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Linearized Coupled Cluster Doubles (LinCCD) often provides near-singular energies in small-gap systems that exhibit static correlation. This has been attributed to the lack of quadratic $T_2^2$ terms that typically balance out small energy…

Chemical Physics · Physics 2025-05-13 Kevin Carter-Fenk

We present new results for LambdaCC and MotifCC, two recently introduced variants of the well-studied correlation clustering problem. Both variants are motivated by applications to network analysis and community detection, and have…

Computational Complexity · Computer Science 2018-09-26 David F. Gleich , Nate Veldt , Anthony Wirth

A new method that accurately describes strongly correlated states and captures dynamical correlation is presented. It is derived as a modification of coupled-cluster theory with single and double excitations (CCSD) through consideration of…

Chemical Physics · Physics 2013-07-15 Daniel Kats , Frederick R. Manby

Chromatic Correlation Clustering (CCC) generalizes Correlation Clustering by assigning multiple categorical relationships (colors) to edges and imposing chromatic constraints on the clusters. Unlike traditional Correlation Clustering, which…

Data Structures and Algorithms · Computer Science 2025-07-22 Dahoon Lee , Chenglin Fan , Euiwoong Lee

Correlation clustering is a widely studied framework for clustering based on pairwise similarity and dissimilarity scores, but its best approximation algorithms rely on impractical linear programming relaxations. We present faster…

Data Structures and Algorithms · Computer Science 2022-06-27 Nate Veldt

This paper presents Constrained Centroid Clustering (CCC), a method that extends classical centroid-based clustering by enforcing a constraint on the maximum distance between the cluster center and the farthest point in the cluster. Using a…

Machine Learning · Computer Science 2025-08-19 Sowmini Devi Veeramachaneni , Ramamurthy Garimella

Correlation Clustering (CC) is a foundational problem in unsupervised learning that models binary similarity relations using labeled graphs. While classical CC has been widely studied, many real-world applications involve more nuanced…

Data Structures and Algorithms · Computer Science 2025-09-23 Chenglin Fan , Dahoon Lee , Euiwoong Lee

While restricted single-reference coupled cluster theory truncated to singles and doubles (CCSD) provides very accurate results for weakly correlated systems, it usually fails in the presence of static or strong correlation. This failure is…

Chemical Physics · Physics 2016-02-25 Ireneusz W. Bulik , Thomas M. Henderson , Gustavo E. Scuseria

We propose a streamlined combination scheme of the transcorrelation (TC) and coupled cluster (CC) theory, which not only increases the convergence rate with respect to the basis set, but also extends the applicability of the lowest order CC…

Strongly Correlated Electrons · Physics 2021-07-28 Ke Liao , Thomas Schraivogel , Hongjun Luo , Daniel Kats , Ali Alavi

The most essential concept in concurrent multiscale methods involving atomistic-continuum coupling is how to define the relation between atomistic and continuum regions. A well-known coupling method that has been frequently employed in…

Mesoscale and Nanoscale Physics · Physics 2022-07-27 Pouya Towhidi , Manouchehr Salehi

We present LSD-C, a novel method to identify clusters in an unlabeled dataset. Our algorithm first establishes pairwise connections in the feature space between the samples of the minibatch based on a similarity metric. Then it regroups in…

Computer Vision and Pattern Recognition · Computer Science 2020-06-18 Sylvestre-Alvise Rebuffi , Sebastien Ehrhardt , Kai Han , Andrea Vedaldi , Andrew Zisserman

We discuss diagrammatic modifications to the coupled cluster doubles (CCD) equations, wherein different groups of terms out of rings, ladders, crossed-rings and mosaics can be removed to form approximations to the coupled cluster method, of…

Chemical Physics · Physics 2014-05-06 James J. Shepherd , Thomas. M. Henderson , Gustavo E. Scuseria

We develop randomized (block) coordinate descent (CD) methods for linearly constrained convex optimization. Unlike most CD methods, we do not assume the constraints to be separable, but let them be coupled linearly. To our knowledge, ours…

Optimization and Control · Mathematics 2015-06-11 Sashank Reddi , Ahmed Hefny , Carlton Downey , Avinava Dubey , Suvrit Sra

We propose a multireference linearized coupled cluster theory using matrix product states (MPS-LCC) which provides remarkably accurate ground-state energies, at a computational cost that has the same scaling as multireference configuration…

Chemical Physics · Physics 2015-09-02 Sandeep Sharma , Ali Alavi

Most dimensionality reduction methods employ frequency domain representations obtained from matrix diagonalization and may not be efficient for large datasets with relatively high intrinsic dimensions. To address this challenge, Correlated…

Machine Learning · Statistics 2022-06-10 Yuta Hozumi , Rui Wang , Guo-Wei Wei

In Coupled-Cluster (CC) theory, unphysical complex energies may arise in the presence of strong magnetic fields, near conical intersections, or in systems exhibiting complex Abelian point group symmetries. This issue originates from the…

Chemical Physics · Physics 2025-07-28 Laura Grazioli , Marios-Petros Kitsaras , Stella Stopkowicz

Block coordinate descent (BCD) methods approach optimization problems by performing gradient steps along alternating subgroups of coordinates. This is in contrast to full gradient descent, where a gradient step updates all coordinates…

Numerical Analysis · Mathematics 2019-07-29 Simon Rabanser , Lukas Neumann , Markus Haltmeier

We propose to improve the convergence properties of the single-reference coupled cluster (CC) method through an augmented Lagrangian formalism. The conventional CC method changes a linear high-dimensional eigenvalue problem with exponential…

Computational Physics · Physics 2024-03-26 Fabian M. Faulstich , Yuehaw Khoo , Kangbo Li

Coupled cluster theory is a vital cornerstone of electronic structure theory and is being applied to ever-larger systems. Stochastic approaches to quantum chemistry have grown in importance and offer compelling advantages over traditional…

We present a novel enhanced cyclic coordinate descent (ECCD) framework for solving generalized linear models with elastic net constraints that reduces training time in comparison to existing state-of-the-art methods. We redesign the CD…

Machine Learning · Statistics 2025-10-24 Yixiao Wang , Zishan Shao , Ting Jiang , Aditya Devarakonda
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