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The transition-metal tetrachalcogenides are a model system to explore the conjunction of correlated electronic states such as charge density waves (CDW), with topological phases of matter. Understanding the connection between these phases…

Transition metal dichalcogenides (TMDs) are quasi-two-dimensional layered compounds exhibiting strongly competing charge-density wave (CDW) and superconducting (SC) order parameters (OPs). The weak van der Waals interlayer bonding between…

Superconductivity · Physics 2015-05-26 Richard A. Klemm

The intercalated layered nitride $\beta$-HfNCl has attracted much attention due to the high superconducting transition temperature up to 25.5 K. Electrons can be introduced into $\beta$-$M$NCl ($M$=Zr and Hf) through alkali-metals…

Superconductivity · Physics 2013-05-30 Guojun Ye , Jianjun Ying , Yajun Yan , Xigang Luo , Peng Cheng , Ziji Xiang , Aifeng Wang , Xianhui Chen

Transition metal dichalcogenides exhibit rich phase diagrams dominated by the interplay of superconductivity and charge density waves, which often result in anomalies in the electric transport properties. Here, we employ the ionic gating…

Mesoscale and Nanoscale Physics · Physics 2022-06-28 Erik Piatti , Jessica Montagna Bozzone , Dario Daghero

The layered transition metal dichalcogenides host a rich collection of charge density wave (CDW) phases in which both the conduction electrons and the atomic structure display translational symmetry breaking. Manipulating these complex…

Mesoscale and Nanoscale Physics · Physics 2016-11-15 A. W. Tsen , R. Hovden , D. Z. Wang , Y. D. Kim , J. Okamoto , K. A. Spoth , Y. Liu , W. J. Lu , Y. P. Sun , J. Hone , L. F. Kourkoutis , P. Kim , A. N. Pasupathy

Introducing foreign ions, atoms, or molecules into emerging functional materials is crucial for manipulating material physical properties and innovating device applications. The intercalation of emerging new materials can induce multiple…

Applied Physics · Physics 2024-10-15 Xin He , Hua Wang , Jian Sun , Xixiang Zhang , Kai Chang , Fei Xue

Phase engineering strategies in two-dimensional transition metal dichalcogenides (2D-TMDs) have garnered significant attention due to their potential applications in electronics, optoelectronics, and energy storage. Various methods,…

Due to their unique two-dimensional nature, charge carriers in semiconducting transition metal dichalcogenides (TMDs) exhibit strong unscreened Coulomb interactions and sensitivity to defects and impurities. The versatility of van der Waals…

As superconductors are thinned down to the 2D limit, their critical temperature $T_c$ typically decreases. Here we report the opposite behavior, a substantial enhancement of $T_c$ with decreasing thickness, in 2D crystalline superconductor…

Common substitutional isovalent semiconductor alloys usually form disordered metastable phases with positive excess formation enthalpies ({\Delta}H). In contrast, monolayer alloys of transition metal dichalcogenides (TMDs) MX2 (M = Mo, W; X…

Materials Science · Physics 2017-10-17 Ji-Hui Yang , Boris I. Yakobson

Superconducting layered transition metal dichalcogenides (TMDs) stand out among other superconductors due to the tunable nature of the superconducting transition, coexistence with other collective electronic excitations (charge density…

Van der Waals materials enable the construction of atomically sharp interfaces between compounds with distinct crystal and electronic properties. This is dramatically exploited in moir\'e systems, where a lattice mismatch or twist between…

Low-dimensional electron systems, as realized naturally in graphene or created artificially at the interfaces of heterostructures, exhibit a variety of fascinating quantum phenomena with great prospects for future applications. Once…

Strongly Correlated Electrons · Physics 2016-08-03 T. Ritschel , J. Trinckauf , K. Koepernik , B. Büchner , M. v. Zimmermann , H. Berger , Y. I. Joe , P. Abbamonte , J. Geck

Bi2Se3 and Bi2Te3 are layered compounds of technological importance, being excellent thermoelectric materials as well as topological insulators. We report density functional theory calculations of the atomic, electronic and thermoelectric…

Materials Science · Physics 2013-08-08 Xin Luo , Michael B. Sullivan , Su Ying Quek

In the recently synthesized Li$_x$(NH$_2$)$_y$(NH$_3$)$_z$Fe$_2$Se$_2$ family of iron chalcogenides a molecular spacer consisting of lithium ions, lithium amide and ammonia separates layers of FeSe. It has been shown that upon variation of…

Superconductivity · Physics 2015-01-16 Daniel Guterding , Harald O. Jeschke , P. J. Hirschfeld , Roser Valenti

Thermal boundary conductance (TBC) at dissimilar interfaces imposes a fundamental limit on electronic device performance, yet predicting and understanding heat transport across realistic, disordered boundaries remains elusive. Here, we…

Correlated electron systems that host multiple electronic orders offer routes to multifunctional quantum materials, but strong competition between these orders often prevents their coexistence. Here we show that nanoscale, metastable…

Van der Waals hosts intercalated with transition metal (TM) ions exhibit a range of magnetic properties strongly influenced by the structural order of the intercalants. However, predictive computational models for the intercalant ordering…

Materials Science · Physics 2024-10-28 Isaac M. Craig , B. Junsuh Kim , David T. Limmer , D. Kwabena Bediako , Sinéad M. Griffin

We investigate the single crystals of Ni$_{0.19}$NbSe$_2$, revealing that Ni intercalation profoundly alters the physical properties of NbSe$_2$. Magnetic measurements clearly show that the system is magnetically frustrated with…

The beta-modification of FeSe, which has an anti-PbO type structure, achieves superconductivity at 8 K without external doping or pressure and exhibits a nematic phase, which has been crucial for studies of unconventional pairing…

Superconductivity · Physics 2025-03-04 Nadine Lammer , Dominik Werhahn , Dirk Johrendt