interaction techniques are employed. The correlations between core and valence electrons are…

Atomic Physics · Physics 2022-01-07 T. H. Dinh , V. A. Dzuba , V. V. Flambaum , J. S. M. Ginges

We perform accurate calculations of the dependence of transition frequencies in two valence electron atoms and ions on a variation of the fine structure constant, alpha. The relativistic Hartree-Fock method is used with many-body…

Atomic Physics · Physics 2009-02-05 E. J. Angstmann , V. A. Dzuba , V. V. Flambaum

While the ongoing search to discover new high-entropy systems is slowly expanding beyond metals, a rational and effective method for predicting "in silico" the solid solution forming ability of multi-component systems remains yet to be…

Materials Science · Physics 2018-07-16 Yoav Lederer , Cormac Toher , Kenneth S. Vecchio , Stefano Curtarolo

Ab initio linear-response calculations are reported of the phonon spectra and the electron-phonon interaction for several transition metal carbides and nitrides in a NaCl-type structure. For NbC, the kinetic, optical, and superconducting…

Superconductivity · Physics 2009-11-11 E. G. Maksimov , S. V. Ebert , M. V. Magnitskaya , A. E. Karakozov , S. Yu. Savrasov

Precision spectroscopy of atomic systems is an invaluable tool for the advancement of our understanding of fundamental interactions and symmetries. Recently, highly charged ions (HCI) have been proposed for sensitive tests of physics beyond…

Roles of electron correlation effects in the determination of attachment energies, magnetic dipole hyperfine structure constants and electric dipole (E1) matrix elements of the low-lying states in the singly charged cadmium ion (Cd$^+$)…

Atomic Physics · Physics 2018-03-14 Cheng-Bin Li , Yan-Mei Yu , B. K. Sahoo
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