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In the near future, material and drug design may be aided by quantum computer assisted simulations. These have the potential to target chemical systems intractable by the most powerful classical computers. However, the resources offered by…

We present an embedding scheme for periodic systems that facilitates the treatment of the physically important part (here the unit cell) with advanced electronic-structure methods, that are computationally too expensive for periodic…

Materials Science · Physics 2016-04-08 Wael Chibani , Xinguo Ren , Matthias Scheffler , Patrick Rinke

Strongly correlated quantum impurity problems appear in a wide variety of contexts ranging from nanoscience and surface physics to material science and the theory of strongly correlated lattice models, where they appear as auxiliary systems…

Strongly Correlated Electrons · Physics 2013-02-19 Hartmut Hafermann , Philipp Werner , Emanuel Gull

We investigate the ground-state properties of the Anderson single impurity model (finite Coulomb impurity repulsion) with the Coupled Cluster Method. We consider different CCM reference states and approximation schemes and make comparison…

Strongly Correlated Electrons · Physics 2009-06-26 Jin-Jun Liang , Clive Emary , Tobias Brandes

Quantum computing presents a promising path toward precise quantum chemical simulations, particularly for systems that challenge classical methods. This work investigates the performance of the Variational Quantum Eigensolver (VQE) in…

Quantum Physics · Physics 2025-10-28 Zakaria Boutakka , Nouhaila Innan , Muhammed Shafique , Mohamed Bennai , Z. Sakhi

We conducted a thorough evaluation of various state-of-the-art strategies to prepare the ground state wavefunction of a system on a quantum computer, specifically within the framework of variational quantum eigensolver (VQE). Despite the…

Quantum Physics · Physics 2024-03-05 M. R. Nirmal , Sharma S. R. K. C. Yamijala , Kalpak Ghosh , Sumit Kumar , Manoj Nambiar

Variational quantum eigensolver (VQE) solves the ground state problem of a given Hamiltonian by finding the parameters of a quantum circuit ansatz that minimizes the Hamiltonian expectation value. Among possible quantum circuit ans\"{a}tze,…

Quantum Physics · Physics 2024-01-31 Chae-Yeun Park

We introduce a representation of electron operators as a product of a spin-carry ing fermion and of a phase variable dual to the total charge (slave quantum rotor). Based on this representation, a new method is proposed for solving…

Strongly Correlated Electrons · Physics 2009-11-07 Serge Florens , Antoine Georges

Neural quantum states (NQS) have emerged as a promising approach to solve second-quantized Hamiltonians, because of their scalability and flexibility. In this work, we design and benchmark an NQS impurity solver for the quantum embedding…

Strongly Correlated Electrons · Physics 2026-03-16 Yinzhanghao Zhou , Tsung-Han Lee , Ao Chen , Nicola Lanatà , Hong Guo

We implement an efficient numerical method to calculate response functions of complex impurities based on the Density Matrix Renormalization Group (DMRG) and use it as the impurity-solver of the Dynamical Mean Field Theory (DMFT). This…

Strongly Correlated Electrons · Physics 2017-11-27 Y. Núñez Fernández , K. Hallberg

We generalized the recently introduced new impurity solver based on the diagrammatic expansion around the atomic limit and Quantum Monte Carlo summation of the diagrams. We present generalization to the cluster of impurities, which is at…

Strongly Correlated Electrons · Physics 2009-11-11 Kristjan Haule

We review two analytical approaches in Dynamical Mean-Field Theory (DMFT) based on a perturbation theory expansion over the electron hopping to and from the self consistent environment. In the first approach the effective single impurity…

Strongly Correlated Electrons · Physics 2007-05-23 I. V. Stasyuk , A. M. Shvaika

We propose a divide-and-conquer method for the quantum-classical hybrid algorithm to solve larger problems with small-scale quantum computers. Specifically, we concatenate a variational quantum eigensolver (VQE) with a reduction in the…

Quantum Physics · Physics 2022-01-26 Keisuke Fujii , Kaoru Mizuta , Hiroshi Ueda , Kosuke Mitarai , Wataru Mizukami , Yuya O. Nakagawa

Dynamical and variational frameworks have long been viewed as distinct paradigms. In particular, in quantum embedding (QE) frameworks, dynamical mean-field theory (DMFT) captures nonperturbative dynamical correlations through a…

Strongly Correlated Electrons · Physics 2026-04-03 Samuele Giuli , Tsung-Han Lee , Yong-Xin Yao , Gabriel Kotliar , Andrei E. Ruckenstein , Olivier Gingras , Nicola Lanatà

Solving the single-impurity Anderson model (SIAM) is a basic problem of solid state physics. The SIAM model is very important, at present it is also used for systems with quantum impurities, e.g. semiconductor quantum dots and molecular…

Strongly Correlated Electrons · Physics 2023-07-19 Grzegorz Górski , Jerzy Mizia , Krzysztof Kucab

The variational quantum eigensolver (VQE) is a hybrid quantum-classical algorithm designed for current and near-term quantum devices. Despite its initial success, there is a lack of understanding involving several of its key aspects. There…

Quantum Physics · Physics 2023-03-22 Manpreet Singh Jattana , Fengping Jin , Hans De Raedt , Kristel Michielsen

We investigate the dynamical mean-field theory (DMFT) from a quantum chemical perspective. Dynamical mean-field theory offers a formalism to extend quantum chemical methods for finite systems to infinite periodic problems within a local…

Strongly Correlated Electrons · Physics 2016-11-15 Dominika Zgid , Garnet Kin-Lic Chan

We use the time dependent variational matrix product state (tVMPS) approach to investigate the dynamical properties of the single impurity Anderson model (SIAM). Under the Jordan-Wigner transformation, the SIAM is reformulated into two…

Strongly Correlated Electrons · Physics 2010-02-04 Lei Wang , Jia-Ning Zhuang , Xi Dai , X. C. Xie

The variational quantum eigensolver (or VQE) uses the variational principle to compute the ground state energy of a Hamiltonian, a problem that is central to quantum chemistry and condensed matter physics. Conventional computing methods are…

This manuscript presents the Quantum Finite Element Method (Q-FEM) developed for use in noisy intermediate-scale quantum (NISQ) computers and employs the variational quantum linear solver (VQLS) algorithm. The proposed method leverages the…

Quantum Physics · Physics 2025-04-01 Abhishek Arora , Benjamin M. Ward , Caglar Oskay