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We developed methods for protein synthesis and performed two-dimensional electronic spectroscopy (2D-ES) to examine the influence of pigment arrangement on the photoexcitation dynamics of light-harvesting proteins in phycobilisome. We…

Biological Physics · Physics 2026-01-29 Masaaki Tsubouchi , Takatoshi Fujita , Motoyasu Adachi , Ryuji Itakura

Metal-dielectric interfaces of various geometries are fundamental photonic material platforms for surface plasmons. Surface plasmon polaritons and localized surface plasmons are two surface plasmon modes that are excited on planar and…

We studied the mechanism of half-metallicity (HM) formation in transition metal doped (TM) conjugated carbon based structures by first-principles electronic structure simulations. It is found that the HM is a rather complex phenomenon,…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 Lida Pan , Boqun Song , Jiatao Sun , Lizhi Zhang , Werner Hofer , Shixuan Du , Hong-jun Gao

We investigate the adsorption of a single tetracyanoethylene (TCNE) molecule on the silver (001) surface. Adsorption structures, electronic properties, and scanning tunneling microscopy (STM) images are calculated within density-functional…

Mesoscale and Nanoscale Physics · Physics 2016-06-22 Thorsten Deilmann , Peter Krüger , Michael Rohlfing , Daniel Wegner

We study a highly controllable perfect plasmonic absorber -- a thin metamaterial layer which possess balanced electric and magnetic responses in some frequency range. We show that this regime is compatible with both metal-backed variant of…

Optics · Physics 2016-01-25 Mikhail Omelyanovich , Younes Ra'di , Constantin Simovski

Plasmonic structures are known to support the modes with subwavelength volumes in which the field matter interactions are greatly enhanced. Coupling between the molecular excitations and plasmons leading to formation of plexcitons has been…

Optics · Physics 2018-11-27 Jacob B Khurgin

Linear and nonlinear optical lineshapes reveal details of excitonic structure in semiconductor polymers. We implement absorption, photoluminescence, and transient absorption spectroscopies in DPP-DTT, an electron push-pull copolymer, to…

Single-layer transition metal dichalcogenides (TMDCs) can adopt two distinct structures corresponding to different coordination of the metal atoms. TMDCs adopting the T-type structure exhibit a rich and diverse set of phenomena, including…

Mesoscale and Nanoscale Physics · Physics 2020-07-29 Daniel T. Larson , Wei Chen , Steven B. Torrisi , Jennifer Coulter , Shiang Fang , Efthimios Kaxiras

The design of low-dimensional organic-inorganic interfaces for the next generation of opto-electronic applications requires an in-depth understanding of the microscopic mechanisms ruling electronic interactions in these systems. In this…

Photonic bound states in the continuum (BICs) are a standout nanophotonic platform for strong light-matter coupling with transition metal dichalcogenides (TMDCs), but have so far mostly been employed as all-dielectric metasurfaces with…

Shape-controlled synthesis of multiply twinned nanostructures is heavily emphasized in nanoscience, in large part due to the desire to control the size, shape, and terminating facets of metal nanoparticles for applications in catalysis.…

Magneto-plasmonic nanostructures have emerged as promising candidates for advanced sensing applications. However, conventional fabrication methods, such as lithography and sputtering, often involve high costs and complex processes. This…

Recent advances in the experimental growth and control of disordered thin films, heterostructures, and interfaces provide a fertile ground for the observation and characterisation of the collective superconducting excitations emerging below…

Deciphering the three-dimensional atomic structure of solid-solid interfaces in core-shell nanomaterials is the key to understand their remarkable catalytical, optical and electronic properties. Here, we probe the three-dimensional atomic…

Materials Science · Physics 2023-06-21 Zezhou Li , Zhiheng Xie , Yao Zhang , Xilong Mu , Hai-jing Yin , Ya-wen Zhang , Colin Ophus , Jihan Zhou

The migration of grain boundaries leads to grain growth in polycrystals and is one mechanism of grain-boundary-mediated plasticity, especially in nanocrystalline metals. This migration is due to the movement of dislocation-like defects,…

Materials Science · Physics 2024-05-09 Swetha Pemma , Rebecca Janisch , Gerhard Dehm , Tobias Brink

The migration of grain boundaries leads to grain growth in polycrystals and is one mechanism of grain-boundary-mediated plasticity, especially in nanocrystalline metals. This migration is due to the movement of dislocation-like defects,…

Materials Science · Physics 2024-07-08 Swetha Pemma , Rebecca Janisch , Gerhard Dehm , Tobias Brink

Molten iron chlorides are central to emerging energy technologies, including electrochemical iron production and redox flow batteries. Optimizing their electrochemical performance and transport properties requires atomic-scale structural…

Helical structures are exciting and are utilized in numerous applications ranging from biotechnology to displays to medicine. Accurate description and understanding of resonance effects in helical structures provides crucial knowledge on…

Soft Condensed Matter · Physics 2020-02-04 Yu Cao , Jun Feng , Asritha Nallapaneni , Yuki Arakawa , Keqing Zhao , Georg H. Mehl , Feng Liu , Chenhui Zhu

Self-assembled, semimetallic ErSb single crystal nanostructures, grown by molecular beam epitaxy, are embedded within a semiconductor GaSb matrix. Formation, evolution and orientation of a variety of nanostructures, including spherical…

Hybrid systems of excitons strongly coupled to localized surface plasmons supported by metallic nanoparticles define a new approach to control light-matter interactions. Here, we report exciton-plasmon coupling in two-dimensional (2D)…