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We investigated the temperature dependence of the superlattice intensity and thermal diffuse scattering intensity of BaAl2O4, which has a network structure with corner-sharing AlO4 tetrahedra, via synchrotron X-ray diffraction experiments.…

Materials Science · Physics 2016-04-27 Y. Ishii , S. Mori , Y. Nakahira , C. Moriyoshi , H. Taniguchi , H. Moriwake , Y. Kuroiwa

Synchrotron X-ray diffraction (XRD) experiments were performed on the network compounds Ba1-xSrxAl2O4 at temperatures between 15 and 800 K. The ferroelectric phase of the parent BaAl2O4 is largely suppressed by the Sr-substitution and…

Materials Science · Physics 2016-09-07 S. Kawaguchi , Y. Ishii , E. Tanaka , H. Tsukasaki , Y. Kubota , S. Mori

We have studied structural phase transitions in high quality underdoped La$_{2-x}$Ba$_x$CuO$_4$ single crystals using high resolution x-ray scattering techniques. Critical properties associated with the continuous High Temperature…

Superconductivity · Physics 2009-11-13 Y. Zhao , B. D. Gaulin , J. P. Castellan , J. P. C. Ruff , S. R. Dunsiger , G. D. Gu , H. A. Dabkowska

The A-site spinel material, CoAl2O4, is a physical realization of the frustrated diamond-lattice antiferromagnet, a model in which is predicted to contain unique incommensurate or `spin-spiral liquid' ground states. Our previous…

The ferrimagnetic spinel $\mathrm{CoV_2O_4}$ has been a topic of intense recent interest, both as a frustrated insulator with unquenched orbital degeneracy and as a near-itinerant magnet which can be driven metallic with moderate applied…

Strongly Correlated Electrons · Physics 2016-02-03 D. Reig-i-Plessis , D. Casavant , V. O. Garlea , A. A. Aczel , M. Feygenson , J. Neuefeind , H. D. Zhou , S. E. Nagler , G. J. MacDougall

Soft phonon behavior associated with a structural phase transition from the low-temperature-orthorhombic (LTO) phase ($Bmab$ symmetry) to the low-temperature-tetragonal (LTT) phase ($P4_{2}/ncm$ symmetry) was investigated in…

Superconductivity · Physics 2009-11-10 H. Kimura , Y. Noda , H. Goka , M. Fujita , K. Yamada , G. Shirane

The surface structural phases of Ca(2-x)Sr(x)RuO(4) are investigated using quantitative Low Energy Electron Diffraction. The broken symmetry at the surface enhances the structural instability against the RuO6 rotational distortion while…

Strongly Correlated Electrons · Physics 2009-11-13 R. G. Moore , V. B. Nascimento , Jiandi Zhang , J. Rundgren , R. Jin , D. Mandrus , E. W. Plummer

We have observed a softening of phonons and a structural phase transition in a superconducting Ba0.59K0.41BiO3 (Tc = 31 K) single crystal using elastic and inelastic neutron scattering measurements. The soft phonon occurs for the [111]…

Superconductivity · Physics 2011-07-27 H. J. Kang , Y. S. Lee , J. W. Lynn , S. V. Shiryaev , S. N. Barilo

Historically, the soft mode theory of ferroelectric phase transitions has been developed for the high-temperature (paraelectric) phase, where the phonon mode softens upon decreasing the temperature. In the low-temperature ferroelectric…

Materials Science · Physics 2021-03-19 Luigi Casella , Alessio Zaccone

In this work we present the results of an inelastic x-ray scattering experiment detailing the behavior of the transverse acoustic [110] phonon in BaFe2As2 as a function of temperature. When cooling through the structural transition…

Superconductivity · Physics 2012-01-04 Jennifer L. Niedziela , D. Parshall , K. A. Lokshin , A. S. Sefat , A. Alatas , T. Egami

Relaxor ferroelectrics are difficult to study and understand. The experiment shows that at low energy scattering there is an acoustic mode, an optic mode, dynamic quasi-elastic scattering and strictly elastic scattering as well as Bragg…

Materials Science · Physics 2008-08-29 R. A. Cowley , S. N. Gvasaliya , B. Roessli

Inelastic neutron scattering is used to measure the temperature dependent phonon dispersion in Ca$_{2-x}$Sr$_{x}$RuO$_{4}$ ($x=0.4$, 0.6). The in-plane $\Sigma_{4}$ octahedral tilt mode softens significantly at the zone boundary of the high…

Strongly Correlated Electrons · Physics 2015-05-13 R. G. Moore , M. D. Lumsden , M. B. Stone , Jiandi Zhang , Y. Chen , J. W. Lynn , R. Jin , D. Mandrus , E. W. Plummer

The semiconductor-insulator phase transition of the single-layer manganite La0.5Sr1.5MnO4 has been studied by means of high resolution synchrotron x-ray powder diffraction and resonant x-ray scattering at the Mn K edge. We conclude that a…

Strongly Correlated Electrons · Physics 2015-05-27 J. Herrero-Martin , J. Blasco , J. Garcia , G. Subias , C. Mazzoli

We examine the low-energy excitations in the vicinity of the quantum critical point in LiHoF$_4$, a physical realization of the Transverse Field Ising Model, focusing on the long-range fluctuations which soften to zero energy at the…

Strongly Correlated Electrons · Physics 2024-10-25 P. C. E. Stamp , D. M. Silevitch , M. Libersky , Ryan McKenzie , A. A. Geim , T. F. Rosenbaum

We have studied the high-frequency dynamics of salol by inelastic x-ray scattering over a wide temperature range between 50 and 450 K, across the glass transition. We find that salol efficiently realizes the mechanism of dynamical arrest…

Soft Condensed Matter · Physics 2019-12-05 L. Comez , D. Fioretto , J. Gapinski , G. Monaco , A. Patkowski , W. Steffen

We report the results of Raman spectroscopy high-pressure studies of alkali metal fluoroargentates (M2AgF4, where M=Na, K, Rb) associated with theoretical and x-ray diffraction studies for the K member of the series. Theoretical density…

Using resonant soft X-ray techniques we follow the magnetic behavior of a strained epitaxial film of CoCr2O4, a type-II multiferroic. The film is [110]-oriented, such that both the ferroelectric and ferromagnetic moments can coexist in…

In a previous work a model was proposed for the phase transitions of crystals with localized magnetic moments which at low temperature have a "conical" arrangement that at higher T transforms into a more symmetrical structure (depending on…

Statistical Mechanics · Physics 2009-11-13 Vittorio Massidda

Barium zirconate BaZrO3 is one of few perovskites that is claimed to retain an average cubic structure down to 0K at ambient pressure, while being energetically very close to a tetragonal phase obtained by condensation of a soft phonon mode…

Materials Science · Physics 2024-03-22 Erik Fransson , Petter Rosander , Paul Erhart , Göran Wahnström

In this paper, we present a thorough investigation of vibrational, structural, and electronic properties of perovskite-type rhombohedral Ba$_2$ZnTeO$_6$ (BZTO) under systematic application of pressure. To carry out the analysis, we have…

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