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We carried out a joint theoretical and experimental study of the polarization of high-order harmonics generated from ZnO by intense infrared laser pulses. Experimentally we found that the dependence of parallel and perpendicular…

High-harmonic generation (HHG) provides short-wavelength light that is useful for precision spectroscopy and probing ultrafast dynamics. We report efficient, phase-coherent harmonic generation up to 9th-order (333 nm) in chirped…

Numerous optical phenomena and applications have been enabled by nanophotonic structures. Their current fabrication from high refractive index dielectrics, such as silicon or gallium phosphide, pose restricting fabrication challenges, while…

The emission of high-order harmonics from solids \cite{ghimire11a,schubert14a,luu15a,golde08a} under intense laser-pulse irradiation is revolutionizing our understanding of strong-field solid-light interactions…

Complex oxide heterointerfaces and van der Waals heterostructures present two versatile but intrinsically different platforms for exploring emergent quantum phenomena and designing new functionalities. The rich opportunity offered by the…

Mesoscale and Nanoscale Physics · Physics 2020-03-19 Dawei Li , Xi Huang , Zhiyong Xiao , Hanying Chen , Le Zhang , Yifei Hao , Jingfeng Song , Ding-Fu Shao , Evgeny Y. Tsymbal , Yongfeng Lu , Xia Hong

High harmonic generation (HHG) opens a window on the fundamental science of strong-field light-mater interaction and serves as a key building block for attosecond optics and metrology. Resonantly enhanced HHG from hot spots in…

Second-harmonic generation (SHG) is a direct measure of the strength of second-order nonlinear optical effects, which also include frequency mixing and parametric oscillations. Natural and artificial materials with broken…

Accelerating and colliding particles has been a key strategy to explore the texture of matter. Strong lightwaves can control and recollide electronic wavepackets, generating high-harmonic (HH) radiation which encodes the structure and…

Mesoscale and Nanoscale Physics · Physics 2016-04-14 M. Hohenleutner , F. Langer , O. Schubert , M. Knorr , U. Huttner , S. W. Koch , M. Kira , R. Huber

We theoretically study high-order harmonic generation (HHG) from solid-phase systems in spatially inhomogeneous strong laser fields originated by resonant plasmons within a metallic nanostructure. The intensity of the second plateau in HHG…

Optics · Physics 2016-09-12 Tao-Yuan Du , Zhong Guan , Xiao-Xin Zhou , Xue-Bin Bian

Thermotropic liquid crystals are versatile optical materials that exhibit a state of matter intermediate between liquids and solids. Their properties can change significantly with temperature, pressure, or other external factors, leading to…

In this work, the nonlinear optical response, and in particular, the high harmonic generation of semiconductors is addressed by using the Wannier gauge. One of the main problems in the time evolution of the Semiconductor Bloch equations…

Mesoscale and Nanoscale Physics · Physics 2019-11-20 R. E. F. Silva , F. Martín , M. Ivanov

We present theoretical investigations of high-order harmonic generation (HHG) resulting from the interaction of noble gases with localized surface plasmons. These plasmonic fields are produced when a metal nanoparticle is subject to a…

The discovery of atomically thin van der Waals ferroelectric and magnetic materials encourages the exploration of 2D multiferroics, which holds the promise to understand fascinating magnetoelectric interactions and fabricate advanced…

Materials Science · Physics 2023-07-21 Shuang Wu , Xinyu Chen , Canyu Hong , Xiaofei Hou , Zhanshan Wang , Zhiyuan Sheng , Zeyuan Sun , Yanfeng Guo , Shiwei Wu

High-order harmonic generation (HHG) is a fundamental process which can be simplified as the production of high energetic photons from a material subjected to a strong driving laser field. This highly nonlinear optical process contains rich…

Optics · Physics 2021-12-21 Dasol Kim , Yeon Lee , Alexis Chacón , Dong Eon Kim

In our recent study [Commun. Phys. 3, 92 (2020)], we have developed an approach for energy-scaling of high-order harmonic generation in water-window region under neutral-medium condition. More specifically, we obtained nanojoule-class…

In this paper, the nonlinear interaction of Weyl semimetal (WSM) with a strong driving electromagnetic wave-field is investigated. In the scope of the structure-gauge invariant low-energy nonlinear electrodynamic theory, the…

Mesoscale and Nanoscale Physics · Physics 2022-06-22 H. K. Avetissian , V. N. Avetisyan , B. R. Avchyan , G. F. Mkrtchian

Van der Waals (vdW) ferroelectrics are emerging nonlinear photonic materials that combine large second-order susceptibility \c{hi}(2) with heterostructure compatibility, offering an attractive route toward miniaturized spontaneous…

Since the new millennium coherent extreme ultra-violet and soft x-ray radiation has revolutionized the understanding of dynamical physical, chemical and biological systems at the electron's natural timescale. Unfortunately, coherent…

Second harmonic generation in a two dimensional nonlinear quasi-crystal is demonstrated for the first time. Temperature and wavelength tuning of the crystal reveal the uniformity of the pattern while angle tuning reveals the dense nature of…

Optics · Physics 2007-05-23 Neil Broderick , Anna Peacock , Katia Gallo , Ruth Lewen , Radu Bratfalean

High-order harmonic generation (HHG) from crystals offers a new source of coherent extreme ultraviolet (XUV) attosecond radiation.