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Vibrational properties of solids are key to determining stability, response and functionality. However, they are challenging to computationally predict at Ab-Initio accuracy, even for elemental systems. Ab-Initio methods for modeling atomic…

Materials Science · Physics 2024-06-25 Mgcini Keith Phuthi , Yang Huang , Michael Widom , Venkatasubramanian Viswanathan

The development of machine learning models has led to an abundance of datasets containing quantum mechanical (QM) calculations for molecular and material systems. However, traditional training methods for machine learning models are unable…

Machine-learning interatomic potential (MLIP) has been of growing interest as a useful method to describe the energetics of systems of interest. In the present study, we examine the accuracy of linearized pairwise MLIPs and…

Materials Science · Physics 2018-08-01 Akira Takahashi , Atsuto Seko , Isao Tanaka

As with many parts of the natural sciences, machine learning interatomic potentials (MLIPs) are revolutionizing the modeling of molecular crystals. However, challenges remain for the accurate and efficient calculation of sublimation…

Computational Physics · Physics 2025-09-03 Flaviano Della Pia , Benjamin X. Shi , Venkat Kapil , Andrea Zen , Dario Alfè , Angelos Michaelides

Atomistic modeling of solid-solid battery interfaces is essential for understanding electro-chemo-mechanical coupling, but the complex interfacial chemistry and heterogeneous environments pose major challenges for quantum-accurate,…

Materials Science · Physics 2026-01-27 Xiaoqing Liu , Xinyu Yu , Yangshuai Wang , Zhe-Tao Sun , Zedong Luo , Kehan Zeng , Teng Zhao , Shou-Hang Bo , Zhenli Xu

Machine learning interatomic potentials (MLIPs) have proven to be wildly useful for molecular dynamics simulations, powering countless drug and materials discovery applications. However, MLIPs face two primary bottlenecks preventing them…

Machine Learning · Computer Science 2026-01-30 Kevin Han , Haolin Cong , Bowen Deng , Amir Barati Farimani

Artificial intelligence techniques have achieved strong performance in classifying Windows Portable Executable (PE) malware, but their reliability often degrades under dataset shifts, leading to misclassifications with severe security…

Cryptography and Security · Computer Science 2025-12-23 Rahul Yumlembam , Biju Issac , Seibu Mary Jacob

Machine learning interatomic potentials (MLIPs) have become a workhorse of modern atomistic simulations, and recently published universal MLIPs, pre-trained on large datasets, have demonstrated remarkable accuracy and generalizability.…

Materials Science · Physics 2024-12-04 Juno Nam , Jiayu Peng , Rafael Gómez-Bombarelli

Machine learning interatomic potentials (ML-IAPs) enable quantum-accurate, classical molecular dynamics simulations of large systems, beyond reach of density functional theory (DFT). Yet, their efficiency and ability to predict systems…

Materials Science · Physics 2023-11-07 Lei Zhang , Gábor Csányi , Erik van der Giessen , Francesco Maresca

Multivalent batteries are an energy storage technology with the potential to surpass lithium-ion batteries, however their performance has been limited by the low voltages and poor solid-state ionic mobility of available cathodes. A…

Materials Science · Physics 2022-04-13 Ann Rutt , Jimmy-Xuan Shen , Matthew Horton , Jiyoon Kim , Jerry Lin , Kristin A. Persson

Machine Learning Inter-atomic Potentials (MLIPs) have become a common tool in use by computational chemists due to their combination of accuracy and speed. Yet, it is still not clear how well these tools behave at or near transitions states…

Chemical Physics · Physics 2022-11-15 Aaron Philip , Guoqing Zhou , Benjamin Nebgen

Uranium mononitride (UN) is a promising accident-tolerant fuel because of its high fissile density and high thermal conductivity. In this study, we developed the first machine learning interatomic potentials for reliable atomic-scale…

Understanding the mechanical properties of solid-state materials at the atomic scale is crucial for developing novel materials. For example, amorphous LiSi alloys are attractive anode materials for solid-state Li-ion batteries but face…

Disordered Systems and Neural Networks · Physics 2024-02-15 Zixiong Wei , Nongnuch Artrith

Active learning for machine-learning interatomic potentials (MLIPs) must address several challenges to be practical: scaling to large candidate pools, leveraging energy-force supervision, and maintaining robustness when candidate pools are…

Machine Learning · Computer Science 2026-05-18 Eszter Varga-Umbrich , Zachary Weller-Davies , Paul Duckworth , Jules Tilly , Olivier Peltre , Shikha Surana

Graph neural network universal interatomic potentials (GNN-UIPs) have demonstrated remarkable generalization and transfer capabilities in material discovery and property prediction. These models can accelerate molecular dynamics (MD)…

Distributed, Parallel, and Cluster Computing · Computer Science 2025-07-25 Yuanchang Zhou , Siyu Hu , Chen Wang , Lin-Wang Wang , Guangming Tan , Weile Jia

A machine learned interatomic potential for AlN was developed using the ultra-fast force field (UF3) methodology. A strong agreement with density functional theory calculations in predicting key structural and mechanical properties,…

Materials Science · Physics 2025-11-12 Nicholas Taormina , Emir Bilgili , Jason Gibson , Richard Hennig , Simon Phillpot , Youping Chen

Understanding ion adsorption at electrified metal-electrolyte interfaces is essential for accurate modeling of electrochemical systems. Here, we systematically investigate the free energy profiles of Na$^+$, Cl$^-$, and F$^-$ ions at the…

Chemical Physics · Physics 2026-02-27 Fabrice Roncoroni , Abrar Faiyad , Yichen Li , Tao Ye , Ashlie Martini , David Prendergast

High-entropy alloys (HEAs) have attracted increasing attention due to their unique structural and functional properties. In the study of HEAs, thermodynamic properties and phase stability play a crucial role, making phase diagram…

Materials Science · Physics 2025-12-01 Siya Zhu , Doguhan Sariturk , Raymundo Arroyave

Accurate prediction of the Remaining Useful Life (RUL) is essential for enabling timely maintenance of lithium-ion batteries, impacting the operational efficiency of electric applications that rely on them. This paper proposes a RUL…

Machine Learning · Computer Science 2026-02-03 Khoa Tran , Tri Le , Bao Huynh , Hung-Cuong Trinh , Vy-Rin Nguyen , T. Nguyen-Thoi , Vin Nguyen-Thai

The development of machine learning models for electrocatalysts requires a broad set of training data to enable their use across a wide variety of materials. One class of materials that currently lacks sufficient training data is oxides,…

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