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Terahertz two-dimensional coherent spectroscopy (THz-2DCS) is transforming our ability to probe, visualize, and control quantum materials far from equilibrium. This emerging technique brings multi-dimensional resolution to the ultrafast…

Superconductivity · Physics 2026-02-09 Chuankun Huang , Martin Mootz , Liang Luo , Ilias E. Perakis , Jigang Wang

Recent advances in techniques for generating quantum light have stimulated research on novel spectroscopic measurements using quantum entangled photons. One such spectroscopy technique utilizes non-classical correlations among entangled…

Chemical Physics · Physics 2021-07-28 Yuta Fujihashi , Akihito Ishizaki

Two-dimensional electronic spectroscopy (2DES) is one of the most powerful spectroscopic techniques, capable of attaining a nearly complete picture of a quantum system including its couplings, quantum coherence properties and its real-time…

Conformational dynamics of biomolecules are of fundamental importance for their function. Single-molecule F\"orster Resonance Energy Transfer (smFRET) is a powerful approach to inform on the structure and the dynamics of labeled molecules.…

We present a new physical model resolving a long-standing mystery of the power-law distributions of the blinking times in single colloidal quantum dot fluorescence. The model considers the non-radiative relaxation of the exciton through…

Statistical Mechanics · Physics 2009-11-16 Pavel A. Frantsuzov , Sandor Volkan-Kacso , Bolizsar Janko

Resonance fluorescence of a two-level emitter displays persistently anti-bunching irrespective of the excitation intensity, but inherits the driving laser's linewidth under weak monochromatic excitation. These properties are commonly…

Single molecule time traces reveal the time evolution of unsynchronized kinetic systems. Especially single molecule F\"orster resonance energy transfer (smFRET) provides access to enzymatically important timescales, combined with molecular…

Quantitative Methods · Quantitative Biology 2018-01-17 Sonja Schmid , Thorsten Hugel

The Hanbury Brown-Twiss (HBT) effect, discovered in the 1950s and further developed in the 1960s, was originally used to estimate stellar angular diameters through intensity correlations measured by spatially separated detectors. Further…

Quantum-optical coherence tomography (QOCT) is an optical sectioning modality based on the quantum interference of photon pairs, obtained from a spontaneous parametric downconversion (SPDC) source. The promise of QOCT derives from two…

We present Full SMS, a multipurpose graphical user interface (GUI)-based software package for analysing single-molecule spectroscopy (SMS) data. SMS typically delivers multiparameter data -- such as fluorescence brightness, lifetime, and…

Biological Physics · Physics 2024-05-01 Joshua L. Botha , Bertus van Heerden , Tjaart P. J. Krüger

We present in this letter a scheme for optical interferometry. We utilize coherent-beam-stimulated two-mode squeezed light, which interacts with a phase shifter and is then squeezed again before detection. Our theoretical device has the…

Quantum Physics · Physics 2015-06-16 William N. Plick , Jonathan P. Dowling , G. S. Agarwal

Two-photon interference underlies the functioning of many quantum photonics devices. It also serves as the prominent tool for testing the indistinguishability of distinct photons. However, as their time-spectral profile becomes more…

The subtle and fundamental issue of indistinguishability and interference between independent pathways to the same target state is examined in the context of coherent control of atomic and molecular processes, with emphasis placed on…

Quantum Physics · Physics 2015-05-18 Jiangbin Gong , Paul Brumer

Single-photon detectors have achieved impressive performance, and have led to a number of new scientific discoveries and technological applications. Existing models of photodetectors are semiclassical in that the field-matter interaction is…

Optics · Physics 2018-03-28 Steve M. Young , Mohan Sarovar , François Léonard

We investigate the intensity correlation properties of single photons emitted from an optically excited single semiconductor quantum dot. The second order temporal coherence function of the photons emitted at various wavelengths is measured…

Strongly Correlated Electrons · Physics 2009-11-07 D. V. Regelman , U. Mizrahi , D. Gershoni , E. Ehrenfreund , W. V. Schoenfeld , P. M. Petroff

A new approach to measure the second order correlation function $g^{(2)}$ and the coherence time was investigated. The $g^{(2)}$ was calculated from the photon pair time interval distribution by direct numerical self-convolution with the…

Optics · Physics 2016-04-20 Chen-How Huang , Yung-Hsiang Wen , Yi-Wei Liu

In this chapter we will discuss the technology and experimental techniques to realize quantum dot (QD) single photon sources combining high outcoupling efficiencies and highest degrees of non-postselected photon indistinguishability. The…

Quantum Physics · Physics 2015-02-03 C. Schneider , P. Gold , C. -Y. Lu , S. Höfling , J. -W. Pan , M. Kamp

Unlike one-photon (first order) intensity correlation, two-photon (second order) intensity correlation is known to be impossible to achieve by any classical means. Over the last several decades, such quantum features have been intensively…

Quantum Physics · Physics 2023-09-22 Byoung S. Ham

The slowdown of optical pulses due to quantum-coherence effects is investigated theoretically for an "active material" consisting of InGaAs-based double quantum-dot molecules. These are designed to exhibit a long lived coherence between two…

Mesoscale and Nanoscale Physics · Physics 2014-04-11 Stephan Michael , Weng W. Chow , Hans Christian Schneider

Ultrafast single-photon pulses with tailored time-frequency properties are highly attractive for quantum information science, offering high-dimensional encoding and compatibility with integrated optics platforms. However, accurate…

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