English
Related papers

Related papers: Relativistic quintuple-zeta basis sets for the p b…

200 papers

In this work we develop new finite element discretisations of the shear-deformable Reissner--Mindlin plate problem based on the Hellinger-Reissner principle of symmetric stresses. Specifically, we use conforming Hu-Zhang elements to…

Numerical Analysis · Mathematics 2023-05-30 Adam Sky , Michael Neunteufel , Jack S. Hale , Andreas Zilian

We present a systematic study of the performance of numerical pseudo-atomic orbital basis sets in the calculation of dielectric matrices of extended systems using the self-consistent Sternheimer approach of [F. Giustino et al., Phys. Rev. B…

Materials Science · Physics 2015-06-04 Hannes Hübener , Miguel A. Pérez-Osorio , Pablo Ordejón , Feliciano Giustino

Localization of molecular orbitals finds its importance in the representation of chemical bonding (and anti-bonding) and in the local correlation treatments beyond mean-field approximation. In this paper, we generalize the intrinsic atomic…

Chemical Physics · Physics 2021-02-11 Bruno Senjean , Souloke Sen , Michal Repisky , Gerald Knizia , Lucas Visscher

This work presents a first time accurate calculation of the magnetic dipole hyperfine structure constants for the ground state and some low-lying excited states of Pb$^+$. By comparing different levels of approximation with experimental…

Atomic Physics · Physics 2009-11-10 Bijaya K. Sahoo , Rajat K. Chaudhuri , B. P. Das , Holger Merlitz , Debashis Mukherjee

This review addresses the practical convergence of the ChPT series in the p-regime. In the SU(2) framework there is a number of new results, and improved estimates of \bar\ell_3 and \bar\ell_4 are available. In the SU(3) framework few new…

High Energy Physics - Lattice · Physics 2013-05-27 Stephan Durr

Electronic structure methods for accurate calculation of molecular properties have a high cost that grows steeply with the problem size, therefore, it is helpful to have the underlying atomic basis functions that are less in number but of…

Chemical Physics · Physics 2019-03-15 Dimitri N. Laikov

Core-level spectra of 1s electrons of elements heavier than Ne show significant relativistic effects. We combine advances in orbital optimized DFT (OO-DFT) with the spin-free exact two-component (X2C) model for scalar relativistic effects,…

Chemical Physics · Physics 2022-04-19 Leonardo A. Cunha , Diptarka Hait , Richard Kang , Yuezhi Mao , Martin Head-Gordon

We illustrate how the systematic inclusion of multi-spin correlations of the quantum spin-lattice systems can be efficiently implemented within the framework of the coupled-cluster method by examining the ground-state properties of both the…

Statistical Mechanics · Physics 2017-08-24 Chen Zeng , D. J. J. Farnell , R. F. Bishop

This paper presents the derivation of a kinetic-balance condition for explicitly correlated basis functions employed in semi-classical relativistic calculations. Such a condition is important to ensure variational stability in algorithms…

Chemical Physics · Physics 2015-10-26 Benjamin Simmen , Edit Mátyus , Markus Reiher

It is shown that four-component (4C), quasi-four-component (Q4C), and exact two-component (X2C) relativistic Hartree-Fock (HF) equations can be implemented in an unified manner, by making use of the atomic nature of the small components of…

Chemical Physics · Physics 2023-11-28 Wenjian Liu

A new family of Gaussian-type basis sets named sigma basis sets is presented and preliminarily tested. Sigma basis sets for H, C, N, O and P are reported and their performance is tested in some atomic and molecular calculations.

Computational Physics · Physics 2022-07-07 Ignacio Ema , Guillermo Ramírez , Rafael López , José Manuel García de la Vega

We consider ground state energies (GSE) of multipartite $p$-spin models. Relying on partially lifted random duality theory (pl RDT) concepts we introduce an analytical mechanism that produces easy to compute lower and upper GSE bounds for…

Probability · Mathematics 2025-09-09 Mihailo Stojnic

In this paper, we consider the Dirac-Hartree-Fock equations for system has many-particles. The difficulties associated with Gaussians model are likely to be more complex in relativistic Dirac-Hartree-Fock calculations. To processing these…

Atomic Physics · Physics 2019-12-11 Bilal K. Jasim , Ayad A. Al-Ani. Saad N. Abood

The total atomization energy of a molecule is the thermochemical cognate of the heat of formation in the gas phase, its most fundamental thermochemical property. We decompose it into different components and provide a survey of them. It…

Chemical Physics · Physics 2022-11-01 Jan M. L. Martin

Atomic cluster expansion (ACE) methods provide a systematic way to describe particle local environments of arbitrary body order. For practical applications it is often required that the basis of cluster functions be symmetrized with respect…

Materials Science · Physics 2024-02-27 James M. Goff , Charles Sievers , Mitchell A. Wood , Aidan P. Thompson

In this study, we present a general workflow that enables the automatic generation of auxiliary density basis sets for all elements of the periodic table (from H to Og) to facilitate the general applicability of relativistic Dirac-Kohn-Sham…

Chemical Physics · Physics 2025-06-19 Nicolo' Antonini , Enrico Ronca , Loriano Storchi , Leonardo Belpassi

The concepts of localizable set, localization of a ring and a module at a localizable set are introduced and studied. Localizable sets are generalization of Ore sets and denominator sets, and the localization of a ring/module at a…

Rings and Algebras · Mathematics 2021-12-28 V. V. Bavula

A thorough consideration of the relation between the lattice parameters of 185 binary and ternary spinel compounds, on one side, and ionic radii and electronegativities of the constituting ions, on the other side, allowed for establishing a…

Materials Science · Physics 2014-05-20 M. G. Brik , A. Suchocki , A. Kamińska

New low-order $H(\textrm{div})$-conforming finite elements for symmetric tensors are constructed in arbitrary dimension. The space of shape functions is defined by enriching the symmetric quadratic polynomial space with the $(d+1)$-order…

Numerical Analysis · Mathematics 2024-02-22 Xuehai Huang , Chao Zhang , Yaqian Zhou , Yangxing Zhu

Rigorous quantum formulation of the Parity-Time (PT) symmetry phenomenon in the RF/microwave regime for a coupled coil resonators with lump elements has been presented. The coil resonator is described by the lump-element model that consists…

Systems and Control · Electrical Eng. & Systems 2020-07-06 Shaolin Liao , Lu Ou