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We develop photoelectron interferometry based on laser-assisted extreme ultraviolet ionization for flexible and robust control of photoelectron circular dichroism in randomly oriented chiral molecules. A comb of XUV photons ionizes a sample…

Laser-driven high-order harmonic generation (HHG) provides tabletop sources of broadband extreme-ultraviolet (XUV) light with excellent spatial and temporal coherence. These sources are typically operated at low repetition rates,…

The irradiation of atoms by a strong IR laser field of frequency $\omega$ results in the emission of odd-harmonics of $\omega$ ("IR harmonics") up to some maximal cut-off frequency. The addition of an XUV field of frequency…

Atomic Physics · Physics 2008-02-04 Avner Fleischer , Nimrod Moiseyev

The goal to control short-wavelength radiation for the investigation and manipulation of ultrafast dynamics in quantum systems coevolves with the growing availability of extreme-ultraviolet (XUV) and x-ray sources from high-harmonic…

In this work we study the impact of chromatic focusing of few-cycle laser pulses on high-order harmonic generation (HHG) through analysis of the emitted extreme ultraviolet (XUV) radiation. Chromatic focusing is usually avoided in the…

Ionization of atoms and molecules in laser fields can lead to various interesting interference structures in the photoelectron spectrum. For the case of a super-intense extreme ultraviolet laser pulse, we identify a novel petal-like…

Atomic Physics · Physics 2022-03-29 Lei Geng , Hao Liang , K. Krajewska , Liang-You Peng , Qihuang Gong

We study the generation of attosecond XUV pulses via high-order frequency mixing (HFM) of two intense generating fields, and compare this process with the more common high-order harmonic generation (HHG) process. We calculate the…

Optics · Physics 2023-08-07 V. A. Birulia , M. A. Khokhlova , V. V. Strelkov

In this Letter, it is experimentally and theoretically shown that weak odd harmonics generated during the propagation of an infrared ultrashort ultra-intense pulse unexpectedly modify the nonlinear properties of the medium and lead to a…

Optics · Physics 2015-06-18 P. Béjot , G. Karras , F. Billard , E. Hertz , B. Lavorel , E. Cormier , O. Faucher

High harmonic generation (HHG) is a manifestation of the strongly nonlinear response of matter to intense laser fields and has, as the basis for coherent XUV sources a variety of applications. Recently, HHG from atoms in a phase and…

Optics · Physics 2020-05-20 Jonas Wätzel , Jamal Berakdar

We show how bright, fully coherent, hard x-ray beams can be generated through nonlinear upconversion of femtosecond laser light. By using longer-wavelength mid-infrared driving lasers of moderate peak intensity, full phase matching of the…

We study theoretically the two-center interferences occurring in high harmonic generation from diatomic molecules. By solving the time-dependent Schroedinger equation, either numerically or with the molecular strong-field approximation, we…

Harmonic generation is a general characteristic of driven nonlinear systems, and serves as an efficient tool for investigating the fundamental principles that govern the ultrafast nonlinear dynamics. In atomic gases, high-harmonic radiation…

The emission of high-order harmonics from solids \cite{ghimire11a,schubert14a,luu15a,golde08a} under intense laser-pulse irradiation is revolutionizing our understanding of strong-field solid-light interactions…

We demonstrate the generation of a train of attosecond XUV pulses that are in a superposition of wavefront states. Such superposition yields a high precision, self-referencing, common path XUV interferometer setup to produce pairs of…

Circularly polarized extreme ultraviolet (XUV) radiation is highly interesting for investigation of chirality-sensitive light-matter interactions. Recent breakthroughs have enabled generation of such light sources via high harmonic…

Optics · Physics 2019-02-19 Zi-Yu Chen , Rui Qin

The production of brighter coherent XUV radiation by intense laser pulses through the process of high-harmonic generation (HHG) is a central challenge in contemporary nonlinear optics. We study the generation and spatial propagation of high…

Optics · Physics 2025-06-03 Margarita Khokhlova , Vasily Strelkov

Attosecond pulses created by high-order harmonic generation in gases often exhibit strong chromatic aberrations, arising from the broad bandwidth and wavelength-dependent nonlinear light-matter interaction. When the driving laser intensity…

Coherent sources of attosecond extreme ultraviolet (XUV) radiation present many challenges if their full potential is to be realized. While many applications benefit from the broadband nature of these sources, it is also desirable to…

We present a theoretical analysis of high-order harmonic generation from ion-atom collisions in the presence of linearly polarized intense laser pulses. Photons with frequencies significantly higher than in standard atomic high-harmonic…

Atomic Physics · Physics 2009-11-10 Manfred Lein , Jan M. Rost

High-order harmonic generation (HHG) in gases leads to short-pulse extreme ultraviolet (XUV) radiation useful in a number of applications, for example, attosecond science and nanoscale imaging. However, this process depends on many…