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Using grand canonical Monte Carlo simulations, we investigate the percolation behavior of a square well fluid with an ultra-short range of attraction in three dimension (3D) and in confined geometry. The latter is defined through two…

Soft Condensed Matter · Physics 2012-11-07 Helge Neitsch , Sabine H. L. Klapp

Using molecular dynamics calculations and the Voronoi tessellation, we study the evolution of the local structure of a soft-sphere glass versus temperature starting from the liquid phase at different quenching rates. This study is done for…

Disordered Systems and Neural Networks · Physics 2009-10-31 Philippe Jund , Remi Jullien

Quantum confinement increases the spacing between energy levels as the nanocrystallite size is decreased. Its qualitative features hold both for states localized near the center of a nanocrystallite and those near the surface, such as…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 K. E. Andersen , C. Y. Fong , W. E. Pickett

Using grand canonical Monte Carlo simulations, we have explored the phenomenon of capillary condensation (CC) of Ar at the triple temperature inside infinitely long, cylindrical pores. Pores of radius R= 1 nm, 1.7 nm and 2.5 nm have been…

Materials Science · Physics 2009-11-11 Silvina M. Gatica , Milton W. Cole

The freezing of colloidal suspensions is encountered in many natural and engineering processes such as the freezing of soils, food engineering, and cryobiology. It can also be used as a bio-inspired, versatile, and environmentally-friendly…

Applied Physics · Physics 2018-05-16 Sylvain Deville , Jérôme Adrien , Eric Maire , Mario Scheel , Marco Di Michiel

Most ice in nature forms thanks to impurities which boost the exceedingly low nucleation rate of pure supercooled water. However, the microscopic details of ice nucleation on these substances remain largely unknown. Here, we have unraveled…

Materials Science · Physics 2016-11-23 Gabriele C. Sosso , Tianshu Li , Davide Donadio , Gareth A. Tribello , Angelos Michaelides

Amorphous solids, confined on the nano-scale, exhibit a wealth of novel phenomena yet to be explored. In particular, the response of such solids to a mechanical load is not well understood and, as has been demonstrated experimentally, it…

Statistical Mechanics · Physics 2019-07-10 Kallol Paul , Ratul Dasgupta , Jürgen Horbach , Smarajit Karmakar

We implement molecular dynamics simulations in canonical ensemble to study the effect of confinement on a $2d$ crystal of point particles interacting with an inverse power law potential proportional to $r^{-12}$ in a narrow channel. This…

Soft Condensed Matter · Physics 2014-09-30 M. Ebrahim Foulaadvand , Neda Ojaghlou

We combine experiments and simulations to study the link between criticality and gelation in sticky spheres. We employ confocal microscopy to image colloid-polymer mixtures, and Monte Carlo simulations of the square-well (SW) potential as a…

Soft Condensed Matter · Physics 2018-08-17 David Richard , James Hallett , Thomas Speck , C. Patrick Royall

Designing and fabricating self-assembled open colloidal crystals have become one major direction in soft matter community because of many promising applications associated with open colloidal crystals. However, most of the self-assembled…

Soft Condensed Matter · Physics 2019-04-16 Krongtum Sankaewtong , Qun-li Lei , Ran Ni

It is now possible to create perfect crystal nanowires of many metals. The deformation of such objects requires a good understanding of the processes involved in plasticity at the nanoscale. Isotropic compression of such nanometre scale…

Materials Science · Physics 2019-06-05 Con J. Healy , Graeme J. Ackland

Acoustic levitation is a container-free method for examining novel crystallization effects, though liquid-to-solid phase change has seen little investigation for levitated nanofluids. Recent developments have allowed for examining the…

Applied Physics · Physics 2024-09-13 Adam McElligott , André Guerra , Alejandro D. Rey , Phillip Servio

Contact freezing is a mode of atmospheric ice nucleation in which a collision between a dry ice nucleating particle (INP) and a water droplet results in considerably faster heterogeneous nucleation. The molecular mechanism of such…

Soft Condensed Matter · Physics 2021-01-29 Sarwar Hussain , Amir Haji-Akbari

In this article, we present direct numerical simulation results for the expansion of spherical cap bubbles attached to a rigid wall due to a sudden drop in the ambient pressure. The critical pressure drop beyond which the bubble growth…

Fluid Dynamics · Physics 2024-05-28 Mandeep Saini , Xiang Bin Chen , Stephane Zaleski , Daniel Fuster

We study a strongly interacting dense hard-sphere system confined between two parallel plates by event-driven molecular dynamics simulations to address the fundamental question of the nature of the 3D to 2D crossover. As the fluid becomes…

Soft Condensed Matter · Physics 2017-02-09 Suvendu Mandal , Thomas Franosch

Segregation at surfaces of metal-covalent binary liquids is often non-classical and in extreme cases such as AuSi, the surface crystallizes above the melting point. In this study, we employ atomic-scale computational frameworks to study the…

Materials Science · Physics 2021-07-21 Hailong Wang , Alireza Shahabi , Alain Karma , Moneesh Upmanyu

Quasi-two-dimensional (quasi-2D) colloidal hard-sphere suspensions confined in a slit geometry are widely used as two dimensional (2D) model systems in experiments that probe the glassy relaxation dynamics of 2D systems. However, the…

Soft Condensed Matter · Physics 2023-02-15 Jiting Tian , Walter Kob , Jean-Louis Barrat

The confinement of an ionic liquid between charged solid surfaces is treated using an exactly solvable 1D Coulomb gas model. The theory highlights the importance of two dimensionless parameters: the fugacity of the ionic liquid, and the…

Soft Condensed Matter · Physics 2014-09-08 Alpha A Lee , Dominic Vella , Susan Perkin , Alain Goriely

Steady progress in the miniaturization of structures and devices has reached a scale where thermal fluctuations become relevant and it is thus important to understand how such fluctuations affect their mechanical stability. Here, we…

Soft Condensed Matter · Physics 2021-02-24 Ali Morshedifard , Miguel Ruiz-Garcia , Mohammad Javad Abdolhosseini Qomi , Andrej Kosmrlj

Recent experiments on ice formed by water under nanoconfinement provide evidence for a two-dimensional (2D) `square ice' phase. However, the interpretation of the experiments has been questioned and the stability of square ice has become a…

Chemical Physics · Physics 2016-12-07 Ji Chen , Andrea Zen , Jan Gerit Brandenburg , Dario Alfè , Angelos Michaelides