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Few-shot learning is a promising approach to molecular property prediction as supervised data is often very limited. However, many important molecular properties depend on complex molecular characteristics -- such as the various 3D…

Machine Learning · Computer Science 2023-10-10 Christopher Fifty , Joseph M. Paggi , Ehsan Amid , Jure Leskovec , Ron Dror

We introduce machine learning models of quantum mechanical observables of atoms in molecules. Instant out-of-sample predictions for proton and carbon nuclear chemical shifts, atomic core level excitations, and forces on atoms reach…

Chemical Physics · Physics 2015-08-26 Matthias Rupp , Raghunathan Ramakrishnan , O. Anatole von Lilienfeld

Two-dimensional noncollinear magnetic states, such as spin-spiral magnets, offer an excellent platform for investigating fundamental phenomena, with potential for advancing stray-field-free spintronics. However, detection and…

Mesoscale and Nanoscale Physics · Physics 2026-04-06 Fedor Nigmatulin , Greta Lupi , Jose L. Lado , Zhipei Sun

Reconstructing a system Hamiltonian through measurements on its eigenstates is an important inverse problem in quantum physics. Recently, it was shown that generic many-body local Hamiltonians can be recovered by local measurements without…

Quantum Physics · Physics 2022-02-14 Chenfeng Cao , Shi-Yao Hou , Ningping Cao , Bei Zeng

Schr\"odinger's equation serves as a fundamental component in characterizing quantum systems, wherein both quantum state tomography and Hamiltonian learning are instrumental in comprehending and interpreting quantum systems. While numerous…

Quantum Physics · Physics 2024-01-25 Zheng An , Jiahui Wu , Muchun Yang , D. L. Zhou , Bei Zeng

The study explores machine learning methods for revealing chemical sensitivity in Helium spin-echo spectroscopy, in order to obtain ultra-sensitive surface analytic technique. We model bi-species co-adsorbed systems and demonstrate that by…

Chemical Physics · Physics 2020-12-04 Reinis Irmejs , Nadav Avidor

Atomistic structures of materials offer valuable insights into their functionality. Determining these structures remains a fundamental challenge in materials science, especially for systems with defects. While both experimental and…

Materials Science · Physics 2025-01-16 Haili Jia , Yiming Chen , Gi-Hyeok Lee , Jacob Smith , Miaofang Chi , Wanli Yang , Maria K. Y. Chan

The nature of the atomic defects on the hydrogen passivated Si (100) surface is analyzed using deep learning and scanning tunneling microscopy (STM). A robust deep learning framework capable of identifying atomic species, defects, in the…

Materials Science · Physics 2020-02-19 Maxim Ziatdinov , Udi Fuchs , James H. G. Owen , John N. Randall , Sergei V. Kalinin

In this article we present a machine learning model to obtain fast and accurate estimates of the molecular Hessian matrix. In this model, based on a random forest, the second derivatives of the energy with respect to redundant internal…

Chemical Physics · Physics 2024-01-10 Giorgio Domenichini , Christoph Dellago

We present a machine-learning method for predicting sharp transitions in a Hamiltonian phase diagram by extrapolating the properties of quantum systems. The method is based on Gaussian Process regression with a combination of kernels chosen…

Other Condensed Matter · Physics 2019-04-26 Rodrigo A. Vargas-Hernández , John Sous , Mona Berciu , Roman V. Krems

The observation and description of collective excitations in solids is a fundamental issue when seeking to understand the physics of a many-body system. Analysis of these excitations is usually carried out by measuring the dynamical…

Interacting spin networks are fundamental to quantum computing. Data-based tomography of time-independent spin networks has been achieved, but an open challenge is to ascertain the structures of time-dependent spin networks using time…

Quantum Physics · Physics 2021-12-15 Chen-Di Han , Bryan Glaz , Mulugeta Haile , Ying-Cheng Lai

We study the problem of Hamiltonian structure learning from real-time evolution: given the ability to apply $e^{-\mathrm{i} Ht}$ for an unknown local Hamiltonian $H = \sum_{a = 1}^m \lambda_a E_a$ on $n$ qubits, the goal is to recover $H$.…

Quantum Physics · Physics 2026-05-11 Ainesh Bakshi , Allen Liu , Ankur Moitra , Ewin Tang

Machine learning has emerged as an invaluable tool in many research areas. In the present work, we harness this power to predict highly accurate molecular infrared spectra with unprecedented computational efficiency. To account for…

Chemical Physics · Physics 2021-03-16 Michael Gastegger , Jörg Behler , Philipp Marquetand

The study of topological bandstructures is an active area of research in condensed matter physics and beyond. Here, we combine recent progress in this field with developments in machine-learning, another rising topic of interest.…

Mesoscale and Nanoscale Physics · Physics 2020-06-03 Mathias S. Scheurer , Robert-Jan Slager

Machine-Learned Interatomic Potentials (MLIPs) require vast amounts of atomic structure data to learn forces and energies, and their performance continues to improve with training set size. Meanwhile, the even greater quantities of…

Chemical Physics · Physics 2025-12-09 Manasa Kaniselvan , Benjamin Kurt Miller , Meng Gao , Juno Nam , Daniel S. Levine

Single crystal inelastic neutron scattering data contain rich information about the structure and dynamics of a material. Yet the challenge of matching sophisticated theoretical models with large data volumes is compounded by computational…

Learning quantum Hamiltonians with high precision is important for quantum physics and quantum information science. We propose a multi-stage neural network framework that significantly enhances Hamiltonian learning precision through…

Quantum Physics · Physics 2025-03-11 Zhengjie Kang , Hao Li , Shuo Wang , Jiaojiao Li , Yuanjie Zhang , Zhihuang Luo

We develop a structured theoretical framework used in our recent articles [Eur. Phys. J. B 92, 93 (2019) and Phys. Rev. B 101, 094427 (2020)] to characterize the unusual behavior of the magnetic spectrum, magnetization and magnetic…

Strongly Correlated Electrons · Physics 2022-05-19 M. Georgiev , H. Chamati

Spectroscopic measurements with low-temperature scanning tunneling microscopes have been used very successfully for studying not only individual atomic or molecular spins on surfaces but also complexly designed coupled systems. The symmetry…

Mesoscale and Nanoscale Physics · Physics 2017-03-28 Markus Ternes