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We investigate the effect of charge self-consistency (CSC) in density functional theory plus dynamical mean-field theory (DFT+DMFT) calculations compared to simpler "one-shot" calculations for materials where interaction effects lead to a…

Strongly Correlated Electrons · Physics 2020-07-22 Alexander Hampel , Sophie Beck , Claude Ederer

We study the optical properties of small gold chains doped with different transition metal (TM) atoms (Ni,Rh,Fe) by using the time-dependent density-functional theory (TDDFT) approach. The optical absorption spectrum of such systems…

Mesoscale and Nanoscale Physics · Physics 2011-09-06 N. Nayyar , A. Kabir , V. Turkowski , Talat S. Rahman

The two-dimensional transition metal dichalcogenides (TMDs) have been proposed as candidates for the channel material in future field effect transistor designs. The heterophase design which utilizes the metallic T- or T' phase of the TMD as…

Mesoscale and Nanoscale Physics · Physics 2021-08-04 Line Jelver , Ole Hansen , Karsten Wedel Jacobsen

Using interlayer interaction to control functional heterostructures with atomic-scale designs has become one of the most effective interface-engineering strategies nowadays. Here, we demonstrate the effect of a crystalline LaFeO3 buffer…

We study the charge induced in a Thomas-Fermi metal by an ion in vacuum, using an atomistic description employed in constant-potential molecular dynamics simulations, and compare the results with the predictions from continuum…

Computational Physics · Physics 2024-03-08 Swetha Nair , Giovanni Pireddu , Benjamin Rotenberg

We study the relation between nitrogen and oxygen abundances as a function of metallicity for a sample of emission-line objects for which a direct measurement of the metallicity has been possible. This sample is representative of the very…

Cosmology and Nongalactic Astrophysics · Physics 2015-05-13 Enrique Perez-Montero , Thierry Contini

Interfaces between transition-metal oxides are able to host two-dimensional electron gases (2DEGs) and exhibit exotic quantum phenomena. Here we report the observation of superconductivity below 230 mK for the heterostructure composed of…

Superconductivity · Physics 2022-12-27 Haoran Wei , Shengru Chen , Yuting Zou , Yuxin Wang , Meng Yang , Qinghua Zhang , Lin Gu , Kun Jiang , Er-Jia Guo , Zhi Gang Cheng

Interfacial thermal transport is a critical bottleneck in nanoscale systems, where heat dissipation and energy efficiency are strongly modulated by molecular ordering at solid-liquid boundaries. Here, using atomistic simulations of…

Mesoscale and Nanoscale Physics · Physics 2026-01-14 Viktor Mandrolko , Mykola Isaiev

We determined the interface state density ($D_{\rm it}$) distributions in the vicinity of the conduction band edge in silicon carbide (SiC) metal-oxide-semiconductor (MOS) structures by reproducing the experimental current-voltage…

Materials Science · Physics 2020-09-07 Koji Ito , Takuma Kobayashi , Tsunenobu Kimoto

Metal-insulator transitions (MITs) in correlated oxides offer immense potential for next-generation Mottronic devices. However, their integration into practical applications is often hindered by the coupling of MITs with symmetry-lowering…

Here, we report orbital-free density-functional theory (OF DFT) molecular dynamics simulations of the displacement cascade in aluminum. The electronic effect is our main concern. The displacement threshold energies are calculated using OF…

Materials Science · Physics 2017-09-26 Ruizhi Qiu

We investigate the interplay between electronic screening inside a metal and screening by a polar molecular solvent, focusing on their impact on the charge induced by an ion and the solvent structure at the interface. To that end, we…

Chemical Physics · Physics 2025-03-17 Swetha Nair , Guillaume Jeanmairet , Benjamin Rotenberg

Charge transfer induced interfacial ferromagnetism and its impact on the exchange bias effect in La$_{0.7}$Sr$_{0.3}$MnO$_3$/NdNiO$_3$ correlated oxide heterostructures were investigated by soft x-ray absorption and x-ray magnetic circular…

Materials Science · Physics 2020-04-29 K. Chen , C. Luo , B. B. Chen , R. M. Abrudan , G. Koster , S. K. Mishra , F. Radu

It has been proposed that an extended version of the Hubbard model which potentially hosts rich correlated physics may be well simulated by the transition metal dichalcogenide (TMD) moir\'{e} heterostructures. Motivated by recent reports of…

Strongly Correlated Electrons · Physics 2022-06-30 Yichen Xu , Xiao-Chuan Wu , Mengxing Ye , Zhu-Xi Luo , Chao-Ming Jian , Cenke Xu

Molecular-scale manipulation of electronic/ionic charge accumulation in materials is a preeminent challenge, particularly in electrochemical energy storage. Layered van der Waals (vdW) crystals exemplify a diverse family of materials that…

The electronic structure of ZnPc, from sub-monolayers to thick films, on bare and iodated Pt(111) is studied by means of X-ray photoelectron spectroscopy (XPS), X-ray absorption spectroscopy (XAS) and scanning tunneling microscopy (STM).…

Materials Science · Physics 2014-05-01 S. Ahmadi , B. Agnarsson , I. Bidermane , B. M. Wojek , Q. Noël , C. H. Sun , M. Göthelid

Two-dimensional (2D) metallic states induced by oxygen vacancies at oxide surfaces and interfaces provide new opportunities for the development of advanced applications, but the ability to control the behavior of these states is still…

Nanoscale investigations by scanning probe microscopy have provided major contributions to the rapid development of organic-inorganic halide perovskites (OIHP) as optoelectronic devices. Further improvement of device level properties…

Charge disproportionation transitions in complex oxides most commonly link high-temperature phases containing identical cations with the same oxidation state and crystallographic site, to low-temperature phases in which charge transfer…

Materials Science · Physics 2019-01-09 Ulrich Aschauer , Nathalie Vonrüti , Nicola A. Spaldin

Density functional theory $(DFT)$ studies show that doping of $3d TM$ atoms into $Mg_4^{0,+} (TMMg_3^{0,+})$ can alter the endothermic nature of molecular hydrogen adsorption on bare $Mg_4^{0,+}$. $H_2$ adsorption on $TMMg_3^{0,+}$ clusters…

Materials Science · Physics 2021-12-21 Bishwajit Boruah , Bulumoni Kalita