Related papers: Rotational Memory Function of SPC/E water
Liquid water is fundamentally important, and its accurate computer simulation has been the driving force for myriad methodological developments. Ab initio molecular dynamics with forces obtained from density functional theory (DFT) is now a…
We consider the correlations and the hydrodynamic description of random walkers with a general finite memory moving on a $d$ dimensional hypercubic lattice. We derive a drift-diffusion equation and identify a memory-dependent critical…
The complementarity of the liquid and plasma descriptions of the classical one-component plasma (OCP) is explored by studying wavevector and frequency dependent dynamical quantities: the dynamical structure factor (DSF), and the dynamic…
A probability density function describing the angular evolution of a fixed-length atom-atom vector as a L\'{e}vy rotor is derived containing just two dynamical parameters: the L\'{e}vy parameter $\alpha$ and a rotational time constant…
In this contribution, we compute the $^1$H nuclear magnetic resonance (NMR) relaxation rate of liquid water at ambient conditions. We are using structural and dynamical information from Coupled Cluster Molecular Dynamics (CCMD) trajectories…
The Debye-Stokes-Einstein (DSE) model of rotational diffusion predicts that the rotational correlation times $\tau_{l}$ vary as $[l(l+1)]^{-1}$, where $l$ is the rank of the orientational correlation function (given in terms of the Legendre…
Over the last decade, an increasing body of evidence has emerged, supporting the existence of a metastable liquid-liquid critical point in supercooled water, whereby two distinct liquid phases of different densities coexist. Analysing long…
Physical arguments and comparisons with published experimental data suggest that in simple liquids: i) single-molecule-scale viscous forces are produced by temperature-dependent London dispersion forces, ii) viscosity decay with increasing…
Employing a simple ideal magnetohydrodynamic model in spherical geometry,we show that the presence of either rotation or finite magnetic helicity is sufficient to induce dynamical reversals of the magnetic dipole moment. The statistical…
At temperatures below 1 K, the capacitance of a glass sample changes due to the application of a DC field in accordance with A. Burins dipole gap theory. However, we now report that below 20 mK, during the first sweep cycle of the DC…
Memory can remarkably modify the collective behaviors of active particles. We show that in a micellar fluid, Quincke particles driven by a square-wave electric field exhibit a frequency-dependent memory. Upon increasing the frequency, a…
We study the collective dissipative dynamics of dipoles modeled as harmonic oscillators coupled to 1-D electromagnetic reservoirs. The bosonic nature of the dipole oscillators as well as the reservoir modes allows an exact numerical…
We expand on a recent study of a lattice model of interacting particles [Phys. Rev. Lett. 111, 110601 (2013)]. The adsorption isotherm and equilibrium fluctuations in particle number are discussed as a function of the interaction. Their…
Contemporary three-dimensional physics-based simulations of the solar convection zone disagree with observations. They feature differential rotation substantially different from the true rotation inferred by solar helioseismology and…
Here we characterize the motility of athermal swimming droplets within the framework of active rotational diffusion. Just like active colloids, their trajectories can be modeled with a constant velocity $V$ and a slow angular diffusion, but…
While Landauer's Principle sets a lower bound for the work required for a computation, that work is recoverable for efficient computations. However, practical physical computers, such as modern digital computers or biochemical systems, are…
Spin dynamics of a single electron and an exciton confined in CdTe/ZnTe quantum dot is investigated by polarization-resolved correlation spectroscopy. Spin memory effects extending over at least a few tens of nanoseconds have been directly…
A diagrammatic kinetic theory of density fluctuations in simple dense liquids at long times, described in the preceding paper, is applied to a high density Lennard-Jones liquid to calculate various equilibrium time correlation functions.…
The molecular theory of Rayleigh light scattering in dense isotropic polar fluids is reconsidered by suitably adapting local field concepts of electrostatics to propagating electromagnetic waves, hence accounting for both the rotational and…
We propose a dynamic structure of coupled dynamic molecular strings for supercooled small polar molecule liquids and accordingly we obtain the Hamiltonian of the rotational degrees of freedom of the system. From the Hamiltonian, the…